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Title: Topological Nernst effect, anomalous Nernst effect, and anomalous thermal Hall effect in the Dirac semimetal Fe 3 Sn 2

Abstract

Topological semimetals have been a focal point of research in recent years. One of the salient characters of topological semimetals is the anomalous Hall effect arising from the nontrivial momentum-space Berry phase. In contrast, anomalous transverse thermoelectric coefficient and thermal Hall effect are much less explored up to date. In this paper, we report thermoelectric and thermal transport properties of Fe3Sn2, a prototypical Dirac semimetal. We find that Fe3Sn2 exhibits large topological Nernst effect which is associated with the non-zero spin chirality of the skyrmion bubble phase. Furthermore, Fe3Sn2 shows prominent anomalous thermal Hall effect and anomalous Nernst effect with features similar to the anomalous Hall effect. The anomalous Nernst signal is about 2.1 μV/K at room temperature, which is comparable to the largest value reported thus far. These results highlight the synergic effects of Berry phase in both real space and momentum space of Fe3Sn2, and this study demonstrates an effective strategy of investigating topological materials by measuring their transverse thermal and thermoelectric responses.

Authors:
ORCiD logo [1];  [2]; ORCiD logo [1]
  1. Michigan State Univ., East Lansing, MI (United States)
  2. Michigan State Univ., East Lansing, MI (United States); Southeast Univ., Nanjing (China)
Publication Date:
Research Org.:
Michigan State Univ., East Lansing, MI (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division
OSTI Identifier:
1780856
Grant/Contract Number:  
SC0019259
Resource Type:
Accepted Manuscript
Journal Name:
Physical Review B
Additional Journal Information:
Journal Volume: 103; Journal Issue: 20; Journal ID: ISSN 2469-9950
Publisher:
American Physical Society (APS)
Country of Publication:
United States
Language:
English
Subject:
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY

Citation Formats

Zhang, H., Xu, C.Q., and Ke, Xianglin. Topological Nernst effect, anomalous Nernst effect, and anomalous thermal Hall effect in the Dirac semimetal Fe 3 Sn 2. United States: N. p., 2021. Web. doi:10.1103/physrevb.103.l201101.
Zhang, H., Xu, C.Q., & Ke, Xianglin. Topological Nernst effect, anomalous Nernst effect, and anomalous thermal Hall effect in the Dirac semimetal Fe 3 Sn 2. United States. https://doi.org/10.1103/physrevb.103.l201101
Zhang, H., Xu, C.Q., and Ke, Xianglin. Mon . "Topological Nernst effect, anomalous Nernst effect, and anomalous thermal Hall effect in the Dirac semimetal Fe 3 Sn 2". United States. https://doi.org/10.1103/physrevb.103.l201101. https://www.osti.gov/servlets/purl/1780856.
@article{osti_1780856,
title = {Topological Nernst effect, anomalous Nernst effect, and anomalous thermal Hall effect in the Dirac semimetal Fe 3 Sn 2},
author = {Zhang, H. and Xu, C.Q. and Ke, Xianglin},
abstractNote = {Topological semimetals have been a focal point of research in recent years. One of the salient characters of topological semimetals is the anomalous Hall effect arising from the nontrivial momentum-space Berry phase. In contrast, anomalous transverse thermoelectric coefficient and thermal Hall effect are much less explored up to date. In this paper, we report thermoelectric and thermal transport properties of Fe3Sn2, a prototypical Dirac semimetal. We find that Fe3Sn2 exhibits large topological Nernst effect which is associated with the non-zero spin chirality of the skyrmion bubble phase. Furthermore, Fe3Sn2 shows prominent anomalous thermal Hall effect and anomalous Nernst effect with features similar to the anomalous Hall effect. The anomalous Nernst signal is about 2.1 μV/K at room temperature, which is comparable to the largest value reported thus far. These results highlight the synergic effects of Berry phase in both real space and momentum space of Fe3Sn2, and this study demonstrates an effective strategy of investigating topological materials by measuring their transverse thermal and thermoelectric responses.},
doi = {10.1103/physrevb.103.l201101},
journal = {Physical Review B},
number = 20,
volume = 103,
place = {United States},
year = {Mon May 03 00:00:00 EDT 2021},
month = {Mon May 03 00:00:00 EDT 2021}
}

Works referenced in this record:

Large anomalous Nernst effect at room temperature in a chiral antiferromagnet
journal, July 2017

  • Ikhlas, Muhammad; Tomita, Takahiro; Koretsune, Takashi
  • Nature Physics, Vol. 13, Issue 11
  • DOI: 10.1038/nphys4181

Room‐Temperature Skyrmion Thermopower in Fe 3 Sn 2
journal, September 2020

  • Du, Qianheng; Han, Myung‐Geun; Liu, Yu
  • Advanced Quantum Technologies, Vol. 3, Issue 10
  • DOI: 10.1002/qute.202000058

Finite-temperature violation of the anomalous transverse Wiedemann-Franz law
journal, April 2020


Giant anomalous Hall effect in a ferromagnetic kagome-lattice semimetal
journal, July 2018


Mott's formula for the thermopower and the Wiedemann-Franz law
journal, May 1980


Skyrmions and anomalous Hall effect in a Dzyaloshinskii-Moriya spiral magnet
journal, August 2009


Anomalous Nernst Effect in the Dirac Semimetal Cd 3 As 2
journal, March 2017


Magnetic-Field Control of Topological Electronic Response near Room Temperature in Correlated Kagome Magnets
journal, November 2019


Non-collinearity and spin frustration in the itinerant kagome ferromagnet Fe 3 Sn 2
journal, October 2009


Ueber die Wärme-Leitungsfähigkeit der Metalle
journal, January 1853


The Connections between the Four Transverse Galvanomagnetic and Thermomagnetic Phenomena
journal, December 1924


Giant anomalous Nernst effect and quantum-critical scaling in a ferromagnetic semimetal
journal, July 2018


Massive Dirac fermions in a ferromagnetic kagome metal
journal, March 2018


Real-Space and Reciprocal-Space Berry Phases in the Hall Effect of Mn 1 x Fe x Si
journal, May 2014


Topological Nernst effect in a three-dimensional skyrmion-lattice phase
journal, August 2013


Giant anomalous Nernst effect in the magnetic Weyl semimetal Co 3 Sn 2 S 2
journal, February 2020


Enhanced anomalous Nernst effect in disordered Dirac and Weyl materials
journal, February 2021


Dirac fermions and flat bands in the ideal kagome metal FeSn
journal, December 2019


Intrinsic Anomalous Nernst Effect Amplified by Disorder in a Half-Metallic Semimetal
journal, December 2019


Anomalous Nernst effect beyond the magnetization scaling relation in the ferromagnetic Heusler compound Co2MnGa
journal, April 2019


Berry curvature unravelled by the anomalous Nernst effect in Mn 3 Ge
journal, August 2019


Large topological Hall effect in a geometrically frustrated kagome magnet Fe 3 Sn 2
journal, May 2019

  • Li, Hang; Ding, Bei; Chen, Jie
  • Applied Physics Letters, Vol. 114, Issue 19
  • DOI: 10.1063/1.5088173

Nernst effect in metals and superconductors: a review of concepts and experiments
journal, March 2016


Berry-Phase Effect in Anomalous Thermoelectric Transport
journal, July 2006


Magnetotransport as a diagnostic of spin reorientation: Kagome ferromagnet as a case study
journal, December 2019


Anomalous Hall effect
journal, May 2010


Topological Nernst Effect of the Two-Dimensional Skyrmion Lattice
journal, August 2020