Advanced Materials for Energy-Water Systems: The Central Role of Water/Solid Interfaces in Adsorption, Reactivity, and Transport

Barry, Edward; Burns, Raelyn; Chen, Wei; De Hoe, Guilhem X.; Montes De Oca, Joan Manuel; de Pablo, Juan J.; Dombrowski, James; Elam, Jeffrey W.; Felts, Alanna M.; Galli, Giulia; Hack, John; He, Qiming; He, Xiang; Hoenig, Eli; Iscen, Aysenur; Kash, Benjamin; Kung, Harold H.; Lewis, Nicholas H. C.; Liu, Chong; Ma, Xinyou; Mane, Anil; Martinson, Alex B. F.; Mulfort, Karen L.; Murphy, Julia; Mølhave, Kristian; Nealey, Paul; Qiao, Yijun; Rozyyev, Vepa; Schatz, George C.; Sibener, Steven J.; Talapin, Dmitri; Tiede, David M.; Tirrell, Matthew V.; Tokmakoff, Andrei; Voth, Gregory A.; Wang, Zhongyang; Ye, Zifan; Yesibolati, Murat; Zaluzec, Nestor J.; Darling, Seth B.

doi:10.1021/acs.chemrev.1c00069

Title: Advanced Materials for Energy-Water Systems: The Central Role of Water/Solid Interfaces in Adsorption, Reactivity, and Transport

Journal Article · 02 July 2021 · Chemical Reviews

DOI: https://doi.org/10.1021/acs.chemrev.1c00069 · OSTI ID:1845829

Barry, Edward ^[1]; Burns, Raelyn ^[1];

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^[2]; Dombrowski, James ^[3];

^[1]; Felts, Alanna M. ^[3];

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^[1]; Hoenig, Eli ^[2];

^[3]; Kash, Benjamin ^[4];

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Energy Frontier Research Centers (EFRC) (United States). Advanced Materials for Energy-Water Systems (AMEWS) Center; Argonne National Lab. (ANL), Lemont, IL (United States)
Energy Frontier Research Centers (EFRC) (United States). Advanced Materials for Energy-Water Systems (AMEWS) Center; Argonne National Lab. (ANL), Lemont, IL (United States); Univ. of Chicago, IL (United States)
Energy Frontier Research Centers (EFRC) (United States). Advanced Materials for Energy-Water Systems (AMEWS) Center; Argonne National Lab. (ANL), Lemont, IL (United States); Northwestern Univ., Evanston, IL (United States)
Univ. of Chicago, IL (United States)
Energy Frontier Research Centers (EFRC) (United States). Advanced Materials for Energy-Water Systems (AMEWS) Center; Argonne National Lab. (ANL), Lemont, IL (United States); Technical Univ. of Denmark, Lyngby (Denmark)

The structure, chemistry, and charge of interfaces between materials and aqueous fluids play a central role in determining properties and performance of numerous water systems. Sensors, membranes, sorbents, and heterogeneous catalysts almost uniformly rely on specific interactions between their surfaces and components dissolved or suspended in the water-and often the water molecules themselves-to detect and mitigate contaminants. Deleterious processes in these systems such as fouling, scaling (inorganic deposits), and corrosion are also governed by interfacial phenomena. Despite the importance of these interfaces, much remains to be learned about their multiscale interactions. Developing a deeper understanding of the molecular- and mesoscale phenomena at water/solid interfaces will be essential to driving innovation to address grand challenges in supplying sufficient fit-for-purpose water in the future. In this Review, we examine the current state of knowledge surrounding adsorption, reactivity, and transport in several key classes of water/solid interfaces, drawing on a synergistic combination of theory, simulation, and experiments, and finally, provide an outlook for prioritizing strategic research directions.

