Atomic/molecular layer deposition for energy storage and conversion
Abstract
Energy storage and conversion systems, including batteries, supercapacitors, fuel cells, solar cells, and photoelectrochemical water splitting, have played vital roles in the reduction of fossil fuel usage, addressing environmental issues and the development of electric vehicles. The fabrication and surface/interface engineering of electrode materials with refined structures are indispensable for achieving optimal performances for the different energy-related devices. Atomic layer deposition (ALD) and molecular layer deposition (MLD) techniques, the gas-phase thin film deposition processes with self-limiting and saturated surface reactions, have emerged as powerful techniques for surface and interface engineering in energy-related devices due to their exceptional capability of precise thickness control, excellent uniformity and conformity, tunable composition and relatively low deposition temperature. In the past few decades, ALD and MLD have been intensively studied for energy storage and conversion applications with remarkable progress. In this work, we give a comprehensive summary of the development and achievements of ALD and MLD and their applications for energy storage and conversion, including batteries, supercapacitors, fuel cells, solar cells, and photoelectrochemical water splitting. Moreover, the fundamental understanding of the mechanisms involved in different devices will be deeply reviewed. Furthermore, the large-scale potential of ALD and MLD techniques is discussed and predicted. Finally, wemore »
- Authors:
-
- Univ. of Western Ontario, London, ON (Canada)
- Univ. of British Columbia, Vancouver, BC (Canada)
- Argonne National Lab. (ANL), Argonne, IL (United States)
- Publication Date:
- Research Org.:
- Argonne National Lab. (ANL), Argonne, IL (United States)
- Sponsoring Org.:
- USDOE Office of Energy Efficiency and Renewable Energy (EERE), Transportation Office. Vehicle Technologies Office; Natural Sciences and Engineering Research Council of Canada (NSERC); Ontario Research Fund; Canada Foundation for Innovation (CFI); University of Western Ontario; University of British Columbia
- OSTI Identifier:
- 1833390
- Grant/Contract Number:
- AC02-06CH11357
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Chemical Society Reviews
- Additional Journal Information:
- Journal Volume: 50; Journal Issue: 6; Journal ID: ISSN 0306-0012
- Publisher:
- Royal Society of Chemistry
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 25 ENERGY STORAGE
Citation Formats
Zhao, Yang, Zhang, Lei, Liu, Jian, Adair, Keegan, Zhao, Feipeng, Sun, Yipeng, Wu, Tianpin, Bi, Xuanxuan, Amine, Khalil, Lu, Jun, and Sun, Xueliang. Atomic/molecular layer deposition for energy storage and conversion. United States: N. p., 2021.
Web. doi:10.1039/d0cs00156b.
Zhao, Yang, Zhang, Lei, Liu, Jian, Adair, Keegan, Zhao, Feipeng, Sun, Yipeng, Wu, Tianpin, Bi, Xuanxuan, Amine, Khalil, Lu, Jun, & Sun, Xueliang. Atomic/molecular layer deposition for energy storage and conversion. United States. https://doi.org/10.1039/d0cs00156b
Zhao, Yang, Zhang, Lei, Liu, Jian, Adair, Keegan, Zhao, Feipeng, Sun, Yipeng, Wu, Tianpin, Bi, Xuanxuan, Amine, Khalil, Lu, Jun, and Sun, Xueliang. Mon .
"Atomic/molecular layer deposition for energy storage and conversion". United States. https://doi.org/10.1039/d0cs00156b. https://www.osti.gov/servlets/purl/1833390.
@article{osti_1833390,
title = {Atomic/molecular layer deposition for energy storage and conversion},
author = {Zhao, Yang and Zhang, Lei and Liu, Jian and Adair, Keegan and Zhao, Feipeng and Sun, Yipeng and Wu, Tianpin and Bi, Xuanxuan and Amine, Khalil and Lu, Jun and Sun, Xueliang},
abstractNote = {Energy storage and conversion systems, including batteries, supercapacitors, fuel cells, solar cells, and photoelectrochemical water splitting, have played vital roles in the reduction of fossil fuel usage, addressing environmental issues and the development of electric vehicles. The fabrication and surface/interface engineering of electrode materials with refined structures are indispensable for achieving optimal performances for the different energy-related devices. Atomic layer deposition (ALD) and molecular layer deposition (MLD) techniques, the gas-phase thin film deposition processes with self-limiting and saturated surface reactions, have emerged as powerful techniques for surface and interface engineering in energy-related devices due to their exceptional capability of precise thickness control, excellent uniformity and conformity, tunable composition and relatively low deposition temperature. In the past few decades, ALD and MLD have been intensively studied for energy storage and conversion applications with remarkable progress. In this work, we give a comprehensive summary of the development and achievements of ALD and MLD and their applications for energy storage and conversion, including batteries, supercapacitors, fuel cells, solar cells, and photoelectrochemical water splitting. Moreover, the fundamental understanding of the mechanisms involved in different devices will be deeply reviewed. Furthermore, the large-scale potential of ALD and MLD techniques is discussed and predicted. Finally, we will provide insightful perspectives on future directions for new material design by ALD and MLD and untapped opportunities in energy storage and conversion.},
doi = {10.1039/d0cs00156b},
journal = {Chemical Society Reviews},
number = 6,
volume = 50,
place = {United States},
year = {Mon Feb 01 00:00:00 EST 2021},
month = {Mon Feb 01 00:00:00 EST 2021}
}
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