Structural Evidence for Ultrafast Polarization Rotation in Ferroelectric/Dielectric Superlattice Nanodomains

Lee, Hyeon Jun; Ahn, Youngjun; Marks, Samuel D.; Landahl, Eric C.; Zhuang, Shihao; Yusuf, M. Humed; Dawber, Matthew; Lee, Jun Young; Kim, Tae Yeon; Unithrattil, Sanjith; Chun, Sae Hwan; Kim, Sunam; Eom, Intae; Park, Sang-Yeon; Kim, Kyung Sook; Lee, Sooheyong; Jo, Ji Young; Hu, Jiamian; Evans, Paul G.

doi:10.1103/PhysRevX.11.031031

Title: Structural Evidence for Ultrafast Polarization Rotation in Ferroelectric/Dielectric Superlattice Nanodomains

Abstract

Weakly coupled ferroelectric/dielectric superlattice thin-film heterostructures exhibit complex nanoscale polarization configurations that arise from a balance of competing electrostatic, elastic, and domain-wall contributions to the free energy. A key feature of these configurations is that the polarization can locally have a significant component that is along the thin-film surface normal direction with an overall configuration maintaining zero net in-plane polarization. ${PbTiO}_{3} / {SrTiO}_{3}$ thin-film superlattice heterostructures on a conducting ${SrRuO}_{3}$ bottom electrode on ${SrTiO}_{3}$ have a room-temperature stripe nanodomain pattern with a nanometer-scale lateral period. Ultrafast time-resolved x-ray free electron laser diffraction and scattering experiments reveal that above-bandgap optical pulses induce propagating acoustic pulses and a perturbation of the domain diffuse scattering intensity arising from the nanoscale stripe domain configuration. With 400-nm optical excitation, two separate acoustic pulses are observed: a high-amplitude pulse resulting from strong optical absorption in the bottom electrode and a weaker pulse arising from the depolarization-field-screening effect due to absorption directly within the superlattice. The picosecond scale variation of the nanodomain diffuse scattering intensity is consistent with a larger polarization change than would be expected due to the polarization-tetragonality coupling of uniformly polarized ferroelectrics. The polarization change is consistent, instead, with polarization rotation facilitated by the reorientation of the in-plane component of the polarization at the domain boundaries of the striped polarization structure. The complex steady-state configuration within these ferroelectric heterostructures leads to ultrafast polarization rotation phenomena that have previously been available only through the selection of bulk crystal composition.

Authors:

Lee, Hyeon Jun; Ahn, Youngjun;

; Landahl, Eric C.; Zhuang, Shihao; Yusuf, M. Humed; Dawber, Matthew; Lee, Jun Young; Kim, Tae Yeon; Unithrattil, Sanjith;

; Kim, Sunam; Eom, Intae;

; Kim, Kyung Sook; Lee, Sooheyong;

;

Publication Date:: Mon Aug 09 00:00:00 EDT 2021

Research Org.:: Argonne National Laboratory (ANL), Argonne, IL (United States). Advanced Photon Source (APS); Univ. of Wisconsin, Madison, WI (United States)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

OSTI Identifier:: 1812421

Alternate Identifier(s):: OSTI ID: 1814749

Grant/Contract Number:: FG02-04ER46147; AC02-06CH11357

Resource Type:: Published Article

Journal Name:: Physical Review. X

Additional Journal Information:: Journal Name: Physical Review. X Journal Volume: 11 Journal Issue: 3; Journal ID: ISSN 2160-3308

Publisher:: American Physical Society

Country of Publication:: United States

Language:: English

Subject:: 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; X-ray diffuse scattering; X-ray diffraction; photoexcitation; multilayer thin films; free-electron lasers; ferroelectrics; ultrafast optics; phonons; ferroelectricity; electric polarization

Citation Formats


                    Lee, Hyeon Jun, Ahn, Youngjun, Marks, Samuel D., Landahl, Eric C., Zhuang, Shihao, Yusuf, M. Humed, Dawber, Matthew, Lee, Jun Young, Kim, Tae Yeon, Unithrattil, Sanjith, Chun, Sae Hwan, Kim, Sunam, Eom, Intae, Park, Sang-Yeon, Kim, Kyung Sook, Lee, Sooheyong, Jo, Ji Young, Hu, Jiamian, and Evans, Paul G. Structural Evidence for Ultrafast Polarization Rotation in Ferroelectric/Dielectric Superlattice Nanodomains.  United States: N. p., 2021. 
Web.  doi:10.1103/PhysRevX.11.031031.

