Magnetic Dynamic Polymers for Modular Assembling and Reconfigurable Morphing Architectures

Kuang, Xiao; Wu, Shuai; Ze, Qiji; Yue, Liang; Jin, Yi; Montgomery, S. Macrae; Yang, Fengyuan; Qi, H. Jerry; Zhao, Ruike

doi:10.1002/adma.202102113

Title: Magnetic Dynamic Polymers for Modular Assembling and Reconfigurable Morphing Architectures

Journal Article · 18 June 2021 · Advanced Materials

DOI: https://doi.org/10.1002/adma.202102113 · OSTI ID:1797834

Kuang, Xiao ^[1]; Wu, Shuai ^[2]; Ze, Qiji ^[2]; Yue, Liang ^[1]; Jin, Yi ^[2]; Montgomery, S. Macrae ^[1]; Yang, Fengyuan ^[3];

^[1];

^[2]

The George W. Woodruff School of Mechanical Engineering Georgia Institute of Technology Atlanta GA 30332 USA
Department of Mechanical and Aerospace Engineering The Ohio State University Columbus OH 43210 USA
Department of Physics The Ohio State University Columbus OH 43210 USA

Abstract Shape‐morphing magnetic soft materials, composed of magnetic particles in a soft polymer matrix, can transform shape reversibly, remotely, and rapidly, finding diverse applications in actuators, soft robotics, and biomedical devices. To achieve on‐demand and sophisticated shape morphing, the manufacture of structures with complex geometry and magnetization distribution is highly desired. Here, a magnetic dynamic polymer (MDP) composite composed of hard‐magnetic microparticles in a dynamic polymer network with thermally responsive reversible linkages, which permits functionalities including targeted welding for magnetic‐assisted assembly, magnetization reprogramming, and permanent structural reconfiguration, is reported. These functions not only provide highly desirable structural and material programmability and reprogrammability but also enable the manufacturing of functional soft architected materials such as 3D kirigami with complex magnetization distribution. The welding of magnetic‐assisted modular assembly can be further combined with magnetization reprogramming and permanent reshaping capabilities for programmable and reconfigurable architectures and morphing structures. The reported MDP are anticipated to provide a new paradigm for the design and manufacture of future multifunctional assemblies and reconfigurable morphing architectures and devices.

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Sponsoring Organization:: USDOE

Grant/Contract Number:: SC0001304

OSTI ID:: 1797834

Journal Information:: Advanced Materials, Journal Name: Advanced Materials Journal Issue: 30 Vol. 33; ISSN 0935-9648

Publisher:: Wiley Blackwell (John Wiley & Sons)Copyright Statement

Country of Publication:: Germany

Language:: English

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