Ellipticity controlled dissociative double ionization of ethane by strong fields

Basnayake, Gihan; Hoerner, Paul; Mignolet, Benoit; Lee, Mi Kyung; Lin, Yun Fei; Winney, Alexander H.; Debrah, Duke A.; Popaj, Leon; Shi, Xuetao; Lee, Suk Kyoung; Schlegel, H. Bernhard; Remacle, Francoise; Li, Wen

doi:10.1039/D1CP03585A

Title: Ellipticity controlled dissociative double ionization of ethane by strong fields

Abstract

The ellipticity of a laser can control the dissociation pathways of ethane dications produced by strong fields.

Authors:

Basnayake, Gihan ^[1]; Hoerner, Paul ^[1];

^[2]; Lee, Mi Kyung ^[1]; Lin, Yun Fei ^[1]; Winney, Alexander H. ^[1]; Debrah, Duke A. ^[1]; Popaj, Leon ^[1]; Shi, Xuetao ^[1]; Lee, Suk Kyoung ^[1];

^[1]; Remacle, Francoise ^[2];

^[1]

Department of Chemistry, Wayne State University, Detroit, Michigan 48202, USA
Department of Chemistry, University of Liège, B4000 Liège, Belgium

Publication Date:: 2021-10-27

Sponsoring Org.:: USDOE

OSTI Identifier:: 1825817

Resource Type:: Publisher's Accepted Manuscript

Journal Name:: Physical Chemistry Chemical Physics. PCCP

Additional Journal Information:: Journal Name: Physical Chemistry Chemical Physics. PCCP Journal Volume: 23 Journal Issue: 41; Journal ID: ISSN 1463-9076

Publisher:: Royal Society of Chemistry (RSC)

Country of Publication:: United Kingdom

Language:: English

Citation Formats


                    Basnayake, Gihan, Hoerner, Paul, Mignolet, Benoit, Lee, Mi Kyung, Lin, Yun Fei, Winney, Alexander H., Debrah, Duke A., Popaj, Leon, Shi, Xuetao, Lee, Suk Kyoung, Schlegel, H. Bernhard, Remacle, Francoise, and Li, Wen. Ellipticity controlled dissociative double ionization of ethane by strong fields.  United Kingdom: N. p., 2021. 
Web.  doi:10.1039/D1CP03585A.

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                    Basnayake, Gihan, Hoerner, Paul, Mignolet, Benoit, Lee, Mi Kyung, Lin, Yun Fei, Winney, Alexander H., Debrah, Duke A., Popaj, Leon, Shi, Xuetao, Lee, Suk Kyoung, Schlegel, H. Bernhard, Remacle, Francoise, & Li, Wen. Ellipticity controlled dissociative double ionization of ethane by strong fields.  United Kingdom.  https://doi.org/10.1039/D1CP03585A

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                    Basnayake, Gihan, Hoerner, Paul, Mignolet, Benoit, Lee, Mi Kyung, Lin, Yun Fei, Winney, Alexander H., Debrah, Duke A., Popaj, Leon, Shi, Xuetao, Lee, Suk Kyoung, Schlegel, H. Bernhard, Remacle, Francoise, and Li, Wen. Wed .  
"Ellipticity controlled dissociative double ionization of ethane by strong fields".  United Kingdom.  https://doi.org/10.1039/D1CP03585A.

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@article{osti_1825817,

  title        = {Ellipticity controlled dissociative double ionization of ethane by strong fields},

  author       = {Basnayake, Gihan and Hoerner, Paul and Mignolet, Benoit and Lee, Mi Kyung and Lin, Yun Fei and Winney, Alexander H. and Debrah, Duke A. and Popaj, Leon and Shi, Xuetao and Lee, Suk Kyoung and Schlegel, H. Bernhard and Remacle, Francoise and Li, Wen},

  abstractNote = {The ellipticity of a laser can control the dissociation pathways of ethane dications produced by strong fields.},

  doi          = {10.1039/D1CP03585A},

  journal      = {Physical Chemistry Chemical Physics. PCCP},

  number       = 41,

  volume       = 23,

  place        = {United Kingdom},

  year         = {2021},

  month        = {10}

}

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Title: Ellipticity controlled dissociative double ionization of ethane by strong fields

Abstract

Citation Formats

Doubly charged ion mass spectra: III—N-alkanes journal, January 1982

Wigner phase space method: Analysis for semiclassical applications journal, August 1976

Strong-field ionization rates of linear polyenes simulated with time-dependent configuration interaction with an absorbing potential journal, November 2014

Dissociation of methanol by ion-impact: Breakup dynamics, bond rearrangement and kinetic energy release journal, September 2008

Formation of fragment ions (H+, H3+, CH3+) from ethane in intense femtosecond laser fields – from understanding to control journal, January 2013

Attosecond-Recollision-Controlled Selective Fragmentation of Polyatomic Molecules journal, December 2012

Doubly-charged ethane ions: Solution to the dilemma of stability predicted by theory and instability observed in experiment journal, August 1986

