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Title: Sensitive search for near-symmetric and super-asymmetric fusion-fission of the superheavy element Flerovium (Z=114)

Journal Article · · Physics Letters. B
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  1. The Australian National University, Canberra, ACT (Australia)
  2. Variable Energy Cyclotron Centre, Kolkata (India); Homi Bhabha National Institute, Mumbai (India)
  3. The Australian National University, Canberra, ACT (Australia); Michigan State Univ., East Lansing, MI (United States)
  4. GSI-Helmholtzzentrum fur Schwerionenforschung, Darmstadt (Germany)
  5. GSI-Helmholtzzentrum fur Schwerionenforschung, Darmstadt (Germany); Helmholz Institute Mainz (Germany); Johannes Gutenberg Univ., Mainz (Germany)
  6. GSI-Helmholtzzentrum fur Schwerionenforschung, Darmstadt (Germany); Helmholz Institute Mainz (Germany)
  7. Helmholz Institute Mainz (Germany)
  8. GSI-Helmholtzzentrum fur Schwerionenforschung, Darmstadt (Germany); Johannes Gutenberg Univ., Mainz (Germany)
  9. Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
  10. Helmholz Institute Mainz (Germany); Johannes Gutenberg Univ., Mainz (Germany)
  11. Johannes Gutenberg Univ., Mainz (Germany)

Measurements of mass and angular distributions have been made for fission-like outcomes in reactions forming isotopes of flerovium (Z=114), using 48Ca, 50Ti, and 54Cr projectiles. The dominant fast quasifission process, which masks the presence of fusion-fission, has minimum yield at the most backward angles, where the sensitivity to fusion-fission is thus highest. In fitting the backward angle mass spectra, only weak evidence for a component of super-asymmetric fission was found, but a near-symmetric fission component was consistently required for the 48Ca + 244Pu reaction, giving upper limit to the fusion probabilities PCN of ~10-2, ~5 times lower than previous results. PCN for the 50Ti reaction was lower than 48Ca, whilst no evidence of fusion-fission was found for the 54Cr reaction.

Research Organization:
Lawrence Livermore National Laboratory (LLNL), Livermore, CA (United States)
Sponsoring Organization:
USDOE National Nuclear Security Administration (NNSA)
Grant/Contract Number:
AC52-07NA27344
OSTI ID:
1860837
Report Number(s):
LLNL-JRNL-832608; 1050286
Journal Information:
Physics Letters. B, Journal Name: Physics Letters. B Journal Issue: N/A Vol. 820; ISSN 0370-2693
Publisher:
ElsevierCopyright Statement
Country of Publication:
United States
Language:
English

References (62)

