Correlation-driven electronic reconstruction in FeTe1–xSex

Huang, Jianwei; Yu, Rong; Xu, Zhijun; Zhu, Jian-Xin; Oh, Ji Seop; Jiang, Qianni; Wang, Meng; Wu, Han; Chen, Tong; Denlinger, Jonathan D.; Mo, Sung-Kwan; Hashimoto, Makoto; Michiardi, Matteo; Pedersen, Tor M.; Gorovikov, Sergey; Zhdanovich, Sergey; Damascelli, Andrea; Gu, Genda; Dai, Pengcheng; Chu, Jiun-Haw; Lu, Donghui; Si, Qimiao; Birgeneau, Robert J.; Yi, Ming

doi:10.1038/s42005-022-00805-6

Title: Correlation-driven electronic reconstruction in FeTe_1–xSe_x

Abstract

Electronic correlation is of fundamental importance to high temperature superconductivity. While the low energy electronic states in cuprates are dominantly affected by correlation effects across the phase diagram, observation of correlation-driven changes in fermiology amongst the iron-based superconductors remains rare. Here we present experimental evidence for a correlation-driven reconstruction of the Fermi surface tuned independently by two orthogonal axes of temperature and Se/Te ratio in the iron chalcogenide family FeTe_1–xSe_x. We demonstrate that this reconstruction is driven by the de-hybridization of a strongly renormalized d_xy orbital with the remaining itinerant iron 3d orbitals in the emergence of an orbital-selective Mott phase. Our observations are further supported by our theoretical calculations to be salient spectroscopic signatures of such a non-thermal evolution from a strongly correlated metallic phase into an orbital-selective Mott phase in d_xy as Se concentration is reduced.

Authors:

Huang, Jianwei ^[1];

^[2]; Xu, Zhijun ^[3];

^[4]; Oh, Ji Seop ^[5]; Jiang, Qianni ^[6];

^[7]; Wu, Han ^[1]; Chen, Tong ^[1];

^[8];

^[9];

^[10];

^[11]; Gorovikov, Sergey ^[11];

^[12];

^[12]; Gu, Genda ^[13]; Dai, Pengcheng ^[1];

^[14] more »

Rice University, Houston, TX (United States)
Renmin University of China, Beijing (China)
National Institute of Standards and Technology (NIST), Gaithersburg, MD (United States); University of Maryland, College Park, MD (United States); University of California, Berkeley, CA (United States)
Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)
Rice University, Houston, TX (United States); University of California, Berkeley, CA (United States)
University of Washington, Seattle, WA (United State
Sun Yat-Sen University, Guangzhou (China)
Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States). Advanced Light Source (ALS)
SLAC National Accelerator Laboratory, Menlo Park, CA (United States). Stanford Synchrotron Radiation Lightsource (SSRL)
University of British Columbia, Vancouver, BC (Canada); Max Planck Institute for Chemical Physics of Solids, Dresden (Germany)
Canadian Light Source (CLS), Saskatoon, SK (Canada)
University of British Columbia, Vancouver, BC (Canada)
Brookhaven National Laboratory (BNL), Upton, NY (United States)
University of Washington, Seattle, WA (United States)
University of California, Berkeley, CA (United States); Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)

Publication Date:: Wed Jan 26 00:00:00 EST 2022

Research Org.:: Brookhaven National Laboratory (BNL), Upton, NY (United States); Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States). Advanced Light Source (ALS); Rice Univ., Houston, TX (United States); Los Alamos National Laboratory (LANL), Los Alamos, NM (United States); SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division; Canada Foundation for Innovation (CFI); Natural Sciences and Engineering Research Council of Canada (NSERC); National Research Council (NRC); Canadian Institutes of Health Research (CIHR); Government of Saskatchewan; Robert A. Welch Foundation; Alfred P. Sloan Foundation; Gordon and Betty Moore Foundation; National Natural Science Foundation of China (NSFC); Ministry of Science and Technology of the People’s Republic of China (MOST); National Program on Key Research Project; USDOE National Nuclear Security Administration (NNSA); USDOE Laboratory Directed Research and Development (LDRD) Program; National Science Foundation (NSF); National Key Research and Development Program of China; Canada First Research Excellence Fund (CFREF)

OSTI Identifier:: 1922015

Alternate Identifier(s):: OSTI ID: 1844568; OSTI ID: 1862011; OSTI ID: 1877037; OSTI ID: 1877048

Report Number(s):: LA-UR-20-27137; BNL-222721-2022-JAAM
Journal ID: ISSN 2399-3650; TRN: US2312254