Strong field ionization rates simulated with time-dependent configuration interaction and an absorbing potential journal, May 2014

Coulomb-repulsion-assisted double ionization from doubly excited states of argon journal, August 2017

Attosecond Electron Correlation Dynamics in Double Ionization of Benzene Probed with Two-Electron Angular Streaking journal, September 2017

Angular dependence of strong field sequential double ionization for neon and acetylene simulated with time-dependent configuration interaction using CIS and CISD-IP journal, February 2020

Formation of H3+ from ethane dication induced by electron impact journal, November 2020

Fragmentation of long-lived hydrocarbons after strong field ionization journal, May 2016

Metastable decomposition and hydrogen migration of ethane dication produced in an intense femtosecond near-infrared laser field journal, February 2011

Coincidence ion imaging with a fast frame camera journal, December 2014

Strong-field control of H3+ production from methanol dications: Selecting between local and extended formation mechanisms journal, February 2020

Formation and decay of doubly charged ions inn-alkanes from methane to triacontane journal, August 1992

Distribution functions in physics: Fundamentals journal, April 1984

Ejection of triatomic hydrogen molecular ion from methanol in intense laser fields journal, October 2005

Angle-Dependent Ionization of Small Molecules by Time-Dependent Configuration Interaction and an Absorbing Potential journal, May 2015

Atomic and Molecular Dynamics in Intense Optical Fields journal, October 1996

The Multielectron Ionization Dynamics Underlying Attosecond Strong-Field Spectroscopies journal, March 2012

Photodissociation Dynamics journal, January 1996

Coincidence momentum imaging of ultrafast hydrogen migration in methanol and its isotopomers in intense laser fields journal, May 2006

Studies of H+, H+2, and H+3 dissociative ionization fragments from methane, ethane, methanol, ethanol, and some deuterated methanols using electron-impact excitation and a time-of-flight method incorporating mass analysis journal, January 1979

Communication: Time- and space-sliced velocity map electron imaging journal, December 2014

Dissociative ionization of ethane with femtosecond pulses of radiation journal, January 2018

Substituent effects on H 3 + formation via H 2 roaming mechanisms from organic molecules under strong-field photodissociation journal, December 2018

Coherent vibrations in methanol cation probed by periodic H3+ ejection after double ionization journal, March 2018

Selective Control over Fragmentation Reactions in Polyatomic Molecules Using Impulsive Laser Alignment journal, April 2014

Time-resolving the ultrafast H2 roaming chemistry and H3+ formation using extreme-ultraviolet pulses journal, April 2020

Hydrogen scrambling in H 3 + generation from ethane induced by ultrashort intense laser fields journal, January 2013

Electron impact dissociative ionization of ethane: Cross sections, appearance potentials, and dissociation pathways journal, August 1998

Electron-capture-induced decomposition of the supposed ethane dication journal, March 1991

Efficient ejection of H3+ from hydrocarbon molecules induced by ultrashort intense laser fields journal, September 2008

Hydrogen scrambling in ethane induced by intense laser fields: Statistical analysis of coincidence events journal, May 2012

Laser Control of Chemical Reactions journal, March 1998

Formation of H 3 + due to Intramolecular Bond Rearrangement in Doubly Charged Methanol journal, November 2006

Disentangling Strong-Field Multielectron Dynamics with Angular Streaking journal, April 2018

The dissociative ionization and Coulomb explosion of ethane by a femtosecond laser field journal, September 2004

Fragmentation dynamics of the methanol dication journal, September 2008

Note: An improved 3D imaging system for electron-electron coincidence measurements journal, September 2015

SHARC: ab Initio Molecular Dynamics with Surface Hopping in the Adiabatic Representation Including Arbitrary Couplings journal, March 2011

The Origin of Primary H+3 Ions in Mass Spectra journal, September 1996

LASER CHEMISTRY AND PHYSICS: The Next Frontier journal, March 2002

Molcas 8: New capabilities for multiconfigurational quantum chemical calculations across the periodic table : Molcas 8 journal, November 2015

Mechanisms and time-resolved dynamics for trihydrogen cation (H3 +) formation from organic molecules in strong laser fields journal, July 2017

Charge stripping of hydrocarbon positive ions journal, August 1983

Unusual mechanism for H 3 + formation from ethane as obtained by femtosecond laser pulse ionization and quantum chemical calculations journal, March 2011

Finite-temperature Wigner phase-space sampling and temperature effects on the excited-state dynamics of 2-nitronaphthalene journal, January 2019

H2 roaming chemistry and the formation of H3+ from organic molecules in strong laser fields journal, December 2018

Doubly charged ion mass spectra: III—N-alkanes
journal, January 1982

Wigner phase space method: Analysis for semiclassical applications
journal, August 1976

Strong-field ionization rates of linear polyenes simulated with time-dependent configuration interaction with an absorbing potential
journal, November 2014

Dissociation of methanol by ion-impact: Breakup dynamics, bond rearrangement and kinetic energy release
journal, September 2008

Formation of fragment ions (H+, H3+, CH3+) from ethane in intense femtosecond laser fields – from understanding to control
journal, January 2013

