Nonuniform Flow Dynamics Probed by Nanosecond X-Ray Speckle Visibility Spectroscopy

Sun, Yanwen; Carini, Gabriella; Chollet, Matthieu; Decker, Franz-Josef; Dunne, Mike; Fuoss, Paul; Hruszkewycz, Stephan O.; Lane, Thomas J.; Nakahara, Kazutaka; Nelson, Silke; Robert, Aymeric; Sato, Takahiro; Song, Sanghoon; Stephenson, G. Brian; Sutton, Mark; Van Driel, Tim B.; Weninger, Clemens; Zhu, Diling

doi:10.1103/physrevlett.127.058001

Title: Nonuniform Flow Dynamics Probed by Nanosecond X-Ray Speckle Visibility Spectroscopy

Journal Article · 28 July 2021 · Physical Review Letters

DOI: https://doi.org/10.1103/physrevlett.127.058001 · OSTI ID:1809065

^[1]; Carini, Gabriella ^[1]; Chollet, Matthieu ^[1]; Decker, Franz-Josef ^[1]; Dunne, Mike ^[1]; Fuoss, Paul ^[1];

^[2]; Lane, Thomas J. ^[1]; Nakahara, Kazutaka ^[1]; Nelson, Silke ^[1];

^[1]; Sato, Takahiro ^[1];

^[1];

^[2]; Sutton, Mark ^[3]; Van Driel, Tim B. ^[1]; Weninger, Clemens ^[1]; Zhu, Diling ^[1]

SLAC National Accelerator Lab., Menlo Park, CA (United States). Linac Coherent Light Source (LCLS)
Argonne National Lab. (ANL), Argonne, IL (United States)
McGill Univ., Montreal, QC (Canada); SLAC National Accelerator Lab., Menlo Park, CA (United States). Linac Coherent Light Source (LCLS)

We report observations of nanosecond nonuniform colloidal dynamics in a free flowing liquid jet using ultrafast x-ray speckle visibility spectroscopy. Utilizing a nanosecond double-bunch mode, the Linac Coherent Light Source free electron laser produced pairs of femtosecond coherent hard x-ray pulses. By exploring anisotropy in the visibility of summed speckle patterns which relates to the correlation functions, we evaluate not only the average particle flow rate in a colloidal nanoparticle jet, but also the nonuniform flow field within. The methodology presented here establishes the foundation for the study of nano- and atomic-scale inhomogeneous fluctuations in complex matter using x-ray free electron laser sources.

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Research Organization:: Argonne National Laboratory (ANL), Argonne, IL (United States); Brookhaven National Laboratory (BNL), Upton, NY (United States); SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC02-06CH11357; AC02-76SF00515; SC0012704

OSTI ID:: 1809065

Report Number(s):: BNL-221842-2021--JAAM

Journal Information:: Physical Review Letters, Journal Name: Physical Review Letters Journal Issue: 5 Vol. 127; ISSN 0031-9007

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

References (45)

