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Title: Femtosecond photocurrents at the FeRh/Pt interface

Abstract

Femtosecond laser excitations of FeRh/Pt bilayers launch an ultrafast pulse of electric photocurrents in the Pt-layer and subsequently result in the emission of electromagnetic radiation in the THz spectral range. Analysis of the THz emission as a function of the polarization of the femtosecond laser pulse, external magnetic field, sample temperature, and sample orientation shows that the photocurrent can emerge due to vertical spin pumping and photo-induced inverse spin–orbit torque at the FeRh/Pt interface. Additionally, the vertical spin pumping from FeRh into Pt does not depend on the polarization of light and originates from ultrafast laser-induced demagnetization of the ferromagnetic phase of FeRh. The photo-induced inverse spin–orbit torque at the FeRh/Pt interface can be described in terms of a helicity-dependent effect of circularly polarized light on the magnetization of the ferromagnetic FeRh and the subsequent generation of a photocurrent.

Authors:
ORCiD logo [1];  [2];  [3];  [4];  [2];  [2];  [3]
  1. Univ. of California San Diego, La Jolla, CA (United States). Center for Memory and Recording Research; National Inst. of Technology, Andhra Pradesh (India)
  2. Radboud Univ., Nijmegen (Netherlands). Inst. for Molecules and Materials
  3. Univ. of California San Diego, La Jolla, CA (United States). Center for Memory and Recording Research
  4. Radboud Univ., Nijmegen (Netherlands). Inst. for Molecules and Materials; Lancaster Univ. (United Kingdom)
Publication Date:
Research Org.:
Univ. of California, San Diego, CA (United States)
Sponsoring Org.:
USDOE Office of Science (SC); European Research Council (ERC)
OSTI Identifier:
1852549
Alternate Identifier(s):
OSTI ID: 1671147
Grant/Contract Number:  
SC0018237; 713481; 856538; 852050
Resource Type:
Accepted Manuscript
Journal Name:
Applied Physics Letters
Additional Journal Information:
Journal Volume: 117; Journal Issue: 14; Journal ID: ISSN 0003-6951
Publisher:
American Institute of Physics (AIP)
Country of Publication:
United States
Language:
English
Subject:
71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS; Physics

Citation Formats

Medapalli, R., Li, G., Patel, Sheena K. K., Mikhaylovskiy, R. V., Rasing, Th., Kimel, A. V., and Fullerton, E. E. Femtosecond photocurrents at the FeRh/Pt interface. United States: N. p., 2020. Web. doi:10.1063/5.0026252.
Medapalli, R., Li, G., Patel, Sheena K. K., Mikhaylovskiy, R. V., Rasing, Th., Kimel, A. V., & Fullerton, E. E. Femtosecond photocurrents at the FeRh/Pt interface. United States. https://doi.org/10.1063/5.0026252
Medapalli, R., Li, G., Patel, Sheena K. K., Mikhaylovskiy, R. V., Rasing, Th., Kimel, A. V., and Fullerton, E. E. Mon . "Femtosecond photocurrents at the FeRh/Pt interface". United States. https://doi.org/10.1063/5.0026252. https://www.osti.gov/servlets/purl/1852549.
@article{osti_1852549,
title = {Femtosecond photocurrents at the FeRh/Pt interface},
author = {Medapalli, R. and Li, G. and Patel, Sheena K. K. and Mikhaylovskiy, R. V. and Rasing, Th. and Kimel, A. V. and Fullerton, E. E.},
abstractNote = {Femtosecond laser excitations of FeRh/Pt bilayers launch an ultrafast pulse of electric photocurrents in the Pt-layer and subsequently result in the emission of electromagnetic radiation in the THz spectral range. Analysis of the THz emission as a function of the polarization of the femtosecond laser pulse, external magnetic field, sample temperature, and sample orientation shows that the photocurrent can emerge due to vertical spin pumping and photo-induced inverse spin–orbit torque at the FeRh/Pt interface. Additionally, the vertical spin pumping from FeRh into Pt does not depend on the polarization of light and originates from ultrafast laser-induced demagnetization of the ferromagnetic phase of FeRh. The photo-induced inverse spin–orbit torque at the FeRh/Pt interface can be described in terms of a helicity-dependent effect of circularly polarized light on the magnetization of the ferromagnetic FeRh and the subsequent generation of a photocurrent.},
doi = {10.1063/5.0026252},
journal = {Applied Physics Letters},
number = 14,
volume = 117,
place = {United States},
year = {Mon Oct 05 00:00:00 EDT 2020},
month = {Mon Oct 05 00:00:00 EDT 2020}
}

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