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                    Lee, Hyeon Jun, Ahn, Youngjun, Marks, Samuel D., Landahl, Eric C., Zhuang, Shihao, Yusuf, M. Humed, Dawber, Matthew, Lee, Jun Young, Kim, Tae Yeon, Unithrattil, Sanjith, Chun, Sae Hwan, Kim, Sunam, Eom, Intae, Park, Sang-Yeon, Kim, Kyung Sook, Lee, Sooheyong, Jo, Ji Young, Hu, Jiamian, & Evans, Paul G. Structural Evidence for Ultrafast Polarization Rotation in Ferroelectric/Dielectric Superlattice Nanodomains.  United States.  https://doi.org/10.1103/PhysRevX.11.031031

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                    Lee, Hyeon Jun, Ahn, Youngjun, Marks, Samuel D., Landahl, Eric C., Zhuang, Shihao, Yusuf, M. Humed, Dawber, Matthew, Lee, Jun Young, Kim, Tae Yeon, Unithrattil, Sanjith, Chun, Sae Hwan, Kim, Sunam, Eom, Intae, Park, Sang-Yeon, Kim, Kyung Sook, Lee, Sooheyong, Jo, Ji Young, Hu, Jiamian, and Evans, Paul G. Mon .  
"Structural Evidence for Ultrafast Polarization Rotation in Ferroelectric/Dielectric Superlattice Nanodomains".  United States.  https://doi.org/10.1103/PhysRevX.11.031031.

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@article{osti_1812421,

  title        = {Structural Evidence for Ultrafast Polarization Rotation in Ferroelectric/Dielectric Superlattice Nanodomains},

  author       = {Lee, Hyeon Jun and Ahn, Youngjun and Marks, Samuel D. and Landahl, Eric C. and Zhuang, Shihao and Yusuf, M. Humed and Dawber, Matthew and Lee, Jun Young and Kim, Tae Yeon and Unithrattil, Sanjith and Chun, Sae Hwan and Kim, Sunam and Eom, Intae and Park, Sang-Yeon and Kim, Kyung Sook and Lee, Sooheyong and Jo, Ji Young and Hu, Jiamian and Evans, Paul G.},

  abstractNote = {Weakly coupled ferroelectric/dielectric superlattice thin-film heterostructures exhibit complex nanoscale polarization configurations that arise from a balance of competing electrostatic, elastic, and domain-wall contributions to the free energy. A key feature of these configurations is that the polarization can locally have a significant component that is along the thin-film surface normal direction with an overall configuration maintaining zero net in-plane polarization. PbTiO3/SrTiO3 thin-film superlattice heterostructures on a conducting SrRuO3 bottom electrode on SrTiO3 have a room-temperature stripe nanodomain pattern with a nanometer-scale lateral period. Ultrafast time-resolved x-ray free electron laser diffraction and scattering experiments reveal that above-bandgap optical pulses induce propagating acoustic pulses and a perturbation of the domain diffuse scattering intensity arising from the nanoscale stripe domain configuration. With 400-nm optical excitation, two separate acoustic pulses are observed: a high-amplitude pulse resulting from strong optical absorption in the bottom electrode and a weaker pulse arising from the depolarization-field-screening effect due to absorption directly within the superlattice. The picosecond scale variation of the nanodomain diffuse scattering intensity is consistent with a larger polarization change than would be expected due to the polarization-tetragonality coupling of uniformly polarized ferroelectrics. The polarization change is consistent, instead, with polarization rotation facilitated by the reorientation of the in-plane component of the polarization at the domain boundaries of the striped polarization structure. The complex steady-state configuration within these ferroelectric heterostructures leads to ultrafast polarization rotation phenomena that have previously been available only through the selection of bulk crystal composition.},

  doi          = {10.1103/PhysRevX.11.031031},

  journal      = {Physical Review. X},

  number       = 3,

  volume       = 11,

  place        = {United States},

  year         = {Mon Aug 09 00:00:00 EDT 2021},

  month        = {Mon Aug 09 00:00:00 EDT 2021}

}

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Title: Structural Evidence for Ultrafast Polarization Rotation in Ferroelectric/Dielectric Superlattice Nanodomains

