Valuation of Surface Coatings in High-Energy Density Lithium-ion Battery Cathode Materials

Nisar, Umair; Muralidharan, Nitin; Essehli, Rachid; Amin, Ruhul; Belharouak, Ilias

doi:10.1016/j.ensm.2021.03.015

Title: Valuation of Surface Coatings in High-Energy Density Lithium-ion Battery Cathode Materials

Abstract

Artificial barriers, usually with either electrochemically active or inactive coating materials, are deployed on cathode material surfaces to mitigate detrimental side reactions by suppressing direct contact of cathode and electrolyte called surface coatings. These surface coatings are commonly known to increase the wettability of liquid electrolyte and reduce the interfacial charge transfer resistance. An important caveat is the selection of appropriate coating material with appropriate thickness for achieving enhanced electrochemical performance. As modern battery materials are increasingly developed with some type of surface coating, a careful and thorough examination of their role in mitigating the cycle life issues of cathode materials is paramount. Here, this comprehensive review article extensively covers the selection criteria of coating materials based on their chemical and physical properties and electrochemical functionalities. Additionally, the article discusses the concept of critical coating thickness and methods of achieving homogeneous coating architectures that deliver desired performance benefits. Furthermore, this comprehensive article summarizes the recent advancements, effectiveness, necessity of cathode surface coatings and identifies the key aspect of structure-property correlation between coating type/thickness and lithium-ion diffusion through coating layers as the linchpin that validates surface coating approaches especially for high capacity nickel-rich cathodes.

Authors:

Nisar, Umair ^[1];

^[2]; Essehli, Rachid ^[2]; Amin, Ruhul ^[2];

^[2]

Centre for Solar Energy and Hydrogen Research Baden-Württemberg (ZSW), Helmholtzstraße (Germany)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)

Publication Date:: Fri Mar 19 00:00:00 EDT 2021

Research Org.:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Sponsoring Org.:: USDOE Office of Energy Efficiency and Renewable Energy (EERE), Transportation Office. Vehicle Technologies Office; USDOE

OSTI Identifier:: 1777732

Alternate Identifier(s):: OSTI ID: 1782897

Grant/Contract Number:: AC05-00OR22725

Resource Type:: Accepted Manuscript

Journal Name:: Energy Storage Materials

Additional Journal Information:: Journal Volume: 38; Journal ID: ISSN 2405-8297

Publisher:: Elsevier

Country of Publication:: United States

Language:: English

Subject:: 25 ENERGY STORAGE; surface coatings; batteries; electrodes; critical thickness; diffusion; lithium; solid-state

Citation Formats


                    Nisar, Umair, Muralidharan, Nitin, Essehli, Rachid, Amin, Ruhul, and Belharouak, Ilias. Valuation of Surface Coatings in High-Energy Density Lithium-ion Battery Cathode Materials.  United States: N. p., 2021. 
Web.  doi:10.1016/j.ensm.2021.03.015.

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                    Nisar, Umair, Muralidharan, Nitin, Essehli, Rachid, Amin, Ruhul, & Belharouak, Ilias. Valuation of Surface Coatings in High-Energy Density Lithium-ion Battery Cathode Materials.  United States.  https://doi.org/10.1016/j.ensm.2021.03.015

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                    Nisar, Umair, Muralidharan, Nitin, Essehli, Rachid, Amin, Ruhul, and Belharouak, Ilias. Fri .  
"Valuation of Surface Coatings in High-Energy Density Lithium-ion Battery Cathode Materials".  United States.  https://doi.org/10.1016/j.ensm.2021.03.015.  https://www.osti.gov/servlets/purl/1777732.

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@article{osti_1777732,

  title        = {Valuation of Surface Coatings in High-Energy Density Lithium-ion Battery Cathode Materials},

  author       = {Nisar, Umair and Muralidharan, Nitin and Essehli, Rachid and Amin, Ruhul and Belharouak, Ilias},

