Nonuniform Flow Dynamics Probed by Nanosecond X-Ray Speckle Visibility Spectroscopy
Abstract
We report observations of nanosecond nonuniform colloidal dynamics in a free flowing liquid jet using ultrafast x-ray speckle visibility spectroscopy. Utilizing a nanosecond double-bunch mode, the Linac Coherent Light Source free electron laser produced pairs of femtosecond coherent hard x-ray pulses. By exploring anisotropy in the visibility of summed speckle patterns which relates to the correlation functions, we evaluate not only the average particle flow rate in a colloidal nanoparticle jet, but also the nonuniform flow field within. The methodology presented here establishes the foundation for the study of nano- and atomic-scale inhomogeneous fluctuations in complex matter using x-ray free electron laser sources.
- Authors:
-
[1];
[2];
[1];
[1];
[2];
- SLAC National Accelerator Lab., Menlo Park, CA (United States). Linac Coherent Light Source (LCLS)
- Argonne National Lab. (ANL), Argonne, IL (United States)
- McGill Univ., Montreal, QC (Canada); SLAC National Accelerator Lab., Menlo Park, CA (United States). Linac Coherent Light Source (LCLS)
- Publication Date:
- Research Org.:
- Brookhaven National Lab. (BNL), Upton, NY (United States); SLAC National Accelerator Lab., Menlo Park, CA (United States); Argonne National Lab. (ANL), Argonne, IL (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1809065
- Alternate Identifier(s):
- OSTI ID: 1819702; OSTI ID: 1828894
- Report Number(s):
- BNL-221842-2021-JAAM
Journal ID: ISSN 0031-9007; TRN: US2213142
- Grant/Contract Number:
- SC0012704; AC02-76SF00515; AC02-06CH11357
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Physical Review Letters
- Additional Journal Information:
- Journal Volume: 127; Journal Issue: 5; Journal ID: ISSN 0031-9007
- Publisher:
- American Physical Society (APS)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 47 OTHER INSTRUMENTATION; Colloids; X-ray photon correlation spectroscopy; Polymers & Soft Matter; Condensed Matter & Materials Physics
Citation Formats
Sun, Yanwen, Carini, Gabriella, Chollet, Matthieu, Decker, Franz-Josef, Dunne, Mike, Fuoss, Paul, Hruszkewycz, Stephan O., Lane, Thomas J., Nakahara, Kazutaka, Nelson, Silke, Robert, Aymeric, Sato, Takahiro, Song, Sanghoon, Stephenson, G. Brian, Sutton, Mark, Van Driel, Tim B., Weninger, Clemens, and Zhu, Diling. Nonuniform Flow Dynamics Probed by Nanosecond X-Ray Speckle Visibility Spectroscopy. United States: N. p., 2021.
Web. doi:10.1103/physrevlett.127.058001.
Sun, Yanwen, Carini, Gabriella, Chollet, Matthieu, Decker, Franz-Josef, Dunne, Mike, Fuoss, Paul, Hruszkewycz, Stephan O., Lane, Thomas J., Nakahara, Kazutaka, Nelson, Silke, Robert, Aymeric, Sato, Takahiro, Song, Sanghoon, Stephenson, G. Brian, Sutton, Mark, Van Driel, Tim B., Weninger, Clemens, & Zhu, Diling. Nonuniform Flow Dynamics Probed by Nanosecond X-Ray Speckle Visibility Spectroscopy. United States. https://doi.org/10.1103/physrevlett.127.058001
Sun, Yanwen, Carini, Gabriella, Chollet, Matthieu, Decker, Franz-Josef, Dunne, Mike, Fuoss, Paul, Hruszkewycz, Stephan O., Lane, Thomas J., Nakahara, Kazutaka, Nelson, Silke, Robert, Aymeric, Sato, Takahiro, Song, Sanghoon, Stephenson, G. Brian, Sutton, Mark, Van Driel, Tim B., Weninger, Clemens, and Zhu, Diling. Wed .
"Nonuniform Flow Dynamics Probed by Nanosecond X-Ray Speckle Visibility Spectroscopy". United States. https://doi.org/10.1103/physrevlett.127.058001. https://www.osti.gov/servlets/purl/1809065.
@article{osti_1809065,
title = {Nonuniform Flow Dynamics Probed by Nanosecond X-Ray Speckle Visibility Spectroscopy},
author = {Sun, Yanwen and Carini, Gabriella and Chollet, Matthieu and Decker, Franz-Josef and Dunne, Mike and Fuoss, Paul and Hruszkewycz, Stephan O. and Lane, Thomas J. and Nakahara, Kazutaka and Nelson, Silke and Robert, Aymeric and Sato, Takahiro and Song, Sanghoon and Stephenson, G. Brian and Sutton, Mark and Van Driel, Tim B. and Weninger, Clemens and Zhu, Diling},
abstractNote = {We report observations of nanosecond nonuniform colloidal dynamics in a free flowing liquid jet using ultrafast x-ray speckle visibility spectroscopy. Utilizing a nanosecond double-bunch mode, the Linac Coherent Light Source free electron laser produced pairs of femtosecond coherent hard x-ray pulses. By exploring anisotropy in the visibility of summed speckle patterns which relates to the correlation functions, we evaluate not only the average particle flow rate in a colloidal nanoparticle jet, but also the nonuniform flow field within. The methodology presented here establishes the foundation for the study of nano- and atomic-scale inhomogeneous fluctuations in complex matter using x-ray free electron laser sources.},
doi = {10.1103/physrevlett.127.058001},
journal = {Physical Review Letters},
number = 5,
volume = 127,
place = {United States},
year = {Wed Jul 28 00:00:00 EDT 2021},
month = {Wed Jul 28 00:00:00 EDT 2021}
}
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