Multiphase layered transition metal oxide positive electrodes for sodium ion batteries

Gabriel, Eric; Hou, Dewen; Lee, Eungje; Xiong, Hui

doi:10.1002/ese3.1128

Title: Multiphase layered transition metal oxide positive electrodes for sodium ion batteries

Journal Article · 29 March 2022 · Energy Science & Engineering

DOI: https://doi.org/10.1002/ese3.1128 · OSTI ID:1859813

^[1]; Hou, Dewen ^[1]; Lee, Eungje ^[2]; Xiong, Hui ^[1]

Micron School of Materials Science and Engineering Boise State University Boise Idaho USA
Argonne National Laboratory Chemical Sciences and Engineering Division Lemont Illinois USA

Abstract Multiphase layered transition metal oxides (LTMOs) for sodium ion battery (SIB) positive electrodes with phase interfaces across multiple length scales are a promising avenue toward practical, high‐performance SIBs. Combinations of phases can complement each other's strengths and mitigate their weaknesses if their interfaces are carefully controlled. Intra‐ and interparticle phase interactions from nanoscale to macroscale must be carefully tuned to generate distinct effects on properties and performance. An informed design strategy must be paired with relevant synthesis techniques and complemented by spatially resolved characterization tools to manipulate different length scales and interfaces. This review examines the design, synthesis, and characterization strategies that have been demonstrated for the preparation of heterogeneous, multiphasic LTMOs with phase interfaces across varied length scales.

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Research Organization:: Argonne National Laboratory (ANL), Argonne, IL (United States); Boise State Univ., ID (United States)

Sponsoring Organization:: USDOE; USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC02-06CH11357; SC0019121

OSTI ID:: 1859813

Journal Information:: Energy Science & Engineering, Journal Name: Energy Science & Engineering Journal Issue: 5 Vol. 10; ISSN 2050-0505

Publisher:: Wiley Blackwell (John Wiley & Sons)Copyright Statement

Country of Publication:: United Kingdom

Language:: English

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25 ENERGY STORAGE
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Title: Multiphase layered transition metal oxide positive electrodes for sodium ion batteries

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