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Title: Evaluation of a semiconductor-based atmospheric radioxenon detection system

Abstract

A prototype radioxenon detection system for beta–gamma coincidence measurements has been designed using a PIPSBox and a pair of coplanar CdZnTe (CZT) detectors. Coincidence events are identified in real-time using a Field-Programmable Gate Array (FPGA). The measurement of 131mXe and studies on electron backscatter and memory effect in the PIPSBox have been presented previously; this paper details the measurement of 133/133mXe, 135Xe, and background. Here, absolute efficiencies were determined, regions of interest were defined, and Minimum Detectable Concentrations (MDC) for all four radioxenon isotopes were calculated. When neglecting interferences between the radioxenons, the prototype system has an estimated MDC of 0.61 ± 0.15 mBq/m3 for 133Xe when using gas processing parameters associated with Xenon International, satisfying the CTBTO requirement for sensitivity of ≤1 mBq/m3 for 133Xe. Simulation suggests that by increasing number of CZT detectors used by a factor of 16, the MDCs of the system can be improved by a factor of 2-3. The design shows great promise for future improvement and expansion due to its exceptional energy resolution, high background rejection rate, room temperature operation, minimal memory effect, and simple readout electronics.

Authors:
 [1];  [1];  [1]
  1. Oregon State Univ., Corvallis, OR (United States)
Publication Date:
Research Org.:
Univ. of Michigan, Ann Arbor, MI (United States)
Sponsoring Org.:
USDOE National Nuclear Security Administration (NNSA)
OSTI Identifier:
1798657
Alternate Identifier(s):
OSTI ID: 1564280
Grant/Contract Number:  
NA0002534
Resource Type:
Accepted Manuscript
Journal Name:
Nuclear Instruments and Methods in Physics Research. Section A, Accelerators, Spectrometers, Detectors and Associated Equipment
Additional Journal Information:
Journal Volume: 945; Journal ID: ISSN 0168-9002
Publisher:
Elsevier
Country of Publication:
United States
Language:
English
Subject:
46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND TECHNOLOGY; Radioxenon; Beta-Gamma Coincidence; PIPSBox; CZT; Nuclear Explosion Monitoring; CTBTO

Citation Formats

Czyz, Steven A., Farsoni, Abi T., and Gadey, Harish R. Evaluation of a semiconductor-based atmospheric radioxenon detection system. United States: N. p., 2019. Web. doi:10.1016/j.nima.2019.162614.
Czyz, Steven A., Farsoni, Abi T., & Gadey, Harish R. Evaluation of a semiconductor-based atmospheric radioxenon detection system. United States. https://doi.org/10.1016/j.nima.2019.162614
Czyz, Steven A., Farsoni, Abi T., and Gadey, Harish R. Tue . "Evaluation of a semiconductor-based atmospheric radioxenon detection system". United States. https://doi.org/10.1016/j.nima.2019.162614. https://www.osti.gov/servlets/purl/1798657.
@article{osti_1798657,
title = {Evaluation of a semiconductor-based atmospheric radioxenon detection system},
author = {Czyz, Steven A. and Farsoni, Abi T. and Gadey, Harish R.},
abstractNote = {A prototype radioxenon detection system for beta–gamma coincidence measurements has been designed using a PIPSBox and a pair of coplanar CdZnTe (CZT) detectors. Coincidence events are identified in real-time using a Field-Programmable Gate Array (FPGA). The measurement of 131mXe and studies on electron backscatter and memory effect in the PIPSBox have been presented previously; this paper details the measurement of 133/133mXe, 135Xe, and background. Here, absolute efficiencies were determined, regions of interest were defined, and Minimum Detectable Concentrations (MDC) for all four radioxenon isotopes were calculated. When neglecting interferences between the radioxenons, the prototype system has an estimated MDC of 0.61 ± 0.15 mBq/m3 for 133Xe when using gas processing parameters associated with Xenon International, satisfying the CTBTO requirement for sensitivity of ≤1 mBq/m3 for 133Xe. Simulation suggests that by increasing number of CZT detectors used by a factor of 16, the MDCs of the system can be improved by a factor of 2-3. The design shows great promise for future improvement and expansion due to its exceptional energy resolution, high background rejection rate, room temperature operation, minimal memory effect, and simple readout electronics.},
doi = {10.1016/j.nima.2019.162614},
journal = {Nuclear Instruments and Methods in Physics Research. Section A, Accelerators, Spectrometers, Detectors and Associated Equipment},
number = ,
volume = 945,
place = {United States},
year = {Tue Aug 27 00:00:00 EDT 2019},
month = {Tue Aug 27 00:00:00 EDT 2019}
}

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Cited by: 5 works
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Works referenced in this record:

Atmospheric xenon radioactive isotope monitoring
journal, January 2004

  • Fontaine, J.-P.; Pointurier, F.; Blanchard, X.
  • Journal of Environmental Radioactivity, Vol. 72, Issue 1-2, p. 129-135
  • DOI: 10.1016/S0265-931X(03)00194-2

