Fabrication of a Microcavity Prepared by Remote Epitaxy over Monolayer Molybdenum Disulfide

Kim, Yeonhoo; Watt, John; Ma, Xuedan; Ahmed, Towfiq; Kim, Suhyun; Kang, Kibum; Luk, Ting S.; Hong, Young Joon; Yoo, Jinkyoung

doi:10.1021/acsnano.1c08779

Title: Fabrication of a Microcavity Prepared by Remote Epitaxy over Monolayer Molybdenum Disulfide

Journal Article · 08 February 2022 · ACS Nano

DOI: https://doi.org/10.1021/acsnano.1c08779 · OSTI ID:1865029

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^[1]; Kim, Suhyun ^[3];

^[3]; Luk, Ting S. ^[4];

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Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)
Argonne National Laboratory (ANL), Argonne, IL (United States)
Korea Advanced Inst. Science and Technology (KAIST), Daejeon (Korea, Republic of)
Sandia National Laboratory (SNL-NM), Albuquerque, NM (United States)
Sejong Univ., Seoul (Korea, Republic of)

We report advances in epitaxy have enabled the preparation of high-quality material architectures consisting of incommensurate components. Remote epitaxy based on lattice transparency of atomically thin graphene has been intensively studied for cost-effective advanced device manufacturing and heterostructure formation. However, remote epitaxy on nongraphene two-dimensional (2D) materials has rarely been studied even though it has a broad and immediate impact on various disciplines, such as many-body physics and the design of advanced devices. Herein, we report remote epitaxy of ZnO on monolayer MoS₂ and the realization of a whispering-gallery-mode (WGM) cavity composed of a single crystalline ZnO nanorod and monolayer MoS₂. Cross-sectional transmission electron microscopy and first-principles calculations revealed that the nongraphene 2D material interacted with overgrown and substrate layers and also exhibited lattice transparency. The WGM cavity embedding monolayer MoS₂ showed enhanced luminescence of MoS₂ and multimodal emission.

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Research Organization:: Los Alamos National Laboratory (LANL), Los Alamos, NM (United States); Argonne National Laboratory (ANL), Argonne, IL (United States); Sandia National Laboratories (SNL-NM), Albuquerque, NM (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES); USDOE Laboratory Directed Research and Development (LDRD) Program

Grant/Contract Number:: 89233218CNA000001; NA0003525; AC02-06CH11357

OSTI ID:: 1865029

Report Number(s):: LA-UR-21-28942

Journal Information:: ACS Nano, Journal Name: ACS Nano Journal Issue: 2 Vol. 16; ISSN 1936-0851

Publisher:: American Chemical Society (ACS)Copyright Statement

Country of Publication:: United States

Language:: English

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36 MATERIALS SCIENCE
microcavity
polarity inversion
remote epitaxy
transition metal dichalcogenides
two-dimensional material
whispering-gallery-mode

Title: Fabrication of a Microcavity Prepared by Remote Epitaxy over Monolayer Molybdenum Disulfide

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