Toward a mechanically stable solid electrolyte interphase

Tsai, Wan-Yu; Thundat, Thomas; Nanda, Jagjit

doi:10.1016/j.matt.2021.06.014

Title: Toward a mechanically stable solid electrolyte interphase

Journal Article · 06 July 2021 · Matter (Online)

DOI: https://doi.org/10.1016/j.matt.2021.06.014 · OSTI ID:1811380

^[1]; Thundat, Thomas ^[2];

^[1]

Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Chemical Science Division
State Univ. of New York at Buffalo, NY (United States). Dept. of Chemical and Biological Engineering

The correlation between solid electrolyte interphase (SEI) mechanical properties and battery electrochemical performances is complex and remains poorly understood. Gao et al. recently proposed a new mechanical parameter to predict the SEI stability, bringing new insights onto future battery design.

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Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: USDOE Laboratory Directed Research and Development (LDRD) Program

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 1811380

Journal Information:: Matter (Online), Journal Name: Matter (Online) Journal Issue: 7 Vol. 4; ISSN 2590-2385

Publisher:: Cell Press/ElsevierCopyright Statement

Country of Publication:: United States

Language:: English

References (8)

An Artificial Solid Electrolyte Interphase with High Li-Ion Conductivity, Mechanical Strength, and Flexibility for Stable Lithium Metal Anodes Liu, Yayuan; Lin, Dingchang; Yuen, Pak Yan Advanced Materials, Vol. 29, Issue 10 https://doi.org/10.1002/adma.201605531	journal	December 2016
Unraveling the Nanoscale Heterogeneity of Solid Electrolyte Interphase Using Tip-Enhanced Raman Spectroscopy Nanda, Jagjit; Yang, Guang; Hou, Tingzheng Joule, Vol. 3, Issue 8 https://doi.org/10.1016/j.joule.2019.05.026	journal	August 2019
Unraveling the mechanical origin of stable solid electrolyte interphase Gao, Yao; Du, Xiaoqiong; Hou, Zhen Joule, Vol. 5, Issue 7 https://doi.org/10.1016/j.joule.2021.05.015	journal	July 2021
Determination of mechanical properties of the SEI in sodium ion batteries via colloidal probe microscopy Weadock, Nicholas; Varongchayakul, Nitinun; Wan, Jiayu Nano Energy, Vol. 2, Issue 5 https://doi.org/10.1016/j.nanoen.2013.08.005	journal	September 2013
Challenges for Rechargeable Li Batteries Goodenough, John B.; Kim, Youngsik Chemistry of Materials, Vol. 22, Issue 3, p. 587-603 https://doi.org/10.1021/cm901452z	journal	February 2010
Tip-enhanced Raman spectroscopy for surfaces and interfaces Wang, Xiang; Huang, Sheng-Chao; Huang, Teng-Xiang Chemical Society Reviews, Vol. 46, Issue 13 https://doi.org/10.1039/C7CS00206H	journal	January 2017
Anomalous interfacial stress generation during sodium intercalation/extraction in MoS ₂ thin-film anodes Li, Zhi; Jiang, Keren; Khan, Faheem Science Advances, Vol. 5, Issue 1 https://doi.org/10.1126/sciadv.aav2820	journal	January 2019
Band Excitation in Scanning Probe Microscopy: Recognition and Functional Imaging Jesse, S.; Vasudevan, R. K.; Collins, L. Annual Review of Physical Chemistry, Vol. 65, Issue 1 https://doi.org/10.1146/annurev-physchem-040513-103609	journal	April 2014

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