Fast-Charging Aging Considerations: Incorporation and Alignment of Cell Design and Material Degradation Pathways

Chinnam, Parameswara R.; Colclasure, Andrew M.; Chen, Bor-Rong; Tanim, Tanvir R.; Dufek, Eric J.; Smith, Kandler; Evans, Michael C.; Dunlop, Alison R.; Trask, Stephen E.; Polzin, Bryant J.; Jansen, Andrew N.

doi:10.1021/acsaem.1c01398

Title: Fast-Charging Aging Considerations: Incorporation and Alignment of Cell Design and Material Degradation Pathways

Journal Article · 08 September 2021 · ACS Applied Energy Materials

DOI: https://doi.org/10.1021/acsaem.1c01398 · OSTI ID:1822826

Chinnam, Parameswara R. ^[1];

^[2];

^[1]; Tanim, Tanvir R. ^[1];

^[1]; Smith, Kandler ^[2]; Evans, Michael C. ^[1]; Dunlop, Alison R. ^[3];

^[3]; Polzin, Bryant J. ^[3]; Jansen, Andrew N. ^[3]

Idaho National Lab. (INL), Idaho Falls, ID (United States)
National Renewable Energy Lab. (NREL), Golden, CO (United States)
Argonne National Lab. (ANL), Argonne, IL (United States)

Fast charging of batteries for electric vehicles is seen as one of the most direct ways to enhance adoption. Currently, fast charging is limited by increased cell aging, which is primarily driven by Li plating and degradation of cathode materials. Here, using combined sets of experimental and computational analysis and a suite of different charge protocols, we begin to examine the interplay between failure mode, cell designs, and ultimately aging mechanisms. Slight variation in cell design and the subsequent impacts that charge protocols have on aging can create distinct cell-to-cell variation. As little as 2% difference in porosity change at the cell negative electrode during cycling due to early Li metal plating has been found to alter the aging pathway and either accelerate or inhibit the loss due to Li plating.

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Research Organization:: Argonne National Laboratory (ANL), Argonne, IL (United States); Idaho National Laboratory (INL), Idaho Falls, ID (United States); National Renewable Energy Laboratory (NREL), Golden, CO (United States)

Sponsoring Organization:: USDOE Office of Energy Efficiency and Renewable Energy (EERE), Transportation Office. Vehicle Technologies Office

Grant/Contract Number:: AC02-06CH11357; AC07-05ID14517; AC36-08GO28308

OSTI ID:: 1822826

Report Number(s):: INL/JOU--21-61371-Rev000; NREL/JA--5700-78800; MainId:32717; UUID:ccaa3f6a-e213-4c4d-93bd-903e94b113e0; MainAdminID:62989

Journal Information:: ACS Applied Energy Materials, Journal Name: ACS Applied Energy Materials Journal Issue: 9 Vol. 4; ISSN 2574-0962

Publisher:: American Chemical Society (ACS)Copyright Statement

Country of Publication:: United States

Language:: English

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Title: Fast-Charging Aging Considerations: Incorporation and Alignment of Cell Design and Material Degradation Pathways

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