  abstractNote = {Artificial barriers, usually with either electrochemically active or inactive coating materials, are deployed on cathode material surfaces to mitigate detrimental side reactions by suppressing direct contact of cathode and electrolyte called surface coatings. These surface coatings are commonly known to increase the wettability of liquid electrolyte and reduce the interfacial charge transfer resistance. An important caveat is the selection of appropriate coating material with appropriate thickness for achieving enhanced electrochemical performance. As modern battery materials are increasingly developed with some type of surface coating, a careful and thorough examination of their role in mitigating the cycle life issues of cathode materials is paramount. Here, this comprehensive review article extensively covers the selection criteria of coating materials based on their chemical and physical properties and electrochemical functionalities. Additionally, the article discusses the concept of critical coating thickness and methods of achieving homogeneous coating architectures that deliver desired performance benefits. Furthermore, this comprehensive article summarizes the recent advancements, effectiveness, necessity of cathode surface coatings and identifies the key aspect of structure-property correlation between coating type/thickness and lithium-ion diffusion through coating layers as the linchpin that validates surface coating approaches especially for high capacity nickel-rich cathodes.},

  doi          = {10.1016/j.ensm.2021.03.015},

  journal      = {Energy Storage Materials},

  number       = ,

  volume       = 38,

  place        = {United States},

  year         = {Fri Mar 19 00:00:00 EDT 2021},

  month        = {Fri Mar 19 00:00:00 EDT 2021}

}

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Title: Valuation of Surface Coatings in High-Energy Density Lithium-ion Battery Cathode Materials

Abstract

Citation Formats

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Surface modifications of electrode materials for lithium-ion batteries: status and trends journal, May 2014

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Facile formation of a Li3PO4 coating layer during the synthesis of a lithium-rich layered oxide for high-capacity lithium-ion batteries journal, May 2016

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Electrically Conductive Hierarchical Carbon Nanotube Networks with Tunable Mechanical Response journal, October 2016

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Ultrathin ZrO2 on LiNi0.5Mn0.3Co0.2O2 electrode surface via atomic layer deposition for high-voltage operation in lithium-ion batteries journal, August 2019

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Highly stable Li 1.2 Mn 0.54 Co 0.13 Ni 0.13 O 2 enabled by novel atomic layer deposited AlPO 4 coating journal, April 2017

Synthesis and Electrochemical Performance of a Lithium Titanium Phosphate Anode for Aqueous Lithium-Ion Batteries journal, January 2011

Nanomaterials for Rechargeable Lithium Batteries journal, April 2008

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Recent progress in cathode materials research for advanced lithium ion batteries journal, May 2012

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Preparation of FePO4 by liquid-phase method and modification on the surface of LiNi0.80Co0.15Al0.05O2 cathode material journal, January 2018

Controllable atomic layer deposition coatings to boost the performance of LiMn x Co y Ni 1 − x − y O 2 in lithium-ion batteries: A review journal, January 2020

Degradation mechanism and performance enhancement strategies of LiNixCoyAl1−x−yO2 (x ≥ 0.8) cathodes for rechargeable lithium-ion batteries: a review journal, May 2020

Lithium diffusion coefficient in amorphous lithium phosphate thin films measured by secondary ion mass spectroscopy with isotope exchange methods journal, October 2016

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Prospective materials and applications for Li secondary batteries journal, January 2011

Synthesis and characterization of advanced Li3V2(PO4)3 nanocrystals@conducting polymer PEDOT for high energy lithium-ion batteries journal, January 2017

Effects of MgO Coating on the Structural and Electrochemical Characteristics of LiCoO 2 as Cathode Materials for Lithium Ion Battery journal, April 2014

One-step hydrothermal synthesis of monolayer MoS 2 quantum dots for highly efficient electrocatalytic hydrogen evolution journal, January 2015

Novel fabrication of Li4Ti5O12 coated LiMn2O4 nanorods as cathode materials with long-term cyclic stability at high ambient temperature journal, August 2019

Investigation on the Electrochemical Properties and Stabilized Surface/Interface of Nano-AlPO 4 -Coated Li 1.15 Ni 0.17 Co 0.11 Mn 0.57 O 2 as the Cathode for Lithium-Ion Batteries journal, July 2018

Ultrafast triggered transient energy storage by atomic layer deposition into porous silicon for integrated transient electronics journal, January 2016

Bifunctional nano-ZrO2 modification of LiNi0·92Co0·08O2 cathode enabling high-energy density lithium ion batteries journal, October 2019

Suppressing Voltage Decay of a Lithium-Rich Cathode Material by Surface Enrichment with Atomic Ruthenium journal, June 2018

Surface modifications of electrode materials for lithium ion batteries journal, February 2006