Abstract

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Ultrafast Photovoltaic Response in Ferroelectric Nanolayers journal, February 2012

Development of an X-ray pixel detector with multi-port charge-coupled device for X-ray free-electron laser experiments journal, March 2014

Thermodynamic theory of PbTiO 3 journal, October 1987

Ultrafast lattice response of photoexcited thin films studied by X-ray diffraction journal, November 2014

Polarization rotation mechanism for ultrahigh electromechanical response in single-crystal piezoelectrics journal, January 2000

Probing Impulsive Strain Propagation with X-Ray Pulses journal, April 2001

Non-thermal fluence threshold for femtosecond pulsed x-ray radiation damage in perovskite complex oxide epitaxial heterostructures journal, December 2019

Theory for displacive excitation of coherent phonons journal, January 1992

Observation of room-temperature polar skyrmions journal, April 2019

Electronic Origin of Ultrafast Photoinduced Strain in BiFeO 3 journal, January 2013

Tailoring the Properties of Artificially Layered Ferroelectric Superlattices journal, December 2007

XCVI. Theory of barium titanate: Part I journal, October 1949

From flexoelectricity to absolute deformation potentials: The case of SrTiO 3 journal, November 2015

Ultrahigh strain and piezoelectric behavior in relaxor based ferroelectric single crystals journal, August 1997

Stabilization of Highly Polar BiFeO 3 -like Structure: A New Interface Design Route for Enhanced Ferroelectricity in Artificial Perovskite Superlattices journal, March 2016

Hard X-ray free-electron laser with femtosecond-scale timing jitter journal, October 2017

Elastic Constants of Strontium Titanate journal, January 1963

Photoinduced Domain Pattern Transformation in Ferroelectric-Dielectric Superlattices journal, July 2017

Thermoelastic study of nanolayered structures using time-resolved X-ray diffraction at high repetition rate journal, January 2014

Thermal conductivity of perovskite ferroelectrics journal, September 2008

Emergent chirality in the electric polarization texture of titanate superlattices journal, January 2018

Surface generation and detection of phonons by picosecond light pulses journal, September 1986

A first-principles study of structural and elastic properties of bulk SrRuO 3 journal, December 2013

Optical Properties and Band Structure of SrTi O 3 and BaTi O 3 journal, October 1965

Negative capacitance in multidomain ferroelectric superlattices journal, June 2016

Structural and energetic properties of domains in PbTiO 3 /SrTiO 3 superlattices from first principles journal, May 2012

X-Ray Diffraction Studies of 180° Ferroelectric Domains in PbTiO 3 / SrTiO 3 Superlattices under an Applied Electric Field journal, May 2010

Dynamical atomic charges: The case of AB O 3 compounds journal, September 1998

Strong Visible-Light Absorption and Hot-Carrier Injection in TiO 2 /SrRuO 3 Heterostructures journal, April 2013

Phase diagrams and physical properties of single-domain epitaxial Pb ( Zr 1 − x Ti x ) O 3 thin films journal, February 2003

Dynamics of the laser-induced ferroelectric excitation in BaTiO3 studied by x-ray diffraction journal, January 2007

Effective medium approximation for the effective optical constants of a bilayer and a multilayer structure based on the characteristic matrix technique journal, March 2003

Thermophysical properties of SrHfO3 and SrRuO3 journal, October 2004

Nanosecond Optically Induced Phase Transformation in Compressively Strained BiFeO 3 on LaAlO 3 journal, July 2019

Role of temperature-dependent electron trapping dynamics in the optically driven nanodomain transformation in a PbTiO 3 /SrTiO 3 superlattice journal, January 2020

Localized Excited Charge Carriers Generate Ultrafast Inhomogeneous Strain in the Multiferroic BiFeO 3 journal, March 2014

Correlations between tetragonality, polarization, and ionic displacement in PbTiO 3 -derived ferroelectric perovskite solid solutions journal, October 2010

Following Strain-Induced Mosaicity Changes of Ferroelectric Thin Films by Ultrafast Reciprocal Space Mapping journal, February 2013

Observation of Nanoscale 180 ° Stripe Domains in Ferroelectric P b T i O 3 Thin Films journal, July 2002

Spatially resolved steady-state negative capacitance journal, January 2019

Observation of polar vortices in oxide superlattices journal, January 2016

Caloric characteristics of PbTiO3 in the temperature range of the ferroelectric phase transition journal, September 2012