Attosecond-Recollision-Controlled Selective Fragmentation of Polyatomic Molecules
journal, December 2012

Doubly-charged ethane ions: Solution to the dilemma of stability predicted by theory and instability observed in experiment
journal, August 1986

Strong field ionization rates simulated with time-dependent configuration interaction and an absorbing potential
journal, May 2014

Coulomb-repulsion-assisted double ionization from doubly excited states of argon
journal, August 2017

Attosecond Electron Correlation Dynamics in Double Ionization of Benzene Probed with Two-Electron Angular Streaking
journal, September 2017

Angular dependence of strong field sequential double ionization for neon and acetylene simulated with time-dependent configuration interaction using CIS and CISD-IP
journal, February 2020

Formation of H3+ from ethane dication induced by electron impact
journal, November 2020

Fragmentation of long-lived hydrocarbons after strong field ionization
journal, May 2016

Metastable decomposition and hydrogen migration of ethane dication produced in an intense femtosecond near-infrared laser field
journal, February 2011

Coincidence ion imaging with a fast frame camera
journal, December 2014

Strong-field control of H3+ production from methanol dications: Selecting between local and extended formation mechanisms
journal, February 2020

Formation and decay of doubly charged ions inn-alkanes from methane to triacontane
journal, August 1992

Distribution functions in physics: Fundamentals
journal, April 1984

Ejection of triatomic hydrogen molecular ion from methanol in intense laser fields
journal, October 2005

Angle-Dependent Ionization of Small Molecules by Time-Dependent Configuration Interaction and an Absorbing Potential
journal, May 2015

Atomic and Molecular Dynamics in Intense Optical Fields
journal, October 1996

The Multielectron Ionization Dynamics Underlying Attosecond Strong-Field Spectroscopies
journal, March 2012

Photodissociation Dynamics
journal, January 1996

Coincidence momentum imaging of ultrafast hydrogen migration in methanol and its isotopomers in intense laser fields
journal, May 2006

Studies of H+, H+2, and H+3 dissociative ionization fragments from methane, ethane, methanol, ethanol, and some deuterated methanols using electron-impact excitation and a time-of-flight method incorporating mass analysis
journal, January 1979

Communication: Time- and space-sliced velocity map electron imaging
journal, December 2014

Dissociative ionization of ethane with femtosecond pulses of radiation
journal, January 2018

Substituent effects on H ₃ ⁺ formation via H ₂ roaming mechanisms from organic molecules under strong-field photodissociation
journal, December 2018

Coherent vibrations in methanol cation probed by periodic H3+ ejection after double ionization
journal, March 2018

Selective Control over Fragmentation Reactions in Polyatomic Molecules Using Impulsive Laser Alignment
journal, April 2014

Time-resolving the ultrafast H2 roaming chemistry and H3+ formation using extreme-ultraviolet pulses
journal, April 2020

Hydrogen scrambling in H ₃ ⁺ generation from ethane induced by ultrashort intense laser fields
journal, January 2013

Electron impact dissociative ionization of ethane: Cross sections, appearance potentials, and dissociation pathways
journal, August 1998

Electron-capture-induced decomposition of the supposed ethane dication
journal, March 1991

Efficient ejection of H3+ from hydrocarbon molecules induced by ultrashort intense laser fields
journal, September 2008

Hydrogen scrambling in ethane induced by intense laser fields: Statistical analysis of coincidence events
journal, May 2012

Laser Control of Chemical Reactions
journal, March 1998

Formation of $H_{3}^{+}$ due to Intramolecular Bond Rearrangement in Doubly Charged Methanol
journal, November 2006

Disentangling Strong-Field Multielectron Dynamics with Angular Streaking
journal, April 2018

The dissociative ionization and Coulomb explosion of ethane by a femtosecond laser field
journal, September 2004

Fragmentation dynamics of the methanol dication
journal, September 2008

Note: An improved 3D imaging system for electron-electron coincidence measurements
journal, September 2015

SHARC: ab Initio Molecular Dynamics with Surface Hopping in the Adiabatic Representation Including Arbitrary Couplings
journal, March 2011

The Origin of Primary H+3 Ions in Mass Spectra
journal, September 1996

LASER CHEMISTRY AND PHYSICS: The Next Frontier
journal, March 2002

Molcas 8: New capabilities for multiconfigurational quantum chemical calculations across the periodic table : Molcas 8
journal, November 2015

Mechanisms and time-resolved dynamics for trihydrogen cation (H3 +) formation from organic molecules in strong laser fields
journal, July 2017

Charge stripping of hydrocarbon positive ions
journal, August 1983

Unusual mechanism for H ₃ ⁺ formation from ethane as obtained by femtosecond laser pulse ionization and quantum chemical calculations
journal, March 2011

Finite-temperature Wigner phase-space sampling and temperature effects on the excited-state dynamics of 2-nitronaphthalene
journal, January 2019

H2 roaming chemistry and the formation of H3+ from organic molecules in strong laser fields
journal, December 2018