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Title: Emergence of superconductivity in doped multiorbital Hubbard chains

Abstract

Abstract We introduce a variational state for one-dimensional two-orbital Hubbard models that intuitively explains the recent computational discovery of pairing in these systems when hole doped. Our ansatz is an optimized linear superposition of Affleck–Kennedy–Lieb–Tasaki valence-bond states, rendering the combination a valence-bond liquid dubbed orbital resonant valence bond. We show that the undoped (one-electron/orbital) quantum state of two sites coupled into a global spin singlet is exactly written employing only spin-1/2 singlets linking orbitals at nearest-neighbor sites. Generalizing to longer chains defines our variational state visualized geometrically expressing our chain as a two-leg ladder, with one orbital per leg. As in Anderson’s resonating valence-bond state, our undoped variational state contains preformed singlet pairs that via doping become mobile, leading to superconductivity. Doped real materials with one-dimensional substructures, two near-degenerate orbitals, and intermediate Hubbard U / W strengths— W the carrier’s bandwidth—could realize spin-singlet pairing if on-site anisotropies are small. If these anisotropies are robust, spin-triplet pairing emerges.

Authors:
; ; ; ; ORCiD logo
Publication Date:
Research Org.:
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Center for Nanophase Materials Sciences (CNMS)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Materials Sciences & Engineering Division; USDOE Office of Science (SC), Advanced Scientific Computing Research (ASCR). Scientific Discovery through Advanced Computing (SciDAC); USDOE Office of Science (SC), Basic Energy Sciences (BES). Scientific User Facilities Division
OSTI Identifier:
1765428
Alternate Identifier(s):
OSTI ID: 1619011
Grant/Contract Number:  
AC05-00OR22725
Resource Type:
Published Article
Journal Name:
npj Quantum Materials
Additional Journal Information:
Journal Name: npj Quantum Materials Journal Volume: 5 Journal Issue: 1; Journal ID: ISSN 2397-4648
Publisher:
Nature Publishing Group
Country of Publication:
United Kingdom
Language:
English
Subject:
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; Superconducting properties and materials; Topological matter

Citation Formats

Patel, Niravkumar D., Kaushal, Nitin, Nocera, Alberto, Alvarez, Gonzalo, and Dagotto, Elbio. Emergence of superconductivity in doped multiorbital Hubbard chains. United Kingdom: N. p., 2020. Web. doi:10.1038/s41535-020-0228-2.
Patel, Niravkumar D., Kaushal, Nitin, Nocera, Alberto, Alvarez, Gonzalo, & Dagotto, Elbio. Emergence of superconductivity in doped multiorbital Hubbard chains. United Kingdom. https://doi.org/10.1038/s41535-020-0228-2
Patel, Niravkumar D., Kaushal, Nitin, Nocera, Alberto, Alvarez, Gonzalo, and Dagotto, Elbio. Fri . "Emergence of superconductivity in doped multiorbital Hubbard chains". United Kingdom. https://doi.org/10.1038/s41535-020-0228-2.
@article{osti_1765428,
title = {Emergence of superconductivity in doped multiorbital Hubbard chains},
author = {Patel, Niravkumar D. and Kaushal, Nitin and Nocera, Alberto and Alvarez, Gonzalo and Dagotto, Elbio},
abstractNote = {Abstract We introduce a variational state for one-dimensional two-orbital Hubbard models that intuitively explains the recent computational discovery of pairing in these systems when hole doped. Our ansatz is an optimized linear superposition of Affleck–Kennedy–Lieb–Tasaki valence-bond states, rendering the combination a valence-bond liquid dubbed orbital resonant valence bond. We show that the undoped (one-electron/orbital) quantum state of two sites coupled into a global spin singlet is exactly written employing only spin-1/2 singlets linking orbitals at nearest-neighbor sites. Generalizing to longer chains defines our variational state visualized geometrically expressing our chain as a two-leg ladder, with one orbital per leg. As in Anderson’s resonating valence-bond state, our undoped variational state contains preformed singlet pairs that via doping become mobile, leading to superconductivity. Doped real materials with one-dimensional substructures, two near-degenerate orbitals, and intermediate Hubbard U / W strengths— W the carrier’s bandwidth—could realize spin-singlet pairing if on-site anisotropies are small. If these anisotropies are robust, spin-triplet pairing emerges.},
doi = {10.1038/s41535-020-0228-2},
journal = {npj Quantum Materials},
number = 1,
volume = 5,
place = {United Kingdom},
year = {Fri May 08 00:00:00 EDT 2020},
month = {Fri May 08 00:00:00 EDT 2020}
}

Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record
https://doi.org/10.1038/s41535-020-0228-2

Citation Metrics:
Cited by: 12 works
Citation information provided by
Web of Science

Figures / Tables:

Fig. 1 Fig. 1: Summary main results. a Sketch of a chain with two active orbitals a and b. b Representation of a splitting the orbitals into legs forming a fictitious two-leg ladder, with legs only connected by the Hund coupling JH. c One component of the variational state proposed in themore » text. Arrows indicate spin-1/2 singlets linking nearest-neighbor sites. Although their spin is zero, they are oriented objects because singlets are antisymmetric under the exchange of spins. The full ORVB state is an optimized linear combination of all possible arrangements of these singlets, that is, a linear combination of AKLT valence-bond solids. d Doped state: holes “h” are effectively paired when a spin singlet is removed.« less

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Figures/Tables have been extracted from DOE-funded journal article accepted manuscripts.