Roadmap of Solid-State Lithium-Organic Batteries toward 500 Wh kg–1

Zhao, Lihong; Lakraychi, Alae Eddine; Chen, Zhaoyang; Liang, Yanliang; Yao, Yan

doi:10.1021/acsenergylett.1c01368

Title: Roadmap of Solid-State Lithium-Organic Batteries toward 500 Wh kg^–1

Journal Article · 25 August 2021 · ACS Energy Letters

DOI: https://doi.org/10.1021/acsenergylett.1c01368 · OSTI ID:1815358

Zhao, Lihong ^[1]; Lakraychi, Alae Eddine ^[2]; Chen, Zhaoyang ^[2];

^[2];

^[2]

Univ. of Houston, TX (United States); University of Houston
Univ. of Houston, TX (United States)

Over the past few years, solid-state electrolytes (SSEs) have attracted tremendous attention due to their credible promise toward high-energy batteries. In parallel, organic battery electrode materials (OBEMs) are gaining momentum as strong candidates thanks to their lower environmental footprint, flexibility in molecular design and high energy metrics. Integration of the two constitutes a potential synergy to enable energy-dense solid-state batteries (SSBs) with high safety, low cost, and long-term sustainability. Here, we present the technological feasibility of combining OBEMs with SSEs along with the possible cell configurations that may result from this peculiar combination. We provide an overview of organic SSBs and discuss their main challenges. We analyze the performance-limiting factors and the critical cell design parameters governing cell-level specific energy and energy density. Lastly, we propose guidelines to achieve 500 Wh kg^–1 cell-level specific energy with solid-state Li–organic batteries.

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Research Organization:: Univ. of Houston, TX (United States)

Sponsoring Organization:: USDOE Office of Energy Efficiency and Renewable Energy (EERE), Transportation Office. Vehicle Technologies Office

Grant/Contract Number:: EE0008234

OSTI ID:: 1815358

Journal Information:: ACS Energy Letters, Journal Name: ACS Energy Letters Vol. 6; ISSN 2380-8195

Publisher:: American Chemical Society (ACS)Copyright Statement

Country of Publication:: United States

Language:: English

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