Anomalously strong near-neighbor attraction in doped 1D cuprate chains

Chen, Zhuoyu; Wang, Yao; Rebec, Slavko N.; Jia, Tao; Hashimoto, Makoto; Lu, Donghui; Moritz, Brian; Moore, Robert G.; Devereaux, Thomas P.; Shen, Zhi-Xun

doi:10.1126/science.abf5174

Title: Anomalously strong near-neighbor attraction in doped 1D cuprate chains

Journal Article · 09 September 2021 · Science

DOI: https://doi.org/10.1126/science.abf5174 · OSTI ID:1814931

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SLAC National Accelerator Lab., Menlo Park, CA (United States). Stanford Institute for Materials and Energy Science (SIMES); Stanford Univ., CA (United States); Stanford Univ., CA (United States). Geballe Lab. for Advanced Materials; SLAC National Accelerator Laboratory/Stanford University
SLAC National Accelerator Lab., Menlo Park, CA (United States). Stanford Institute for Materials and Energy Science (SIMES); Clemson Univ., SC (United States)
SLAC National Accelerator Lab., Menlo Park, CA (United States). Stanford Institute for Materials and Energy Science (SIMES); Stanford Univ., CA (United States); Stanford Univ., CA (United States). Geballe Lab. for Advanced Materials
SLAC National Accelerator Lab., Menlo Park, CA (United States). Stanford Institute for Materials and Energy Science (SIMES); Stanford Univ., CA (United States). Geballe Lab. for Advanced Materials; Stanford Univ., CA (United States)
Clemson Univ., SC (United States); SLAC National Accelerator Lab., Menlo Park, CA (United States). Stanford Synchrotron Radiation Lightsource (SSRL)
Stanford Univ., CA (United States). Geballe Lab. for Advanced Materials; SLAC National Accelerator Lab., Menlo Park, CA (United States). Stanford Synchrotron Radiation Lightsource (SSRL)
SLAC National Accelerator Lab., Menlo Park, CA (United States). Stanford Institute for Materials and Energy Science (SIMES); Stanford Univ., CA (United States); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)

In the cuprates, one-dimensional (1D) chain compounds provide a distinctive opportunity to understand the microscopic physics, owing to the availability of reliable theories. However, progress has been limited by the challenge of controllably doping these materials. We report the synthesis and spectroscopic analysis of the 1D cuprate Ba_2-xSr_xCuO_3+δ over a wide range of hole doping. Our angle-resolved photoemission experiments reveal the doping evolution of the holon and spinon branches. We identify a prominent folding branch whose intensity fails to match predictions of the simple Hubbard model. An additional strong near-neighbor attraction, which may arise from coupling to phonons, quantitatively explains experiments for all accessible doping levels. Furthermore, considering structural and quantum chemistry similarities among cuprates, this attraction may play a similarly important role in high-temperature cuprate superconductors.

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Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States); SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)

Sponsoring Organization:: National Science Foundation (NSF); USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division

Grant/Contract Number:: AC02-05CH11231; AC02-76SF00515; AC05-00OR22725

OSTI ID:: 1814931

Journal Information:: Science, Journal Name: Science Journal Issue: 6560 Vol. 373; ISSN 0036-8075

Publisher:: AAASCopyright Statement

Country of Publication:: United States

Language:: English

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