LiNbO3-coated LiNi0.8Co0.1Mn0.1O2 cathode with high discharge capacity and rate performance for all-solid-state lithium battery journal, January 2020

Ultraslow Li Exchange Processes in Diamagnetic Li 2 ZrO 3 As Monitored by EXSY NMR journal, April 2013

Atomic layer deposition in nanostructured photovoltaics: tuning optical, electronic and surface properties journal, January 2015

Challenges in the development of advanced Li-ion batteries: a review journal, January 2011

Surface structure investigation of LiNi0.8Co0.2O2 by AlPO4 coating and using functional electrolyte journal, April 2009

Elevated-temperature behaviour of LiNi0.5Co0.2Mn0.3O2 cathode modified with rGO-SiO2 composite coating journal, November 2020

High-performance lithium ion batteries using SiO 2 -coated LiNi 0.5 Co 0.2 Mn 0.3 O 2 microspheres as cathodes journal, June 2017

Surface Modification of Li-Rich Cathode Materials for Lithium-Ion Batteries with a PEDOT:PSS Conducting Polymer journal, August 2016

Improved electrochemical performances of LiNi0.8Co0.1Mn0.1O2 cathode via SiO2 coating journal, June 2019

On the Functionality of Coatings for Cathode Active Materials in Thiophosphate‐Based All‐Solid‐State Batteries journal, May 2019

Research advances on cobalt-free cathodes for Li-ion batteries - The high voltage LiMn1.5Ni0.5O4 as an example journal, August 2020

Effect of AlPO[sub 4]-Nanoparticle Coating Concentration on High-Cutoff-Voltage Electrochemical Performances in LiCoO[sub 2] journal, January 2004

Cathode materials modified by surface coating for lithium ion batteries journal, May 2006

Iron catalyzed growth of crystalline multi-walled carbon nanotubes from ambient carbon dioxide mediated by molten carbonates journal, May 2017

Use of Ce to Reinforce the Interface of Ni-Rich LiNi 0.8 Co 0.1 Mn 0.1 O 2 Cathode Materials for Lithium-Ion Batteries under High Operating Voltage journal, January 2019

Al 2 O 3 , SiO 2 and TiO 2 as Coatings for Safer LiNi 0.8 Co 0.15 Al 0.05 O 2 Cathodes: Electrochemical Performance and Thermal Analysis by Accelerating Rate Calorimetry journal, January 2017

Lithium Transport in Amorphous Al 2 O 3 and AlF 3 for Discovery of Battery Coatings journal, April 2013

Controlled Nanoparticle Metal Phosphates (Metal = Al , Fe, Ce, and Sr) Coatings on LiCoO₂ Cathode Materials
journal, January 2005

A review on doping/coating of nickel-rich cathode materials for lithium-ion batteries
journal, April 2020

Significant Improvement of Electrochemical Performance of AlF₃-Coated Li[Ni_0.8Co_0.1Mn_0.1]O₂ Cathode Materials
journal, January 2007

Polysulfide Anchoring Mechanism Revealed by Atomic Layer Deposition of V ₂ O ₅ and Sulfur-Filled Carbon Nanotubes for Lithium–Sulfur Batteries
journal, February 2017

Surface chemistry of LiNi0.5Mn1.5O4 particles coated by Al2O3 using atomic layer deposition for lithium-ion batteries
journal, January 2015

Improvement the electrochemical performance of Cr doped layered-spinel composite cathode material Li 1.1 Ni 0.235 Mn 0.735 Cr 0.03 O 2.3 with Li 4 Ti 5 O 12 coating
journal, August 2017

Origin of Outstanding Stability in the Lithium Solid Electrolyte Materials: Insights from Thermodynamic Analyses Based on First-Principles Calculations
journal, October 2015

A modified Al2O3 coating process to enhance the electrochemical performance of Li(Ni1/3Co1/3Mn1/3)O2 and its comparison with traditional Al2O3 coating process
journal, December 2010

Surface modification of cathodes with nanosized amorphous MnO2 coating for high-power application in lithium-ion batteries
journal, August 2014

Atomic Layer Deposition for Graphene Device Integration
journal, May 2017

Electrochemical behaviours of SiO 2 -coated LiNi 0.8 Co 0.1 Mn 0.1 O 2 cathode materials by a novel modification method
journal, February 2016

Facile and efficient fabrication of Li3PO4-coated Ni-rich cathode for high-performance lithium-ion battery
journal, February 2020

