DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Absolute Measurement of Laser Ionization Yield in Atmospheric Pressure Range Gases over 14 Decades

Journal Article · · Physical Review Letters

Strong-field ionization is central to intense laser-matter interactions. However, standard ionization measurements have been limited to extremely low density gas samples, ignoring potential high density effects. Here, we measure strong-field ionization in atmospheric pressure range air, N2, and Ar over 14 decades of absolute yield, using mid-IR picosecond avalanche multiplication of single electrons. In this work, our results are consistent with theoretical rates for isolated atoms and molecules and quantify the ubiquitous presence of ultralow concentration gas contaminants that can significantly affect laser-gas interactions.

Research Organization:
Krell Institute, Ames, IA (United States)
Sponsoring Organization:
Defense Threat Reduction Agency (DTRA); US Air Force Office of Scientific Research (AFOSR); US Department of the Navy, Office of Naval Research (ONR); USDOE National Nuclear Security Administration (NNSA)
Grant/Contract Number:
NA0003864
OSTI ID:
1801162
Journal Information:
Physical Review Letters, Journal Name: Physical Review Letters Journal Issue: 1 Vol. 124; ISSN 0031-9007
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English

References (32)

Compression of amplified chirped optical pulses journal December 1985
Compression of amplified chirped optical pulses journal October 1985
Semi-empirical model for the rate of tunnel ionization of N2 and O2 molecule in an intense Ti:sapphire laser pulse journal May 1999
Femtosecond filamentation in transparent media journal March 2007
Megafilament in air formed by self-guided terawatt long-wavelength infrared laser journal December 2018
Counting the electrons in a multiphoton ionization by elastic scattering of microwaves journal February 2018
Dispersion interferometer for controlled fusion devices journal April 1993
Microwave diagnostics of small plasma objects journal August 2005
Remote monostatic detection of radioactive material by laser-induced breakdown journal March 2016
Tunnel and multiphoton ionization of atoms and ions in a strong laser field (Keldysh theory) journal September 2004
Tunnel ionisation of Xe in an ultra-intense CO 2 laser field (10 14 W cm -2 ) with multiple charge creation journal April 1985
Laser-induced breakdown of gases journal May 1975
Optical diagnostics of atmospheric pressure air plasmas journal February 2003
(i) Fiducial Limits for the Poisson Distribution journal December 1936
Influence of many-body interactions during the ionization of gases by short intense optical pulses journal March 2014
Interaction-induced nonlinear refractive-index reduction of gases in the midinfrared regime journal January 2016
Strong Field Ionization Rate for Arbitrary Laser Frequencies journal November 2008
Direct Measurement of the Electron Density of Extended Femtosecond Laser Pulse-Induced Filaments journal November 2010
Self-Channeling of High-Power Long-Wave Infrared Pulses in Atomic Gases journal February 2017
Bound-Electron Nonlinearity Beyond the Ionization Threshold journal May 2018
Remote detection of radioactive material using optically induced air breakdown ionization conference May 2019
Remote detection of radioactive material using mid-IR laser–driven electron avalanche journal March 2019
Bright Coherent Ultrahigh Harmonics in the keV X-ray Regime from Mid-Infrared Femtosecond Lasers journal June 2012
Direct experimental evidence of multiphoton ionization of impurities as the initiation process of laser-induced gas breakdown journal June 1970
Influence of optical and interaction-induced dephasing effects on the short-pulse ionization of atomic gases journal January 2015
Control of the filament dynamics of 10  µm pulses via designer pulse trains journal January 2019
Laser ionization of noble gases by Coulomb-barrier suppression journal January 1991
Measuring easily electron plasma densities in gases produced by ultrashort lasers and filaments journal January 2011
90 GW peak power few-cycle mid-infrared pulses from an optical parametric amplifier journal January 2011
Measurement of ultralow radiation-induced charge densities using picosecond mid-IR laser-induced breakdown journal January 2019
Tunnel and multiphoton ionization of atoms and ions in a strong laser field (Keldysh theory) [Tunnel'naya i mnogofotonnaya ionizatsiya atomov i ionov v sil'nom lazernom pole (teoriya Keldysha)] journal January 2004
Strong Field Ionization Rate for Arbitrary Laser Frequencies text January 2008