Title: Real-Frequency Response Functions at Finite Temperature

Journal Article · · Physical Review Letters

Building on previous developments [A. Taheridehkordi, S. H. Curnoe, and J. P. F. LeBlanc, Phys. Rev. B 99, 035120 (2019); A. Taheridehkordi, S. H. Curnoe, and J. P. F. LeBlancPhys. Rev. B101, 125109 (2020); A. Taheridehkordi, S. H. Curnoe, and J. P. F. LeBlancPhys. Rev. B102, 045115 (2020), B. Holm and U. von Barth, Phys. Rev. B 57, 2108 (1998), J. Vičičevic and M. Ferrero, Phys. Rev. B 101, 075113 (2020)], we show that the diagrammatic Monte Carlo technique allows us to compute finite-temperature response functions directly on the real-frequency axis within any field-theoretical formulation of the interacting fermion problem. There are no limitations on the type and nature of the system’s action or whether partial summation and self-consistent treatment of certain diagram classes are used. In particular, by eliminating the need for numerical analytic continuation from a Matsubara representation, our scheme allows us to study spectral densities of arbitrary complexity with controlled accuracy in models with frequency-dependent effective interactions. Finally, for illustrative purposes we consider the problem of the plasmon linewidth in a homogeneous electron gas (jellium).

Research Organization:
Brookhaven National Laboratory (BNL), Upton, NY (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
Grant/Contract Number:
SC0012704
OSTI ID:
1807937
Report Number(s):
BNL-221790-2021-JAAM
Journal Information:
Physical Review Letters, Journal Name: Physical Review Letters Journal Issue: 2 Vol. 127; ISSN 0031-9007
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English

References (25)

Decay Dynamics of Localized Surface Plasmons: Damping of Coherences and Populations of the Oscillatory Plasmon Modes journal May 2019
Hot Electrons Do the Impossible: Plasmon-Induced Dissociation of H 2 on Au journal December 2012
Theoretical predictions for hot-carrier generation from surface plasmon decay journal December 2014
Theory and computation of hot carriers generated by surface plasmon polaritons in noble metals journal June 2015
Plasmonics for improved photovoltaic devices journal February 2010
Plasmonic-metal nanostructures for efficient conversion of solar to chemical energy journal November 2011
Plasmon-enhanced plastic devices journal August 2013
Plasmon-induced hot-electron generation at nanoparticle/metal-oxide interfaces for photovoltaic and photocatalytic devices journal January 2014
A combined variational and diagrammatic quantum Monte Carlo approach to the many-electron problem journal August 2019
Effective classical partition functions journal December 1986
Real-frequency diagrammatic Monte Carlo at finite temperature journal February 2020
Optimal grouping of arbitrary diagrammatic expansions via analytic pole structure journal March 2020
Algorithmic approach to diagrammatic expansions for real-frequency evaluation of susceptibility functions journal July 2020
Signatures of multiple charge excitations in resonant inelastic x-ray scattering spectra of metals journal August 2020
Fully self-consistent GW self-energy of the electron gas journal January 1998
Shifted-action expansion and applicability of dressed diagrammatic schemes journal April 2016
Numerical analytic continuation: Answers to well-posed questions journal January 2017
Dielectric function and thermodynamic properties of jellium in the G W approximation journal May 2017
Controlling Feynman diagrammatic expansions: Physical nature of the pseudogap in the two-dimensional Hubbard model journal July 2017
Algorithmic Matsubara integration for Hubbard-like models journal January 2019
Optimized perturbation theory journal June 1981
Homotopic Action: A Pathway to Convergent Diagrammatic Theories journal June 2021
Analytical solution for time integrals in diagrammatic expansions: Application to real-frequency diagrammatic Monte Carlo journal April 2021
Polynomial complexity despite the fermionic sign journal April 2017
Harvesting the loss: surface plasmon-based hot electron photodetection journal November 2016