Grant/Contract Number:: SC0012704; AC02-76SF00515; AC02-05CH11231; C-2024; GBMF9470; SC0021421; SC0012311; C-1839; SC0018197; C-1411; 11674392; 2016YFA0300504; 18XNLG24; 89233218CNA000001; 11904414; AC02-98CH10886

Resource Type:: Accepted Manuscript

Journal Name:: Communications Physics

Additional Journal Information:: Journal Volume: 5; Journal Issue: 1; Journal ID: ISSN 2399-3650

Publisher:: Springer Nature

Country of Publication:: United States

Language:: English

Subject:: 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; electronic properties and materials; superconducting properties and materials

Citation Formats


                    Huang, Jianwei, Yu, Rong, Xu, Zhijun, Zhu, Jian-Xin, Oh, Ji Seop, Jiang, Qianni, Wang, Meng, Wu, Han, Chen, Tong, Denlinger, Jonathan D., Mo, Sung-Kwan, Hashimoto, Makoto, Michiardi, Matteo, Pedersen, Tor M., Gorovikov, Sergey, Zhdanovich, Sergey, Damascelli, Andrea, Gu, Genda, Dai, Pengcheng, Chu, Jiun-Haw, Lu, Donghui, Si, Qimiao, Birgeneau, Robert J., and Yi, Ming. Correlation-driven electronic reconstruction in FeTe1–xSex.  United States: N. p., 2022. 
Web.  doi:10.1038/s42005-022-00805-6.

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                    Huang, Jianwei, Yu, Rong, Xu, Zhijun, Zhu, Jian-Xin, Oh, Ji Seop, Jiang, Qianni, Wang, Meng, Wu, Han, Chen, Tong, Denlinger, Jonathan D., Mo, Sung-Kwan, Hashimoto, Makoto, Michiardi, Matteo, Pedersen, Tor M., Gorovikov, Sergey, Zhdanovich, Sergey, Damascelli, Andrea, Gu, Genda, Dai, Pengcheng, Chu, Jiun-Haw, Lu, Donghui, Si, Qimiao, Birgeneau, Robert J., & Yi, Ming. Correlation-driven electronic reconstruction in FeTe1–xSex.  United States.  https://doi.org/10.1038/s42005-022-00805-6

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                    Huang, Jianwei, Yu, Rong, Xu, Zhijun, Zhu, Jian-Xin, Oh, Ji Seop, Jiang, Qianni, Wang, Meng, Wu, Han, Chen, Tong, Denlinger, Jonathan D., Mo, Sung-Kwan, Hashimoto, Makoto, Michiardi, Matteo, Pedersen, Tor M., Gorovikov, Sergey, Zhdanovich, Sergey, Damascelli, Andrea, Gu, Genda, Dai, Pengcheng, Chu, Jiun-Haw, Lu, Donghui, Si, Qimiao, Birgeneau, Robert J., and Yi, Ming. Wed .  
"Correlation-driven electronic reconstruction in FeTe1–xSex".  United States.  https://doi.org/10.1038/s42005-022-00805-6.  https://www.osti.gov/servlets/purl/1922015.

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@article{osti_1922015,

  title        = {Correlation-driven electronic reconstruction in FeTe1–xSex},

  author       = {Huang, Jianwei and Yu, Rong and Xu, Zhijun and Zhu, Jian-Xin and Oh, Ji Seop and Jiang, Qianni and Wang, Meng and Wu, Han and Chen, Tong and Denlinger, Jonathan D. and Mo, Sung-Kwan and Hashimoto, Makoto and Michiardi, Matteo and Pedersen, Tor M. and Gorovikov, Sergey and Zhdanovich, Sergey and Damascelli, Andrea and Gu, Genda and Dai, Pengcheng and Chu, Jiun-Haw and Lu, Donghui and Si, Qimiao and Birgeneau, Robert J. and Yi, Ming},

  abstractNote = {Electronic correlation is of fundamental importance to high temperature superconductivity. While the low energy electronic states in cuprates are dominantly affected by correlation effects across the phase diagram, observation of correlation-driven changes in fermiology amongst the iron-based superconductors remains rare. Here we present experimental evidence for a correlation-driven reconstruction of the Fermi surface tuned independently by two orthogonal axes of temperature and Se/Te ratio in the iron chalcogenide family FeTe1–xSex. We demonstrate that this reconstruction is driven by the de-hybridization of a strongly renormalized dxy orbital with the remaining itinerant iron 3d orbitals in the emergence of an orbital-selective Mott phase. Our observations are further supported by our theoretical calculations to be salient spectroscopic signatures of such a non-thermal evolution from a strongly correlated metallic phase into an orbital-selective Mott phase in dxy as Se concentration is reduced.},

  doi          = {10.1038/s42005-022-00805-6},

  journal      = {Communications Physics},

  number       = 1,

  volume       = 5,

  place        = {United States},

  year         = {Wed Jan 26 00:00:00 EST 2022},

  month        = {Wed Jan 26 00:00:00 EST 2022}

}

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DOI: 10.1103/PhysRevB.80.174509

