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Title: Newly Evaluated Neutron Reaction Data on Chromium Isotopes

Journal Article · · Nuclear Data Sheets
 [1]; ORCiD logo [2];  [1];  [3];  [4]; ORCiD logo [2];  [1];  [5];  [1]; ORCiD logo [2];  [4];  [6];  [6]
  1. Brookhaven National Lab. (BNL), Upton, NY (United States)
  2. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
  3. International Atomic Energy Agency (IAEA), Vienna (Austria)
  4. Jozef Stefan Inst. (IJS), Ljubljana (Slovenia)
  5. Gonzaga Univ., Spokane, WA (United States)
  6. Alternative Energies and Atomic Energy Commission (CEA), Saint-Paul-Lez-Durance (France)

In this work, neutron reaction data for the set of major chromium isotopes were reevaluated from the thermal energy range up to 20 MeV. In the low energy region, updates to the thermal values together with an improved R-matrix analysis of the resonance parameters characterizing the cluster of large s-wave resonances for 50,53Cr isotopes were performed. In the intermediate and high energy range up to 20 MeV, the evaluation methodology used statistical nuclear reaction models implemented in the EMPIRE code within the Hauser-Feshbach framework to evaluate the reaction cross sections and angular distributions. Exceptionally, experimental data were used to evaluate relevant cross sections above the resonance region up to 5 MeV in the major 52Cr isotope. Evaluations were benchmarked with Monte Carlo simulations of a small suite of critical assemblies highly sensitive to Chromium data, and with the Oktavian shielding benchmark to judge deep penetration performance with a 14-MeV D-T neutron source. A significant improvement in performance is demonstrated compared to existing evaluations.

Research Organization:
Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States); Brookhaven National Laboratory (BNL), Upton, NY (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Nuclear Physics (NP); USDOE National Nuclear Security Administration (NNSA), Nuclear Criticality Safety Program (NCSP)
Grant/Contract Number:
AC05-00OR22725; SC0012704
OSTI ID:
1798579
Alternate ID(s):
OSTI ID: 1788066
Report Number(s):
BNL-221625-2021-JAAM; TRN: US2210690
Journal Information:
Nuclear Data Sheets, Vol. 173; ISSN 0090-3752
Publisher:
ElsevierCopyright Statement
Country of Publication:
United States
Language:
English

References (120)