Coherent Acoustic Phonon Oscillations in Semiconductor Multiple Quantum Wells with Piezoelectric Fields journal, January 2000

Effects of doping on the lattice parameter of SrTiO 3 journal, June 2012

Soft-mode driven polarity reversal in ferroelectrics mapped by ultrafast x-ray diffraction journal, March 2018

Electric-Field-Driven Nanosecond Ferroelastic-Domain Switching Dynamics in Epitaxial Pb ( Zr , Ti ) O 3 Film journal, November 2019

Nanoscale heat transport studied by high-resolution time-resolved x-ray diffraction journal, September 2011

Electrostatic Coupling and Local Structural Distortions at Interfaces in Ferroelectric/Paraelectric Superlattices journal, May 2012

Thermodynamic theory of epitaxial ferroelectric thin films with dense domain structures journal, November 2001

High-temperature heat capacity and thermal expansion of SrTiO 3 and SrZrO 3 perovskites journal, February 1996

Phase-Transition Temperatures of Strained Single-Crystal SrRuO 3 Thin Films journal, February 2010

Coupled Ultrafast Lattice and Polarization Dynamics in Ferroelectric Nanolayers journal, June 2007

Thermoelectric properties of reduced and La-doped single-crystalline SrTiO3 journal, April 2005

Phase-field simulation of domain structure for PbTiO3/SrTiO3 superlattices journal, September 2009

Evolution of flux-closure domain arrays in oxide multilayers with misfit strain journal, June 2019

Ultrafast Reversal of the Ferroelectric Polarization journal, May 2017

Surface morphology determined by (001) single-crystal SrTiO3 termination journal, November 2000

Ferroelectric Domains in PbTiO 3 /SrTiO 3 Superlattices journal, January 2012

Unusual Behavior of the Ferroelectric Polarization in PbTiO 3 / SrTiO 3 Superlattices journal, October 2005

Structural and Optical Properties of PbTiO3 Grown on SrTiO3 Substrates by Peroxide MBE journal, January 2006

Nanosecond Dynamics of Ferroelectric/Dielectric Superlattices journal, July 2011

Ultrafast Photovoltaic Response in Ferroelectric Nanolayers
journal, February 2012

Development of an X-ray pixel detector with multi-port charge-coupled device for X-ray free-electron laser experiments
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Thermodynamic theory of PbTiO ₃
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Ultrafast lattice response of photoexcited thin films studied by X-ray diffraction
journal, November 2014

Polarization rotation mechanism for ultrahigh electromechanical response in single-crystal piezoelectrics
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Probing Impulsive Strain Propagation with X-Ray Pulses
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Non-thermal fluence threshold for femtosecond pulsed x-ray radiation damage in perovskite complex oxide epitaxial heterostructures
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Theory for displacive excitation of coherent phonons
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Observation of room-temperature polar skyrmions
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Electronic Origin of Ultrafast Photoinduced Strain in ${BiFeO}_{3}$
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Tailoring the Properties of Artificially Layered Ferroelectric Superlattices
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XCVI. Theory of barium titanate: Part I
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From flexoelectricity to absolute deformation potentials: The case of ${SrTiO}_{3}$
journal, November 2015

Ultrahigh strain and piezoelectric behavior in relaxor based ferroelectric single crystals
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Stabilization of Highly Polar ${BiFeO}_{3}$ -like Structure: A New Interface Design Route for Enhanced Ferroelectricity in Artificial Perovskite Superlattices
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Hard X-ray free-electron laser with femtosecond-scale timing jitter
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Elastic Constants of Strontium Titanate
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Photoinduced Domain Pattern Transformation in Ferroelectric-Dielectric Superlattices
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Thermoelastic study of nanolayered structures using time-resolved X-ray diffraction at high repetition rate
journal, January 2014

Thermal conductivity of perovskite ferroelectrics
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Emergent chirality in the electric polarization texture of titanate superlattices
journal, January 2018

Surface generation and detection of phonons by picosecond light pulses
journal, September 1986

A first-principles study of structural and elastic properties of bulk SrRuO ₃
journal, December 2013

Optical Properties and Band Structure of SrTi $O_{3}$ and BaTi $O_{3}$
journal, October 1965

Negative capacitance in multidomain ferroelectric superlattices
journal, June 2016

