A review of composite solid-state electrolytes for lithium batteries: fundamentals, key materials and advanced structures
Abstract
All-solid-state lithium ion batteries (ASSLBs) are considered next-generation devices for energy storage due to their advantages in safety and potentially high energy density. As the key component in ASSLBs, solid-state electrolytes (SSEs) with non-flammability and good adaptability to lithium metal anodes have attracted extensive attention in recent years. Among the current SSEs, composite solid-state electrolytes (CSSEs) with multiple phases have greater flexibility to customize and combine the advantages of single-phase electrolytes, which have been widely investigated recently and regarded as promising candidates for commercial ASSLBs. Based on existing investigations, herein, we present a comprehensive overview of the recent developments in CSSEs. Initially, we introduce the historical development from solid-state ionic conductors to CSSEs, and then summarize the fundamentals including mechanisms of lithium ion transport, key evaluation parameters, design principles, and key materials. Finally, four main types of advanced structures for CSSEs are classified and highlighted according to the recent progress. Moreover, advanced characterization and computational simulation techniques including machine learning are reviewed for the first time, and the main challenges and perspectives of CSSEs are also provided for their future development.
- Authors:
-
[4];
[1];
[1]
- Univ. of Waterloo, ON (Canada)
- Hong Kong Univ. of Science and Technology, Kowloon (Hong Kong)
- Univ. of Waterloo, ON (Canada); Argonne National Lab. (ANL), Argonne, IL (United States)
- Argonne National Lab. (ANL), Argonne, IL (United States)
- Publication Date:
- Research Org.:
- Argonne National Laboratory (ANL), Argonne, IL (United States)
- Sponsoring Org.:
- USDOE Office of Energy Efficiency and Renewable Energy (EERE), Transportation Office; Natural Sciences and Engineering Research Council of Canada (NSERC); USDOE
- OSTI Identifier:
- 1798040
- Alternate Identifier(s):
- OSTI ID: 1690288
- Grant/Contract Number:
- AC02-06CH11357
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Chemical Society Reviews
- Additional Journal Information:
- Journal Volume: 49; Journal Issue: 23; Journal ID: ISSN 0306-0012
- Publisher:
- Royal Society of Chemistry
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 25 ENERGY STORAGE
Citation Formats
Zheng, Yun, Yao, Yuze, Ou, Jiahua, Li, Matthew, Luo, Dan, Dou, Haozhen, Li, Zhaoqiang, Amine, Khalil, Yu, Aiping, and Chen, Zhongwei. A review of composite solid-state electrolytes for lithium batteries: fundamentals, key materials and advanced structures. United States: N. p., 2020.
Web. doi:10.1039/d0cs00305k.
Zheng, Yun, Yao, Yuze, Ou, Jiahua, Li, Matthew, Luo, Dan, Dou, Haozhen, Li, Zhaoqiang, Amine, Khalil, Yu, Aiping, & Chen, Zhongwei. A review of composite solid-state electrolytes for lithium batteries: fundamentals, key materials and advanced structures. United States. https://doi.org/10.1039/d0cs00305k
Zheng, Yun, Yao, Yuze, Ou, Jiahua, Li, Matthew, Luo, Dan, Dou, Haozhen, Li, Zhaoqiang, Amine, Khalil, Yu, Aiping, and Chen, Zhongwei. Tue .
"A review of composite solid-state electrolytes for lithium batteries: fundamentals, key materials and advanced structures". United States. https://doi.org/10.1039/d0cs00305k. https://www.osti.gov/servlets/purl/1798040.
@article{osti_1798040,
title = {A review of composite solid-state electrolytes for lithium batteries: fundamentals, key materials and advanced structures},
author = {Zheng, Yun and Yao, Yuze and Ou, Jiahua and Li, Matthew and Luo, Dan and Dou, Haozhen and Li, Zhaoqiang and Amine, Khalil and Yu, Aiping and Chen, Zhongwei},
abstractNote = {All-solid-state lithium ion batteries (ASSLBs) are considered next-generation devices for energy storage due to their advantages in safety and potentially high energy density. As the key component in ASSLBs, solid-state electrolytes (SSEs) with non-flammability and good adaptability to lithium metal anodes have attracted extensive attention in recent years. Among the current SSEs, composite solid-state electrolytes (CSSEs) with multiple phases have greater flexibility to customize and combine the advantages of single-phase electrolytes, which have been widely investigated recently and regarded as promising candidates for commercial ASSLBs. Based on existing investigations, herein, we present a comprehensive overview of the recent developments in CSSEs. Initially, we introduce the historical development from solid-state ionic conductors to CSSEs, and then summarize the fundamentals including mechanisms of lithium ion transport, key evaluation parameters, design principles, and key materials. Finally, four main types of advanced structures for CSSEs are classified and highlighted according to the recent progress. Moreover, advanced characterization and computational simulation techniques including machine learning are reviewed for the first time, and the main challenges and perspectives of CSSEs are also provided for their future development.},
doi = {10.1039/d0cs00305k},
journal = {Chemical Society Reviews},
number = 23,
volume = 49,
place = {United States},
year = {Tue Oct 27 00:00:00 EDT 2020},
month = {Tue Oct 27 00:00:00 EDT 2020}
}
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