Evidence for Majorana bound states in an iron-based superconductor
journal, August 2018

Wang, Dongfei; Kong, Lingyuan; Fan, Peng
Science, Vol. 362, Issue 6412
DOI: 10.1126/science.aao1797

Nematic transition and nanoscale suppression of superconductivity in Fe(Te,Se)
journal, June 2021

Zhao, He; Li, Hong; Dong, Lianyang
Nature Physics, Vol. 17, Issue 8
DOI: 10.1038/s41567-021-01254-8

Angle-Resolved Photoemission Spectroscopy of the Iron-Chalcogenide Superconductor ${Fe}_{1.03} {Te}_{0.7} {Se}_{0.3}$ : Strong Coupling Behavior and the Universality of Interband Scattering
journal, November 2010

Nakayama, K.; Sato, T.; Richard, P.
Physical Review Letters, Vol. 105, Issue 19
DOI: 10.1103/PhysRevLett.105.197001

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Title: Correlation-driven electronic reconstruction in FeTe1–xSex

Abstract

Citation Formats

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Title: Correlation-driven electronic reconstruction in FeTe_1–xSe_x

Symmetry-breaking orbital anisotropy observed for detwinned Ba(Fe1-xCox)2As2 above the spin density wave transition
journal, April 2011

From (π,0) magnetic order to superconductivity with (π,π) magnetic resonance in Fe1.02Te1−xSex
journal, July 2010

Experimental observation of incoherent-coherent crossover and orbital-dependent band renormalization in iron chalcogenide superconductors
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Observation of universal strong orbital-dependent correlation effects in iron chalcogenides
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Evolution from incoherent to coherent electronic states and its implications for superconductivity in ${FeTe}_{1 - x}$ ${Se}_{x}$
journal, April 2014

Strong Electron Correlations in the Normal State of the Iron-Based ${FeSe}_{0.42} {Te}_{0.58}$ Superconductor Observed by Angle-Resolved Photoemission Spectroscopy
journal, March 2010

Observation of a Novel Orbital Selective Mott Transition in ${Ca}_{1.8} {Sr}_{0.2} {RuO}_{4}$
journal, August 2009

Evolution from non-Fermi- to Fermi-liquid transport via isovalent doping in ${BaFe}_{2} {({As}_{1 - x} P_{x})}_{2}$ superconductors
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Incoherent-coherent crossover and the pseudogap in Te-annealed superconducting ${Fe}_{1 + y} {Te}_{1 - x} {Se}_{x}$ revealed by magnetotransport measurements
journal, May 2019

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Unconventional Hall Effect in Pnictides from Interband Interactions
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Coexistence of superconductivity and short-range double-stripe spin correlations in Te-vapor annealed ${FeTe}_{1 - x} {Se}_{x}$ ( $x \leq 0.2$ )
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Pseudogap opening and formation of Fermi arcs as an orbital-selective Mott transition in momentum space
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Formation of Hubbard-like bands as a fingerprint of strong electron-electron interactions in FeSe
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Orbital-Selective Mott Phase in Multiorbital Models for Alkaline Iron Selenides $K_{1 - x} {Fe}_{2 - y} {Se}_{2}$
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From antiferromagnetism to superconductivity in ${Fe}_{1 + y} {Te}_{1 - x} {Se}_{x}$ $(0 \leq x \leq 0.20)$ : Neutron powder diffraction analysis
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Doping dependence of the spin excitations in the Fe-based superconductors Fe $_{1 + y}$ Te $_{1 - x}$ Se $_{x}$
journal, June 2013

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journal, October 2009

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journal, May 2017

Incoherent strange metal sharply bounded by a critical doping in Bi2212
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Role of chalcogen vapor annealing in inducing bulk superconductivity in ${Fe}_{1 + y} {Te}_{1 - x} {Se}_{x}$
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journal, August 2018

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journal, April 2014

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journal, February 2015

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