Ultrathin Spinel Membrane-Encapsulated Layered Lithium-Rich Cathode Material for Advanced Li-Ion Batteries
journal, May 2014

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journal, May 2014

Modification of Ni-Rich FCG NMC and NCA Cathodes by Atomic Layer Deposition: Preventing Surface Phase Transitions for High-Voltage Lithium-Ion Batteries
journal, May 2016

Facile formation of a Li3PO4 coating layer during the synthesis of a lithium-rich layered oxide for high-capacity lithium-ion batteries
journal, May 2016

The effects of TiO2 coating on the electrochemical performance of Li[Li0.2Mn0.54Ni0.13Co0.13]O2 cathode material for lithium-ion battery
journal, September 2008

Challenges in Lithium Metal Anodes for Solid-State Batteries
journal, February 2020

Interface in Solid-State Lithium Battery: Challenges, Progress, and Outlook
journal, May 2019

Electrically Conductive Hierarchical Carbon Nanotube Networks with Tunable Mechanical Response
journal, October 2016

Use of lithium-ion batteries in electric vehicles
journal, October 2000

Ultrathin ZrO2 on LiNi0.5Mn0.3Co0.2O2 electrode surface via atomic layer deposition for high-voltage operation in lithium-ion batteries
journal, August 2019

Enhancing the performances of Li-ion batteries by carbon-coating: present and future
journal, January 2012

Role of surface coating on cathode materials for lithium-ion batteries
journal, January 2010

Highly stable Li 1.2 Mn 0.54 Co 0.13 Ni 0.13 O 2 enabled by novel atomic layer deposited AlPO 4 coating
journal, April 2017

Synthesis and Electrochemical Performance of a Lithium Titanium Phosphate Anode for Aqueous Lithium-Ion Batteries
journal, January 2011

Nanomaterials for Rechargeable Lithium Batteries
journal, April 2008

Critical Role of Oxygen Evolved from Layered Li–Excess Metal Oxides in Lithium Rechargeable Batteries
journal, July 2012

Enhanced cyclic stability at elevated temperature of spinel LiNi0.5Mn1.5O4 by Li4Ti5O12 coating as cathode material for high voltage lithium ion batteries
journal, March 2019

Recent progress in cathode materials research for advanced lithium ion batteries
journal, May 2012

H3PO4 treatment to enhance the electrochemical properties of Li(Ni1/3Mn1/3Co1/3)O2 and Li(Ni0.5Mn0.3Co0.2)O2 cathodes
journal, April 2019

Conducting Polymer Coating on a High-Voltage Cathode Based on Soft Chemistry Approach toward Improving Battery Performance
journal, July 2018

Extreme fast charging characteristics of zirconia modified LiNi0.5Mn1.5O4 cathode for lithium ion batteries
journal, August 2018

Carbon-enhanced electrodeposited SnO2/carbon nanofiber composites as anode for lithium-ion batteries
journal, October 2014

A modified ZrO2-coating process to improve electrochemical performance of Li(Ni1/3Co1/3Mn1/3)O2
journal, March 2009

Preparation of FePO4 by liquid-phase method and modification on the surface of LiNi0.80Co0.15Al0.05O2 cathode material
journal, January 2018

Controllable atomic layer deposition coatings to boost the performance of LiMn _x Co _y Ni _{1 − x − y} O ₂ in lithium-ion batteries: A review
journal, January 2020

Degradation mechanism and performance enhancement strategies of LiNixCoyAl1−x−yO2 (x ≥ 0.8) cathodes for rechargeable lithium-ion batteries: a review
journal, May 2020

Lithium diffusion coefficient in amorphous lithium phosphate thin films measured by secondary ion mass spectroscopy with isotope exchange methods
journal, October 2016

Enhancing Electrochemical Performance of LiNi0.6Co0.2Mn0.2O2 by Lithium-ion Conductor Surface Modification
journal, January 2017

Surface modification of Li1.2Mn0.54Co0.13Ni0.13O2 with conducting polypyrrole
journal, June 2013

A review on the key issues for lithium-ion battery management in electric vehicles
journal, March 2013

Diffusion of Lithium in Bulk Amorphous Silicon: A Theoretical Study
journal, October 2012

Effectively suppressing dissolution of manganese from spinel lithium manganate via a nanoscale surface-doping approach
journal, December 2014

