Colloidal Quantum Dot Solar Cells: Progressive Deposition Techniques and Future Prospects on Large-area Fabrication

Zhao, Qian; Han, Rui; Marshall, Ashley R.; Wang, Shuo; Wieliczka, Brian M.; Ni, Jian; Zhang, Jianjun; Yuan, Jianyu; Luther, Joseph M.; Hazarika, Abhijit; Li, Guo-Ran

doi:10.1002/adma.202107888

Title: Colloidal Quantum Dot Solar Cells: Progressive Deposition Techniques and Future Prospects on Large-area Fabrication

Journal Article · 12 January 2022 · Advanced Materials

DOI: https://doi.org/10.1002/adma.202107888 · OSTI ID:1841965

Zhao, Qian ^[1]; Han, Rui ^[1]; Marshall, Ashley R. ^[2]; Wang, Shuo ^[1];

^[3]; Ni, Jian ^[1]; Zhang, Jianjun ^[1]; Yuan, Jianyu ^[4];

^[3]; Hazarika, Abhijit ^[5]; Li, Guo-Ran ^[1]

Nankai Univ., Tianjin (China)
Univ. of Oxford (United Kingdom)
National Renewable Energy Lab. (NREL), Golden, CO (United States)
Soochow University, Taipei (Taiwan)
Indian Inst. of Chemical Technology, Tarnaka (India)

Colloidally grown nanosized semiconductors yield extremely high-quality optoelectronic materials. Many examples have pointed to near perfect photoluminescence quantum yields, meaning non-radiative optical processes (losses) can be completely suppressed allowing for technology-leading materials as high purity color centers in display technology and emitters in LEDs. Furthermore, because of high chemical yield, and improved understanding of the surfaces, these materials, particularly colloidal quantum dots (QDs) can also be ideal candidates for other optoelectronic applications. Given the strong drive toward carbon neutrality and limiting climate change, electricity from solar photovoltaics will play a large role in the power generation sector. QDs have been developed and shown dramatic improvements over the past 15 years as photoactive materials in photovoltaics and have unique potential with various innovative deposition properties which could lead to exceptionally low-cost and high-performance devices. Once the key issues related to charge transport in optically thick arrays are addressed, QD-based photovoltaic technology could become a better candidate for practical application. In this article, w e show how the possibilities of different deposition techniques could bring QD-based solar cells to the industrial level and discuss the challenges for perovskite QD solar cells in particular, to achieve large-area fabrication for further advancing technology to solve pivotal energy and environmental issues.

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Research Organization:: National Renewable Energy Laboratory (NREL), Golden, CO (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)

Grant/Contract Number:: AC36-08GO28308

OSTI ID:: 1841965

Report Number(s):: NREL/JA-5900-81126; MainId:79902; UUID:64a22840-786b-4dc9-b9aa-4536968382d4; MainAdminID:63694

Journal Information:: Advanced Materials, Journal Name: Advanced Materials Journal Issue: 17 Vol. 34; ISSN 0935-9648

Publisher:: WileyCopyright Statement

Country of Publication:: United States

Language:: English

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