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Research Organization:: Argonne National Laboratory (ANL), Argonne, IL (United States); Energy Frontier Research Centers (EFRC) (United States). Advanced Materials for Energy-Water Systems (AMEWS) Center

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC02-06CH11357

OSTI ID:: 1845829

Journal Information:: Chemical Reviews, Journal Name: Chemical Reviews Journal Issue: 15 Vol. 121; ISSN 0009-2665

Publisher:: American Chemical SocietyCopyright Statement

Country of Publication:: United States

Language:: English

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Enrichment and Distribution of Pb ²⁺ Ions in Zwitterionic Poly(cysteine methacrylate) Brushes at the Solid–Liquid Interface He, Qiming; Qiao, Yijun; Mandia, David J. Langmuir, Vol. 35, Issue 52 https://doi.org/10.1021/acs.langmuir.9b02770	journal	December 2019
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Understanding Ion Mobility in P2VP/NMP ⁺ I ^– Polymer Electrolytes: A Combined Simulation and Experimental Study Chu, Weiwei; Webb, Michael A.; Deng, Chuting Macromolecules, Vol. 53, Issue 8 https://doi.org/10.1021/acs.macromol.9b02329	journal	April 2020
Controlling the Structure of MoS ₂ Membranes via Covalent Functionalization with Molecular Spacers Hoenig, Eli; Strong, Steven E.; Wang, Mingzhan Nano Letters, Vol. 20, Issue 11 https://doi.org/10.1021/acs.nanolett.0c02114	journal	October 2020
Nanometer Resolution Elemental Mapping in Graphene-Based TEM Liquid Cells Kelly, Daniel J.; Zhou, Mingwei; Clark, Nick Nano Letters, Vol. 18, Issue 2 https://doi.org/10.1021/acs.nanolett.7b04713	journal	January 2018
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Noncovalent Immobilization of Cationic Ruthenium Complex in a Metal–Organic Framework by Ion Exchange Leading to a Heterogeneous Olefin Metathesis Catalyst for Use in Green Solvents Chołuj, Artur; Krzesiński, Paweł; Ruszczyńska, Anna Organometallics, Vol. 38, Issue 18 https://doi.org/10.1021/acs.organomet.9b00287	journal	July 2019
Polymer Brushes for Membrane Separations: A Review Keating, John J.; Imbrogno, Joseph; Belfort, Georges ACS Applied Materials & Interfaces, Vol. 8, Issue 42 https://doi.org/10.1021/acsami.6b09068	journal	October 2016
Engendering Long-Term Air and Light Stability of a TiO ₂ -Supported Porphyrinic Dye via Atomic Layer Deposition Hoffeditz, William L.; Son, Ho-Jin; Pellin, Michael J. ACS Applied Materials & Interfaces, Vol. 8, Issue 50 https://doi.org/10.1021/acsami.6b10844	journal	December 2016
Basal-Plane Ligand Functionalization on Semiconducting 2H-MoS ₂ Monolayers Ding, Qi; Czech, Kyle J.; Zhao, Yuzhou ACS Applied Materials & Interfaces, Vol. 9, Issue 14 https://doi.org/10.1021/acsami.7b01262	journal	March 2017
Surface Grafting of Ru(II) Diazonium-Based Sensitizers on Metal Oxides Enhances Alkaline Stability for Solar Energy Conversion Bangle, Rachel; Sampaio, Renato N.; Troian-Gautier, Ludovic ACS Applied Materials & Interfaces, Vol. 10, Issue 3 https://doi.org/10.1021/acsami.7b16641	journal	January 2018
Silatrane Anchors for Metal Oxide Surfaces: Optimization for Potential Photocatalytic and Electrocatalytic Applications Materna, Kelly L.; Jiang, Jianbing; Crabtree, Robert H. ACS Applied Materials & Interfaces, Vol. 11, Issue 6 https://doi.org/10.1021/acsami.8b04138	journal	June 2018
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Bioinspired, Multidisciplinary, Iterative Catalyst Design Creates the Highest Performance Peroxidase Mimics and the Field of Sustainable Ultradilute Oxidation Catalysis (SUDOC) Warner, Genoa R.; Somasundar, Yogesh; Jansen, Kyle C. ACS Catalysis, Vol. 9, Issue 8 https://doi.org/10.1021/acscatal.9b01409	journal	July 2019
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Insight into the Effects of Water on the Ethene to Aromatics Reaction with HZSM-5 Wang, Huiqiu; Hou, Yilin; Sun, Wenjing ACS Catalysis, Vol. 10, Issue 9 https://doi.org/10.1021/acscatal.9b05552	journal	April 2020
Recent Development of Inorganic Nanoparticles for Biomedical Imaging Kim, Dokyoon; Kim, Jonghoon; Park, Yong Il ACS Central Science, Vol. 4, Issue 3 https://doi.org/10.1021/acscentsci.7b00574	journal	January 2018
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