Slow relaxations in deeply undercooled metallic liquids Wilde, Gerhard Journal of Non-Crystalline Solids, Vol. 312-314 https://doi.org/10.1016/S0022-3093(02)01753-2	journal	October 2002
The measurement of velocity gradients in laminar flow by homodyne light-scattering spectroscopy Fuller, G. G.; Rallison, J. M.; Schmidt, R. L. Journal of Fluid Mechanics, Vol. 100, Issue 03 https://doi.org/10.1017/S0022112080001280	journal	October 1980
Microsecond Structural Rheology Lehmkühler, Felix; Steinke, Ingo; Schroer, Martin A. The Journal of Physical Chemistry Letters, Vol. 8, Issue 15 https://doi.org/10.1021/acs.jpclett.7b01355	journal	July 2017
Relaxation of Bulk Metallic Glasses Studied by Mechanical Spectroscopy Qiao, Jichao; Pelletier, Jean-Marc; Casalini, Riccardo The Journal of Physical Chemistry B, Vol. 117, Issue 43 https://doi.org/10.1021/jp4067179	journal	October 2013
Revealing the atomic dance Stephenson, G. Brian; Robert, Aymeric; Grübel, Gerhard Nature Materials, Vol. 8, Issue 9 https://doi.org/10.1038/nmat2521	journal	September 2009
Towards ultrafast dynamics with split-pulse X-ray photon correlation spectroscopy at free electron laser sources Roseker, W.; Hruszkewycz, S. O.; Lehmkühler, F. Nature Communications, Vol. 9, Issue 1 https://doi.org/10.1038/s41467-018-04178-9	journal	April 2018
Split-pulse X-ray photon correlation spectroscopy with seeded X-rays from X-ray laser to study atomic-level dynamics Shinohara, Yuya; Osaka, Taito; Inoue, Ichiro Nature Communications, Vol. 11, Issue 1 https://doi.org/10.1038/s41467-020-20036-z	journal	December 2020
Demonstration of Feasibility of X-Ray Free Electron Laser Studies of Dynamics of Nanoparticles in Entangled Polymer Melts Carnis, Jerome; Cha, Wonsuk; Wingert, James Scientific Reports, Vol. 4, Issue 1 https://doi.org/10.1038/srep06017	journal	August 2014
Dynamic light scattering at low rates of shear Ackerson, B. J.; Clark, N. A. Journal de Physique, Vol. 42, Issue 7 https://doi.org/10.1051/jphys:01981004207092900	journal	January 1981
Temporal heterogeneity of the slow dynamics of a colloidal paste Ballesta, Pierre SLOW DYNAMICS IN COMPLEX SYSTEMS: 3rd International Symposium on Slow Dynamics in Complex Systems, AIP Conference Proceedings https://doi.org/10.1063/1.1764063	conference	January 2004
Speckle-visibility spectroscopy: A tool to study time-varying dynamics Bandyopadhyay, R.; Gittings, A. S.; Suh, S. S. Review of Scientific Instruments, Vol. 76, Issue 9 https://doi.org/10.1063/1.2037987	journal	September 2005
Dielectric beta relaxations in the glassy state of salol? Wagner, Hermann; Richert, Ranko The Journal of Chemical Physics, Vol. 110, Issue 23 https://doi.org/10.1063/1.479105	journal	June 1999
Design and throughput simulations of a hard x-ray split and delay line for the MID station at the European XFEL Lu, W.; Noll, T.; Roth, T. PROCEEDINGS OF THE 12TH INTERNATIONAL CONFERENCE ON SYNCHROTRON RADIATION INSTRUMENTATION – SRI2015, AIP Conference Proceedings https://doi.org/10.1063/1.4952833	conference	January 2016
ePix100 camera: Use and applications at LCLS Carini, G. A.; Alonso-Mori, R.; Blaj, G. PROCEEDINGS OF THE 12TH INTERNATIONAL CONFERENCE ON SYNCHROTRON RADIATION INSTRUMENTATION – SRI2015, AIP Conference Proceedings https://doi.org/10.1063/1.4952880	conference	January 2016
Velocity measurement by coherent x-ray heterodyning Lhermitte, Julien R. M.; Rogers, Michael C.; Manet, Sabine Review of Scientific Instruments, Vol. 88, Issue 1 https://doi.org/10.1063/1.4974099	journal	January 2017