Impact of the ENDF/B-VIII.0 library on modeling nuclear tools for oil exploration journal January 2020
Thermal Neutron Activation Cross Sections journal November 1947
JENDL-4.0: A New Library for Nuclear Science and Engineering journal January 2011
The experimental nuclear reaction data (EXFOR): Extended computer database and Web retrieval system
  • Zerkin, V. V.; Pritychenko, B.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 888 https://doi.org/10.1016/j.nima.2018.01.045
journal April 2018
Recherche d'une structure intermédiaire dans les sections efficaces totales neutroniques journal September 1967
Cross-Section Measurement for the 52 Cr( n,p ) 52 V Reaction Near Threshold journal October 1980
Angular distributions in a unified model of preequilibrium and equilibrium neutron emission journal July 1980
Gamma rays resulting from nonelastic processes of 14·2 MeV neutrons with sodium, magnesium, silicon, sulphur, titanium, chromium and iron journal April 1973
Measurement of the cross sections for the reactions 52Cr(n,2n)51Cr, 66Zn(n,2n)65Zn, 89Y(n,2n)88Y and 96Zr(n,2n)95Zr from 13.5 to 14.8 MeV journal January 1989
Neutron resonance spectroscopy for n + 52 Cr : Total and differential elastic scattering cross sections journal June 2000
(3He, α) reactions on the chromium isotopes journal April 1969
The systematics of nuclear bound states journal December 1978
Inelastic Scattering of 14MeV Neutrons by Medium Weight Nuclei journal May 1972
Neutron elastic and inelastic scattering from Mg, Si, S, Ca, Cr, Fe and Ni AT En = 21.6 MeV journal July 1990
Approximation of Precompound Effects in Hauser-Feshbach Codes for Calculating Double Differential ( n, xn ) Cross Sections journal September 1988
14·8 MeV neutron activation cross sections for chromium journal November 1967
Measurement of the 53 Cr( n, p ) 53 V Cross Section Below 9.4 MeV Using a Sample Transport Facility journal August 1981
High resolution measurement of neutron inelastic scattering and () cross-sections for 52Cr journal April 2007
High-resolution transmission measurements for Cr 54 + n journal October 2006
Strength function fluctuations in the mass region of the 3s resonance journal March 1971
Thermal neutron capture cross section for Fe 56 ( n , γ ) journal January 2017
A Composite Nuclear-Level Density Formula with Shell Corrections journal August 1965
Neutron Cross-Section Measurements on Structural Materials at ORELA journal August 2011
keV neutron radiative capture and total cross section of 50, 52, 53Cr, 54, 57Fe, and 62, 64Ni journal March 1975
Reactor Neutron Activation Cross Sections for a Number of Elements journal November 1960
The thermal neutron cross-sections and resonance integrals of 50Cr, 109Ag, 123Sb, 133Cs, 191Ir and 202Hg journal February 1968
Nuclear data for accelerator-driven systems journal January 2001
Cross-section measurements for the Fe 57 ( n , n γ ) Fe 57 and Fe 57 ( n , 2 n γ ) Fe 56 reactions journal August 2017
Pile Neutron Absorption Cross Sections journal November 1950
Gamma Rays from Inelastic Neutron Scattering in Chromium journal November 1962
A compilation of infinite dilution resonance integrals, I journal June 1972
Updating and Extending the IRDF-2002 Dosimetry Library journal April 2012
Thermal Neutron Capture Cross Sections journal October 1952
Nucleon-Nucleus Optical-Model Parameters, A > 40 , E < 50 MeV journal June 1969
Neutron Inelastic Scattering Cross Sections for Natural Chromium Determined from the ( n,n′γ ) Reaction journal July 1978
Capture cross sections for neutrons of energy up to 50 kev for Cr, Cr50, Cr53, Cr53 nuclei (E) journal March 1964
Local and global nucleon optical models from 1 keV to 200 MeV journal January 2003
Nuclear data sheets for A = 52 journal October 1978
Direct neutron capture for magic-shell nuclei journal January 1996
Measurement of neutron total cross sections up to 560 MeV journal March 2001
Nonstatistical effects observed with Cr 52 + n resonances journal February 1989
Cross-Section Measurements of ( n,p ) and ( n,np + pn + d ) Reactions for Some Titanium, Chromium, Iron, Cobalt, Nickel, and Zinc Isotopes around 14 MeV journal July 1991
Experimental determination of k 0, Q 0 factors, effective resonance energies and neutron cross-sections for 37 isotopes of interest in NAA journal July 2014
Gamma-ray spectra and level structure of 55Cr from thermal neutron capture in 54Cr journal May 1972
Total cross-section of chromium at low neutron energies journal January 1976
Slow Neutron Velocity Spectrometer Studies. V. Re, Ta, Ru, Cr, Ga journal November 1953
Cross-sections of a few (n,α) and (n, p) reactions induced at 14.7 MeV neutrons journal November 1991
ENDF/B-VIIIβ4 benchmark test with iron and concrete shielding experiments using 40 and 65 MeV neutrons at QST/TIARA journal November 2018
s- and p-wave neutron spectroscopy journal May 1966
Pre-equilibrium emission effect in (n, p) reaction cross-sections at 14.8 MeV journal April 1985
s Wave resonances with square well potentials journal December 1976
Phenomenology of continuum angular distributions. I. Systematics and parametrization journal January 1981
Thermal Neutron Capture Cross Sections journal August 1951
Parity dependence of the level densities of Cr 53 and Cr 55 at high excitation journal December 1984
Cross sections for (n, p) and (n, ?) reactions on chromium, iron, copper, and molybdenum nuclei at a neutron energy of 14.8 MeV journal September 1980
Use the results of measurements on KBR facility for testing of neutron data of main structural materials for fast reactors journal January 2017
EMPIRE: Nuclear Reaction Model Code System for Data Evaluation journal December 2007
Neutron scattering and models: chromium journal February 1997
The Total, Elastic and Inelastic Scattering Fast Neutron Cross Sections of Natural Chromium journal December 1982
