Doubling the Stakes: The Promise of Halide Double Perovskites

Wolf, Nathan R.; Connor, Bridget A.; Slavney, Adam H.; Karunadasa, Hemamala I.

doi:10.1002/ange.202016185

Title: Doubling the Stakes: The Promise of Halide Double Perovskites

Journal Article · 26 March 2021 · Angewandte Chemie

DOI: https://doi.org/10.1002/ange.202016185 · OSTI ID:1786080

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Department of Chemistry Stanford University Stanford California 94305 USA
Department of Chemistry Stanford University Stanford California 94305 USA, Stanford Institute for Materials and Energy Sciences SLAC National Accelerator Laboratory Menlo Park California 94025 USA

Abstract When the stakes are doubled in a wager, a player must correctly place two consecutive bets to win, but the payout is larger. Similarly, two B sites in combination dictate the properties of A ₂ BB′X ₆ (A=monocation, X=halide) double perovskites. Correctly picking two B sites is more challenging than picking just one, as in the A ^I B ^II X ₃ single perovskites, but the options are greater and, we believe, the rewards are higher when the stakes are doubled. In this Minireview, we emphasize fundamental aspects of halide double perovskites to provide a foundation for interested readers to explore this extraordinary class of materials. In particular, we highlight the differences and similarities between double and single perovskites and describe how the double perovskite structure potentially offers greater control over photophysical properties.

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Sponsoring Organization:: USDOE

Grant/Contract Number:: AC02-76SF00515

OSTI ID:: 1786080

Journal Information:: Angewandte Chemie, Journal Name: Angewandte Chemie Journal Issue: 30 Vol. 133; ISSN 0044-8249

Publisher:: Wiley Blackwell (John Wiley & Sons)Copyright Statement

Country of Publication:: Germany

Language:: English

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