Structural and energetic properties of domains in PbTiO $_{3}$ /SrTiO $_{3}$ superlattices from first principles
journal, May 2012

X-Ray Diffraction Studies of 180° Ferroelectric Domains in ${PbTiO}_{3} / {SrTiO}_{3}$ Superlattices under an Applied Electric Field
journal, May 2010

Dynamical atomic charges: The case of $AB O_{3}$ compounds
journal, September 1998

Strong Visible-Light Absorption and Hot-Carrier Injection in TiO ₂ /SrRuO ₃ Heterostructures
journal, April 2013

Phase diagrams and physical properties of single-domain epitaxial $Pb ({Zr}_{1 - x} {Ti}_{x}) O_{3}$ thin films
journal, February 2003

Dynamics of the laser-induced ferroelectric excitation in BaTiO3 studied by x-ray diffraction
journal, January 2007

Effective medium approximation for the effective optical constants of a bilayer and a multilayer structure based on the characteristic matrix technique
journal, March 2003

Thermophysical properties of SrHfO3 and SrRuO3
journal, October 2004

Nanosecond Optically Induced Phase Transformation in Compressively Strained ${BiFeO}_{3}$ on ${LaAlO}_{3}$
journal, July 2019

Role of temperature-dependent electron trapping dynamics in the optically driven nanodomain transformation in a PbTiO ₃ /SrTiO ₃ superlattice
journal, January 2020

Localized Excited Charge Carriers Generate Ultrafast Inhomogeneous Strain in the Multiferroic ${BiFeO}_{3}$
journal, March 2014

Correlations between tetragonality, polarization, and ionic displacement in ${PbTiO}_{3}$ -derived ferroelectric perovskite solid solutions
journal, October 2010

Following Strain-Induced Mosaicity Changes of Ferroelectric Thin Films by Ultrafast Reciprocal Space Mapping
journal, February 2013

Observation of Nanoscale $180 °$ Stripe Domains in Ferroelectric ${P b T i O}_{3}$ Thin Films
journal, July 2002

Spatially resolved steady-state negative capacitance
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Observation of polar vortices in oxide superlattices
journal, January 2016

Caloric characteristics of PbTiO3 in the temperature range of the ferroelectric phase transition
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Coherent Acoustic Phonon Oscillations in Semiconductor Multiple Quantum Wells with Piezoelectric Fields
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Effects of doping on the lattice parameter of SrTiO ₃
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Soft-mode driven polarity reversal in ferroelectrics mapped by ultrafast x-ray diffraction
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Electric-Field-Driven Nanosecond Ferroelastic-Domain Switching Dynamics in Epitaxial $Pb (Zr, Ti) O_{3}$ Film
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Nanoscale heat transport studied by high-resolution time-resolved x-ray diffraction
journal, September 2011

Electrostatic Coupling and Local Structural Distortions at Interfaces in Ferroelectric/Paraelectric Superlattices
journal, May 2012

Thermodynamic theory of epitaxial ferroelectric thin films with dense domain structures
journal, November 2001

High-temperature heat capacity and thermal expansion of ${SrTiO}_{3}$ and ${SrZrO}_{3}$ perovskites
journal, February 1996

Phase-Transition Temperatures of Strained Single-Crystal SrRuO ₃ Thin Films
journal, February 2010

Coupled Ultrafast Lattice and Polarization Dynamics in Ferroelectric Nanolayers
journal, June 2007

Thermoelectric properties of reduced and La-doped single-crystalline SrTiO3
journal, April 2005

Phase-field simulation of domain structure for PbTiO3/SrTiO3 superlattices
journal, September 2009

Evolution of flux-closure domain arrays in oxide multilayers with misfit strain
journal, June 2019

Ultrafast Reversal of the Ferroelectric Polarization
journal, May 2017

Surface morphology determined by (001) single-crystal SrTiO3 termination
journal, November 2000

Ferroelectric Domains in PbTiO ₃ /SrTiO ₃ Superlattices
journal, January 2012

Unusual Behavior of the Ferroelectric Polarization in ${PbTiO}_{3} / {SrTiO}_{3}$ Superlattices
journal, October 2005

Structural and Optical Properties of PbTiO3 Grown on SrTiO3 Substrates by Peroxide MBE
journal, January 2006

Nanosecond Dynamics of Ferroelectric/Dielectric Superlattices
journal, July 2011