Direct-Semidirect Neutron Capture Calculations Applied to R-Matrix Data Evaluations in the Resolved Resonance Region conference January 2005
Evaluation of 50Cr, 52Cr, 53Cr, 54Cr Neutron Cross Section Data for Energies up to 200 MeV journal August 2011
Nuclear Data Sheets for A = 55 journal April 2008
Global deuteron optical model potential for the energy range up to 183 MeV journal May 2006
Pile Neutron Absorption Cross Sections of some of the Elements journal October 1950
Statistical Model of Intermediate Structure journal August 1966
Thermal neutron capture cross-section of 48Ti, 51V, 50,52,53Cr and 58,60,62,64Ni journal April 1997
Spectroscopic factors for ln = 1 and ln = 3 transitions in (d, p) reactions with some calcium and chromium nuclei journal September 1970
Neutron Total Cross Sections of Chromium and Iron in the kev Region journal October 1957
The OKTAVIAN TOF experiments in SINBAD: Evaluation of the experimental uncertainties journal April 2010
A systematic study of (n, p) reactions at 14.7 MeV journal June 1977
Capture Cross Sections for Slow Neutrons journal May 1946
The measurement of the resonance integrals for neutron absorption journal December 1957
IRDFF-II: A New Neutron Metrology Library journal January 2020
keV neutron capture and transmission measurements on 50Cr, 52Cr, 53Cr, 54Cr, 60Ni and V journal March 1971
Excitation functions of ( n , 2 n ) , ( n , p ) , ( n , n p + p n + d ) , and ( n , α ) reactions on isotopes of chromium journal August 1998
Evaluation of the Chromium Resonance Parameters Including Resonance Parameter Covariance journal August 2011
A study of the 54Cr(d, p)55Cr and 53Cr(t, p)55Cr reactions journal December 1972
Preparation and Half-Life of Cr 55 journal August 1954
Cross Sections for Gamma-Ray Production by 14-MeV Neutrons journal January 1978
Cross section and neutron angular distribution measurements of neutron scattering on natural iron journal February 2019
Measurement of (n, p) cross-sections for shortlived products by 13.4–14.9 MeV neutrons journal January 1998
Systematic study of direct neutron capture journal October 2012
ENDF/B-VIII.0: The 8 th Major Release of the Nuclear Reaction Data Library with CIELO-project Cross Sections, New Standards and Thermal Scattering Data journal February 2018
Evaluation of Neutron Reactions on Iron Isotopes for CIELO and ENDF/B-VIII.0 journal February 2018
Nuclear Data Sheets for A = 51 journal August 2006
Neutron Total Cross Sections, 2.5-15 MeV. I. Experimental journal February 1971
The calculation of neutron cross-sections from optical potentials journal June 1964
Calculation of the ORELA neutron moderator spectrum and resolution function journal June 1983
Resonance neutron capture in 52Cr journal January 1980
Dispersive coupled-channels optical-model potential with soft-rotator couplings for Cr, Fe, and Ni isotopes journal May 2013
Fluctuation effects in radiative capture to unstable final states: A test via the Y 89 ( p →,γ) reaction at E p =19.6 MeV journal July 1995
Cr 53 ( n , n ’ γ) reactions and the level structure of Cr 53 journal May 1989
Bestimmung von (n n'γ)-Querschnitten für 14,4 MeV-Neutronen im Massebereich A = 46 — 88 journal March 1971
Gamma-ray production from52Cr(n, xγ) reactions at 14.6 MeV journal July 1992
Nuclear Data Sheets for A = 54 journal June 2006
Global optical potentials for emitted alpha particles journal April 1994
Constraining level densities through quantitative correlations with cross-section data journal March 2020
Neutron activation cross-sections for Cr isotopes at 14.6 MeV neutron energy journal January 1985
Analyses of iron and concrete shielding experiments at JAEA/TIARA with JENDL/HE-2007, ENDF/B-VII.1 and FENDL-3.0 journal October 2015
Critical evaluation and experimental determination of the nuclear activation and decay parameters for the reactions:50Cr(n, ψ)51Cr,58Fe(n, ψ)59Fe,109Ag(n, ψ)110mAg journal February 1984
The joint evaluated fission and fusion nuclear data library, JEFF-3.3 journal July 2020
Measurement of the Neutron Activation Cross Sections of 12 C, 30 Si, 47 Ti, 48 Ti, 52 Cr, 59 Co, and 58 Ni Between 15 and 40 MeV journal February 1996
The excitation function for the reaction 52Cr(n, 2n)51Cr journal January 1989
Excitation of low-lying levels of Al27, Cr52, Fe56, and Bi20.9 in the inelastic scattering of 1?4 MeV neutrons journal December 1967
Activation analysis of high-purity silicon: III. Multi-element activation analysis: Application of the triple comparator method journal October 1971
Neutron activation cross-sections for Cr isotopes at 14.6 MeV neutron energy journal January 1985
The excitation function for the reaction 52Cr(n, 2n)51Cr journal January 1989
Resonance neutron capture in 52Cr journal January 1980
The OKTAVIAN TOF experiments in SINBAD: Evaluation of the experimental uncertainties journal April 2010
Nuclear Data Sheets for A = 54 journal June 2006
Nuclear Data Sheets for A = 51 journal August 2006
Nuclear Data Sheets for A = 55 journal April 2008
Nuclear reactions with 14 MeV neutrons and bremsstrahlungs in giant dipole resonance (GDR) region using small accelerators journal July 2003
Impact of the ENDF/B-VIII.0 library on modeling nuclear tools for oil exploration journal January 2020
Interaction of Neutrons with Matter journal August 1935
Capture Cross Sections for Slow Neutrons. II. Small Capture Cross Sections journal July 1946
Low Energy Neutron Resonance Scattering and Absorption journal July 1950
Neutron Total Cross Sections, 2.5-15 MeV. II. Effects of Nuclear Deformation journal February 1971
Bestimmung von (n n'γ)-Querschnitten für 14,4 MeV-Neutronen im Massebereich A = 46 — 88 journal March 1971
The Total Neutron Cross Sections of ⁵⁰Cr, ⁵²Cr, ⁶²Ni and ⁶⁴Ni in the Energy Region 10 - 300 keV text January 1972

Figures / Tables (58)