A simple hydrodynamic model of a laminar free-surface jet in horizontal or vertical flight Haustein, Herman D.; Harnik, Ron S.; Rohlfs, Wilko Physics of Fluids, Vol. 29, Issue 8 https://doi.org/10.1063/1.4996771	journal	August 2017
Skyrmion fluctuations at a first-order phase transition boundary Esposito, V.; Zheng, X. Y.; Seaberg, M. H. Applied Physics Letters, Vol. 116, Issue 18 https://doi.org/10.1063/5.0004879	journal	May 2020
Dynamics and rheology under continuous shear flow studied by x-ray photon correlation spectroscopy Fluerasu, Andrei; Kwasniewski, Pawel; Caronna, Chiara New Journal of Physics, Vol. 12, Issue 3 https://doi.org/10.1088/1367-2630/12/3/035023	journal	March 2010
Beyond simple exponential correlation functions and equilibrium dynamics in x-ray photon correlation spectroscopy Madsen, Anders; Leheny, Robert L.; Guo, Hongyu New Journal of Physics, Vol. 12, Issue 5 https://doi.org/10.1088/1367-2630/12/5/055001	journal	May 2010
Relaxor Pb ( Mg 1 / 3 Nb 2 / 3 ) O 3 : A Ferroelectric with Multiple Inhomogeneities Fu, Desheng; Taniguchi, Hiroki; Itoh, Mitsuru Physical Review Letters, Vol. 103, Issue 20 https://doi.org/10.1103/PhysRevLett.103.207601	journal	November 2009
Direct Measurement of Microstructural Avalanches during the Martensitic Transition of Cobalt Using Coherent X-Ray Scattering Sanborn, Christopher; Ludwig, Karl F.; Rogers, Michael C. Physical Review Letters, Vol. 107, Issue 1 https://doi.org/10.1103/PhysRevLett.107.015702	journal	June 2011
High Contrast X-ray Speckle from Atomic-Scale Order in Liquids and Glasses Hruszkewycz, S. O.; Sutton, M.; Fuoss, P. H. Physical Review Letters, Vol. 109, Issue 18 https://doi.org/10.1103/PhysRevLett.109.185502	journal	November 2012
X-Ray Photon Correlation Spectroscopy Reveals Intermittent Aging Dynamics in a Metallic Glass Evenson, Zach; Ruta, Beatrice; Hechler, Simon Physical Review Letters, Vol. 115, Issue 17 https://doi.org/10.1103/PhysRevLett.115.175701	journal	October 2015
Nanosecond X-Ray Photon Correlation Spectroscopy on Magnetic Skyrmions Seaberg, M. H.; Holladay, B.; Lee, J. C. T. Physical Review Letters, Vol. 119, Issue 6 https://doi.org/10.1103/PhysRevLett.119.067403	journal	August 2017
High resolution strain measurements in highly disordered materials Sutton, Mark; Lhermitte, Julien R. M.; Ehrburger-Dolle, Françoise Physical Review Research, Vol. 3, Issue 1 https://doi.org/10.1103/PhysRevResearch.3.013119	journal	February 2021
Theoretical perspective on the glass transition and amorphous materials Berthier, Ludovic; Biroli, Giulio Reviews of Modern Physics, Vol. 83, Issue 2 https://doi.org/10.1103/RevModPhys.83.587	journal	June 2011
Linac Coherent Light Source: The first five years Bostedt, Christoph; Boutet, Sébastien; Fritz, David M. Reviews of Modern Physics, Vol. 88, Issue 1 https://doi.org/10.1103/RevModPhys.88.015007	journal	March 2016
X-ray photon correlation spectroscopy under flow Fluerasu, Andrei; Moussaïd, Abdellatif; Falus, Péter Journal of Synchrotron Radiation, Vol. 15, Issue 4 https://doi.org/10.1107/S0909049508006420	journal	May 2008
Design and characterization of an undulator beamline optimized for small-angle coherent X-ray scattering at the Advanced Photon Source Sandy, A. R.; Lurio, L. B.; Mochrie, S. G. J. Journal of Synchrotron Radiation, Vol. 6, Issue 6 https://doi.org/10.1107/S0909049599009590	journal	November 1999
Photon statistics and speckle visibility spectroscopy with partially coherent X-rays Li, Luxi; Kwaśniewski, Paweł; Orsi, Davide Journal of Synchrotron Radiation, Vol. 21, Issue 6 https://doi.org/10.1107/S1600577514015847	journal	October 2014
