Review on Nonconventional Fibrillation Methods of Producing Cellulose Nanofibrils and Their Applications

Wang, Lu; Li, Kai; Copenhaver, Katie; Mackay, Susan; Lamm, Meghan E.; Zhao, Xianhui; Dixon, Brandon; Wang, Jinwu; Han, Yousoo; Neivandt, David; Johnson, Donna A.; Walker, Colleen C.; Ozcan, Soydan; Gardner, Douglas J.

doi:10.1021/acs.biomac.1c00640

Title: Review on Nonconventional Fibrillation Methods of Producing Cellulose Nanofibrils and Their Applications

Journal Article · 10 September 2021 · Biomacromolecules

DOI: https://doi.org/10.1021/acs.biomac.1c00640 · OSTI ID:1826035

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^[2]; Mackay, Susan ^[1];

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^[2]; Dixon, Brandon ^[1];

^[3]; Han, Yousoo ^[1];

^[1]; Johnson, Donna A. ^[1]; Walker, Colleen C. ^[1];

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Univ. of Maine, Orono, ME (United States)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
USDA Forest Service, Madison, WI (United States). Forest Products Lab.

The production of cellulose nanofibrils (CNFs) continues to receive considerable attention because of their desirable material characteristics for a variety of consumer applications. There are, however, challenges that remain in transitioning CNFs from research to widespread adoption in the industrial sectors, including production cost and material performance. Here, we cover CNFs produced from nonconventional fibrillation methods as a potential alternative solution. Pretreating biomass by biological, chemical, mechanical, or physical means can render plant feedstocks more facile for processing and thus lower energy requirements to produce CNFs. CNFs from nonconventional fibrillation methods have been investigated for various applications, including films, composites, aerogels, and Pickering emulsifiers. Continued research is needed to develop protocols to standardize the characterization (e.g., degree of fibrillation) of the lignocellulosic fibrillation processes and resulting CNF products to make them more attractive to the industry for specific product applications.

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Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: USDOE Office of Energy Efficiency and Renewable Energy (EERE), Energy Efficiency Office. Advanced Manufacturing Office

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 1826035

Journal Information:: Biomacromolecules, Journal Name: Biomacromolecules Journal Issue: 10 Vol. 22; ISSN 1525-7797

Publisher:: American Chemical SocietyCopyright Statement

Country of Publication:: United States

Language:: English

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Individualization of Nano-Sized Plant Cellulose Fibrils by Direct Surface Carboxylation Using TEMPO Catalyst under Neutral Conditions Saito, Tsuguyuki; Hirota, Masayuki; Tamura, Naoyuki Biomacromolecules, Vol. 10, Issue 7, p. 1992-1996 https://doi.org/10.1021/bm900414t	journal	July 2009
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Nanocellulose Production: Exploring the Enzymatic Route and Residues of Pulp and Paper Industry Michelin, Michele; Gomes, Daniel G.; Romaní, Aloia Molecules, Vol. 25, Issue 15 https://doi.org/10.3390/molecules25153411	journal	July 2020

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