Dry coating of active material particles with sulfide solid electrolytes for an all-solid-state lithium battery
journal, February 2020

Surface structure decoration of high capacity Li1.2Mn0.54Ni0.13Co0.13O2 cathode by mixed conductive coating of Li1.4Al0.4Ti1.6(PO4)3 and polyaniline for lithium-ion batteries
journal, August 2019

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journal, September 2020

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journal, July 2020

Carbon coating nanostructured-LiNi1/3Co1/3Mn1/3O2 cathode material synthesized by chemical vapor deposition method for high performance lithium-ion batteries
journal, May 2018

High Capacity, Surface-Modified Layered Li [Li _(1−x) ∕ ₃Mn _(2−x) ∕ ₃Ni_x ∕ ₃Co_{x ∕ 3} ] O₂ Cathodes with Low Irreversible Capacity Loss
journal, March 2006

Prospective materials and applications for Li secondary batteries
journal, January 2011

Synthesis and characterization of advanced Li3V2(PO4)3 nanocrystals@conducting polymer PEDOT for high energy lithium-ion batteries
journal, January 2017

Effects of MgO Coating on the Structural and Electrochemical Characteristics of LiCoO ₂ as Cathode Materials for Lithium Ion Battery
journal, April 2014

One-step hydrothermal synthesis of monolayer MoS ₂ quantum dots for highly efficient electrocatalytic hydrogen evolution
journal, January 2015

Novel fabrication of Li4Ti5O12 coated LiMn2O4 nanorods as cathode materials with long-term cyclic stability at high ambient temperature
journal, August 2019

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journal, July 2018

Ultrafast triggered transient energy storage by atomic layer deposition into porous silicon for integrated transient electronics
journal, January 2016

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journal, October 2019

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journal, June 2018

Surface modifications of electrode materials for lithium ion batteries
journal, February 2006

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journal, January 2020

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journal, January 2011

Surface structure investigation of LiNi0.8Co0.2O2 by AlPO4 coating and using functional electrolyte
journal, April 2009

Elevated-temperature behaviour of LiNi0.5Co0.2Mn0.3O2 cathode modified with rGO-SiO2 composite coating
journal, November 2020

High-performance lithium ion batteries using SiO 2 -coated LiNi 0.5 Co 0.2 Mn 0.3 O 2 microspheres as cathodes
journal, June 2017

Surface Modification of Li-Rich Cathode Materials for Lithium-Ion Batteries with a PEDOT:PSS Conducting Polymer
journal, August 2016

Improved electrochemical performances of LiNi0.8Co0.1Mn0.1O2 cathode via SiO2 coating
journal, June 2019

On the Functionality of Coatings for Cathode Active Materials in Thiophosphate‐Based All‐Solid‐State Batteries
journal, May 2019

Research advances on cobalt-free cathodes for Li-ion batteries - The high voltage LiMn1.5Ni0.5O4 as an example
journal, August 2020

Effect of AlPO[sub 4]-Nanoparticle Coating Concentration on High-Cutoff-Voltage Electrochemical Performances in LiCoO[sub 2]
journal, January 2004

Cathode materials modified by surface coating for lithium ion batteries
journal, May 2006

Iron catalyzed growth of crystalline multi-walled carbon nanotubes from ambient carbon dioxide mediated by molten carbonates
journal, May 2017

Use of Ce to Reinforce the Interface of Ni-Rich LiNi _0.8 Co _0.1 Mn _0.1 O ₂ Cathode Materials for Lithium-Ion Batteries under High Operating Voltage
journal, January 2019

Al ₂ O ₃ , SiO ₂ and TiO ₂ as Coatings for Safer LiNi _0.8 Co _0.15 Al _0.05 O ₂ Cathodes: Electrochemical Performance and Thermal Analysis by Accelerating Rate Calorimetry
journal, January 2017

Lithium Transport in Amorphous Al ₂ O ₃ and AlF ₃ for Discovery of Battery Coatings
journal, April 2013

Materials Challenges Facing Electrical Energy Storage
journal, April 2008

Ti surface doping of LiNi _0.5 Mn _1.5 O _4−δ positive electrodes for lithium ion batteries
journal, January 2018

Dual functions of zirconium modification on improving the electrochemical performance of Ni-rich LiNi _0.8 Co _0.1 Mn _0.1 O ₂
journal, January 2018