X-ray photon correlation spectroscopy Shpyrko, Oleg G. Journal of Synchrotron Radiation, Vol. 21, Issue 5 https://doi.org/10.1107/S1600577514018232	journal	August 2014
Focus characterization at an X-ray free-electron laser by coherent scattering and speckle analysis Sikorski, Marcin; Song, Sanghoon; Schropp, Andreas Journal of Synchrotron Radiation, Vol. 22, Issue 3 https://doi.org/10.1107/S1600577515004361	journal	April 2015
The X-ray Correlation Spectroscopy instrument at the Linac Coherent Light Source Alonso-Mori, Roberto; Caronna, Chiara; Chollet, Matthieu Journal of Synchrotron Radiation, Vol. 22, Issue 3 https://doi.org/10.1107/S1600577515004397	journal	April 2015
Application of an ePix100 detector for coherent scattering using a hard X-ray free-electron laser Sikorski, Marcin; Feng, Yiping; Song, Sanghoon Journal of Synchrotron Radiation, Vol. 23, Issue 5 https://doi.org/10.1107/S1600577516010869	journal	August 2016
Pulse intensity characterization of the LCLS nanosecond double-bunch mode of operation Sun, Yanwen; Decker, Franz-Josef; Turner, James Journal of Synchrotron Radiation, Vol. 25, Issue 3 https://doi.org/10.1107/S160057751800348X	journal	March 2018
Accurate contrast determination for X-ray speckle visibility spectroscopy Sun, Yanwen; Montana-Lopez, Jordi; Fuoss, Paul Journal of Synchrotron Radiation, Vol. 27, Issue 4 https://doi.org/10.1107/S1600577520006773	journal	June 2020
Dynamics of soft nanoparticle suspensions at hard X-ray FEL sources below the radiation-damage threshold Lehmkühler, Felix; Valerio, Joana; Sheyfer, Dina IUCrJ, Vol. 5, Issue 6 https://doi.org/10.1107/S2052252518013696	journal	October 2018
Development of a hard x-ray split-delay system at the Linac Coherent Light Source Zhu, Diling; Sun, Yanwen; Schafer, Donald W. SPIE Optics + Optoelectronics, SPIE Proceedings https://doi.org/10.1117/12.2265171	conference	June 2017
Microscopic pathways for stress relaxation in repulsive colloidal glasses Dallari, F.; Martinelli, A.; Caporaletti, F. Science Advances, Vol. 6, Issue 12 https://doi.org/10.1126/sciadv.aaz2982	journal	March 2020
The Onset of Turbulence in Pipe Flow Avila, K.; Moxey, D.; de Lozar, A. Science, Vol. 333, Issue 6039 https://doi.org/10.1126/science.1203223	journal	July 2011
Measurement of the velocity difference by photon correlation spectroscopy: an improved scheme Narayanan, Theyencheri; Cheung, Cecil; Tong, Penger Applied Optics, Vol. 36, Issue 30 https://doi.org/10.1364/AO.36.007639	journal	January 1997
Measuring temporal speckle correlations at ultrafast x-ray sources Gutt, C.; Stadler, L. -M.; Duri, A. Optics Express, Vol. 17, Issue 1 https://doi.org/10.1364/OE.17.000055	journal	December 2008
Wavelength-tunable split-and-delay optical system for hard X-ray free-electron lasers Osaka, Taito; Hirano, Takashi; Sano, Yasuhisa Optics Express, Vol. 24, Issue 9 https://doi.org/10.1364/OE.24.009187	journal	January 2016
Performance of a picosecond x-ray delay line unit at 839 keV Roseker, Wojciech; Franz, Hermann; Schulte-Schrepping, Horst Optics Letters, Vol. 34, Issue 12 https://doi.org/10.1364/OL.34.001768	journal	January 2009
Compact hard x-ray split-delay system based on variable-gap channel-cut crystals Sun, Yanwen; Wang, Nan; Song, Sanghoon Optics Letters, Vol. 44, Issue 10 https://doi.org/10.1364/OL.44.002582	journal	January 2019

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