Absolute Efficiency Calibration of a Beta-Gamma Detector
journal, April 2013

  • Cooper, Matthew W.; Ely, James H.; Haas, Derek A.
  • IEEE Transactions on Nuclear Science, Vol. 60, Issue 2
  • DOI: 10.1109/TNS.2013.2243165

The АРИКС-01 Automatic Facility for Measuring Concentrations of Radioactive Xenon Isotopes in the Atmosphere
journal, May 2005

  • Dubasov, Yu. V.; Popov, Yu. S.; Prelovskii, V. V.
  • Instruments and Experimental Techniques, Vol. 48, Issue 3
  • DOI: 10.1007/s10786-005-0065-3

Improved performance comparisons of radioxenon systems for low level releases in nuclear explosion monitoring
journal, November 2017


Low-level activity measurement of 131Xem, 133Xem, 135Xe and 133Xe in atmospheric air samples using high-resolution dual X–γ spectrometry
journal, October 2006


Spalax™ new generation: A sensitive and selective noble gas system for nuclear explosion monitoring
journal, September 2015


Characteristics of depth-sensing coplanar grid CdZnTe detectors
journal, December 2005

  • He, Zhong; Sturm, Ben W.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 554, Issue 1-3, p. 291-299
  • DOI: 10.1016/j.nima.2005.06.064

Improvements of low-level radioxenon detection sensitivity by a state-of-the art coincidence setup
journal, May 2014


The ARIX-03F mobile semiautomatic facility for measuring low concentrations of radioactive xenon isotopes in air and subsoil gas
journal, May 2007

  • Prelovskii, V. V.; Kazarinov, N. M.; Donets, A. Yu.
  • Instruments and Experimental Techniques, Vol. 50, Issue 3
  • DOI: 10.1134/S0020441207030165

A Phoswich Detector With Compton Suppression Capability for Radioxenon Measurements
journal, February 2013

  • Farsoni, Abi T.; Alemayehu, Bemnet; Alhawsawi, Abdulsalam
  • IEEE Transactions on Nuclear Science, Vol. 60, Issue 1
  • DOI: 10.1109/TNS.2012.2226606

Memory effect, resolution, and efficiency measurements of an Al2O3 coated plastic scintillator used for radioxenon detection
journal, June 2013

  • Bläckberg, L.; Fritioff, T.; Mårtensson, L.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 714
  • DOI: 10.1016/j.nima.2013.02.045

A radioxenon detection system using CdZnTe, an array of SiPMs, and a plastic scintillator
journal, May 2017

  • Czyz, Steven A.; Farsoni, Abi T.
  • Journal of Radioanalytical and Nuclear Chemistry, Vol. 313, Issue 1
  • DOI: 10.1007/s10967-017-5287-x

Measurements of ambient radioxenon levels using the automated radioxenon sampler/analyzer (ARSA)
journal, January 2001

  • McIntyre, J. I.; Abel, K. H.; Bowyer, T. W.
  • Journal of Radioanalytical and Nuclear Chemistry, Vol. 248, Issue 3, p. 629-635
  • DOI: 10.1023/A:1010672107749

Evaluation of phoswich well detectors for radioxenon monitoring
conference, October 2007

  • Hennig, Wolfgang; Tan, Hui; Warburton, William K.
  • 2007 IEEE Nuclear Science Symposium Conference Record
  • DOI: 10.1109/NSSMIC.2007.4436439

Global radioxenon emission inventory based on nuclear power reactor reports
journal, January 2009


Redesigned β–γ radioxenon detector
journal, August 2007

  • Cooper, Matthew W.; McIntyre, Justin I.; Bowyer, Ted W.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 579, Issue 1
  • DOI: 10.1016/j.nima.2007.04.092

A CZT-based radioxenon detection system in support of the Comprehensive Nuclear-Test-Ban Treaty
journal, May 2016

  • Ranjbar, Lily; Farsoni, Abi T.; Becker, Eric M.
  • Journal of Radioanalytical and Nuclear Chemistry, Vol. 310, Issue 3
  • DOI: 10.1007/s10967-016-4872-8

Innovative concept for a major breakthrough in atmospheric radioactive xenon detection for nuclear explosion monitoring
journal, May 2013

  • Le Petit, G.; Cagniant, A.; Morelle, M.
  • Journal of Radioanalytical and Nuclear Chemistry, Vol. 298, Issue 2
  • DOI: 10.1007/s10967-013-2525-8

A stilbene - CdZnTe based radioxenon detection system
journal, August 2019


Contribution to the development of atmospheric radioxenon monitoring
journal, May 2008

  • Le Petit, G.; Armand, P.; Brachet, G.
  • Journal of Radioanalytical and Nuclear Chemistry, Vol. 276, Issue 2
  • DOI: 10.1007/s10967-008-0517-x

135Xe measurements with a two-element CZT-based radioxenon detector for nuclear explosion monitoring
journal, April 2017


Comparison of new and existing algorithms for the analysis of 2D radioxenon beta gamma spectra
journal, January 2017

  • Deshmukh, Nikhil; Prinke, Amanda; Miller, Brian
  • Journal of Radioanalytical and Nuclear Chemistry, Vol. 311, Issue 3
  • DOI: 10.1007/s10967-017-5174-5