Some remarks on the error analysis in the case of poor statistics journal February 1984
Competition between complete fusion and quasi-fission in dinuclear system journal September 1997
Nuclear masses and deformations journal June 1966
Closed shells for Z > 82 and N > 126 in a diffuse potential well journal September 1966
Shell effects in nuclear masses and deformation energies journal April 1967
Experiments to produce isotopes of superheavy elements with atomic numbers 114–116 in 48Ca ion reactions journal January 1978
Towards a better parametrisation of Skyrme-like effective forces: A critical study of the SkM force journal September 1982
Quasi-fission — The mass-drift mode in heavy-ion reactions journal July 1985
Shell effects in fission and quasi-fission of heavy and superheavy nuclei journal April 2004
Actinide targets for the synthesis of super-heavy elements journal December 2015
Chemical studies of elements with Z≥ 104 in liquid phase journal December 2015
Fusion and fission of heavy and superheavy nuclei (experiment) journal December 2015
Chemical studies of elements with Z⩾ 104 in gas phase journal December 2015
Pre-scission model predictions of fission fragment mass distributions for super-heavy elements journal December 2017
Influence of entrance-channel magicity and isospin on quasi-fission journal April 2012
Zeptosecond contact times for element Z=120 synthesis journal September 2020
Experimental studies of the competition between fusion and quasifission in the formation of heavy and superheavy nuclei journal May 2021
Advances in the Production and Chemistry of the Heaviest Elements journal October 2012
The limits of nuclear mass and charge journal June 2018
The periodic table and the physics that drives it journal June 2020
Heaviest nuclei from 48 Ca-induced reactions journal March 2007
Synthetic Paths to the Heaviest Elements journal March 2013
Effect of the doubly magic shell closures in Sn 132 and Pb 208 on the mass distributions of fission fragments of superheavy nuclei journal January 2020
Efficient method for estimation of fission fragment yields of r -process nuclei journal June 2020
Angular distributions in heavy-ion-induced fission journal July 1985
Fission and quasifission in U-induced reactions journal July 1987
Conclusive evidence for the influence of nuclear orientation on quasifission journal March 1996
Fission barriers of superheavy nuclei journal March 2002
Synthesis of the isotopes of elements 118 and 116 in the Cf 249 and Cm 245 + Ca 48 fusion reactions journal October 2006
Measurement of the fusion probability P CN for the reaction of Ti 50 with Pb 208 journal November 2007
Entrance channel dependence of quasifission in reactions forming Th 220 journal March 2008
Effects of nuclear orientation on the mass distribution of fission fragments in the reaction of S 36 + U 238 journal June 2008
Fission and quasifission modes in heavy-ion-induced reactions leading to the formation of Hs * journal June 2011
Fusion probabilities in the reactions 40 , 48 Ca+ 238 U at energies around the Coulomb barrier journal September 2012
Measurement of the fusion probability, P CN , for hot fusion reactions journal July 2013
Mapping quasifission characteristics and timescales in heavy element formation reactions journal November 2013
Shell effects in damped collisions of Sr 88 with Yb 176 at the Coulomb barrier energy journal January 2014
Description of induced nuclear fission with Skyrme energy functionals. II. Finite temperature effects journal March 2015
Exploring quasifission characteristics for S 34 + Th 232 forming Sg 266 journal February 2016
Fusion and quasifission dynamics in the reactions Ca 48 + Bk 249 and Ti 50 + Bk 249 using a time-dependent Hartree-Fock approach journal August 2016
Fission and quasifission of composite systems with Z = 108 − 120 : Transition from heavy-ion reactions involving S and Ca to Ti and Ni ions journal November 2016
Fusion and quasifission studies for the Ca 40 + W 186 , Os 192 reactions journal September 2017
Sub-barrier quasifission in heavy element formation reactions with deformed actinide target nuclei journal February 2018
α decay and cluster radioactivity of nuclei of interest to the synthesis of Z = 119 , 120 isotopes journal April 2018
Cluster radioactivity in superheavy nuclei journal October 2018
Fission and quasifission of the composite system Z = 114 formed in heavy-ion reactions at energies near the Coulomb barrier journal January 2019
Cluster radioactivity of Og 176 118 294 journal April 2019
Fission Barriers of Compound Superheavy Nuclei journal May 2009
Synthesis of a New Element with Atomic Number Z = 117 journal April 2010
Production and Decay of Element 114: High Cross Sections and the New Nucleus Hs 277 journal June 2010
Predominant Time Scales in Fission Processes in Reactions of S, Ti and Ni with W: Zeptosecond versus Attosecond journal February 2011
Heavy-Particle Radioactivity of Superheavy Nuclei journal August 2011
Production and Decay of the Heaviest Nuclei 1 293 , 294 17 and 1 294 18 journal October 2012
Interplay between Quantum Shells and Orientation in Quasifission journal October 2014
Evidence for the Role of Proton Shell Closure in Quasifission Reactions from X-Ray Fluorescence of Mass-Identified Fragments journal November 2017
Attempts to Produce Superheavy Elements by Fusion of Ca 48 with Cm 248 in the Bombarding Energy Range of 4.5-5.2 MeV/u journal February 1985
Synthesis of Superheavy Nuclei in the 48 C a + 244 Pu Reaction journal October 1999
Colloquium : Superheavy elements: Oganesson and beyond journal January 2019
Nuclear ground-state properties from mean-field calculations journal September 2002
Experiment on the Synthesis of Element 113 in the Reaction 209 Bi( 70 Zn,n) 278 113 journal October 2004
On the discovery of new elements (IUPAC/IUPAP Provisional Report): Provisional Report of the 2017 Joint Working Group of IUPAC and IUPAP journal November 2018
Relativity in the electronic structure of the heaviest elements and its influence on periodicities in properties journal July 2019