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Title: Momentum dependent $$d_{xz/yz}$$ band splitting in LaFeAsO

Abstract

The nematic phase in iron based superconductors (IBSs) has attracted attention with a notion that it may provide important clue to the superconductivity. A series of angle-resolved photoemission spectroscopy (ARPES) studies were performed to understand the origin of the nematic phase. However, there is lack of ARPES study on LaFeAsO nematic phase. Here, we report the results of ARPES studies of the nematic phase in LaFeAsO. Degeneracy breaking between the dxz and dyz hole bands near the Γ and M point is observed in the nematic phase. Different temperature dependent band splitting behaviors are observed at the Γ and M points. The energy of the band splitting near the M point decreases as the temperature decreases while it has little temperature dependence near the Γ point. The nematic nature of the band shift near the M point is confirmed through a detwin experiment using a piezo device. Since a momentum dependent splitting behavior has been observed in other iron based superconductors, our observation confirms that the behavior is a universal one among iron based superconductors.

Authors:
 [1];  [1];  [1];  [1];  [2];  [2];  [3];  [4];  [4];  [5];  [5];  [6];  [6];  [7];  [8];  [1]
  1. Inst. for Basic Science (IBS), Seoul (South Korea). Center for Correlated Electron Systems; Seoul National Univ. (SNU) (South Korea)
  2. Leibniz Inst. for Solid State and Materials Research, Dresden (Germany)
  3. Leibniz Inst. for Solid State and Materials Research, Dresden (Germany); Dresden Univ. of Technology (Germany). Inst. of Solid State Physics
  4. Inst. for Basic Science (IBS), Pohang (South Korea). Center for Artificial Low Dimensional Electronic Systems; Pohang Univ. of Science and Technology (South Korea)
  5. Chinese Academy of Sciences (CAS), Beijing (China). Beijing National Lab. for Condensed Matter Physics; Collaborative Innovation Center of Quantum Matter, Beijing (China)
  6. Chinese Academy of Sciences (CAS), Shanghai (China). State Key Lab. of Functional Materials for Informatics, Shanghai Inst. of Microsystem and Information Technology (SIMIT)
  7. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Advanced Light Source (ALS)
  8. Korea Advanced Inst. of Science and Technology, Daejeon (South Korea)
Publication Date:
Research Org.:
Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES); National Research Foundation of Korea (NRF); National Natural Science Foundation of China (NSFC)
OSTI Identifier:
1763674
Grant/Contract Number:  
AC02-05CH11231; XDB07000000; 11227902; 2016K1A4A4A01922028; 2018K1A3A7A09056310
Resource Type:
Accepted Manuscript
Journal Name:
Scientific Reports
Additional Journal Information:
Journal Volume: 10; Journal Issue: 1; Journal ID: ISSN 2045-2322
Publisher:
Nature Publishing Group
Country of Publication:
United States
Language:
English
Subject:
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; Materials science; physics

Citation Formats

Huh, S. S., Kim, Y. S., Kyung, W. S., Jung, J. K., Kappenberger, R., Aswartham, S., Büchner, B., Ok, J. M., Kim, J. S., Dong, C., Hu, J. P., Cho, S. H., Shen, D. W., Denlinger, J. D., Kim, Y. K., and Kim, C. Momentum dependent $d_{xz/yz}$ band splitting in LaFeAsO. United States: N. p., 2020. Web. doi:10.1038/s41598-020-75600-w.
Huh, S. S., Kim, Y. S., Kyung, W. S., Jung, J. K., Kappenberger, R., Aswartham, S., Büchner, B., Ok, J. M., Kim, J. S., Dong, C., Hu, J. P., Cho, S. H., Shen, D. W., Denlinger, J. D., Kim, Y. K., & Kim, C. Momentum dependent $d_{xz/yz}$ band splitting in LaFeAsO. United States. https://doi.org/10.1038/s41598-020-75600-w
Huh, S. S., Kim, Y. S., Kyung, W. S., Jung, J. K., Kappenberger, R., Aswartham, S., Büchner, B., Ok, J. M., Kim, J. S., Dong, C., Hu, J. P., Cho, S. H., Shen, D. W., Denlinger, J. D., Kim, Y. K., and Kim, C. Mon . "Momentum dependent $d_{xz/yz}$ band splitting in LaFeAsO". United States. https://doi.org/10.1038/s41598-020-75600-w. https://www.osti.gov/servlets/purl/1763674.
@article{osti_1763674,
title = {Momentum dependent $d_{xz/yz}$ band splitting in LaFeAsO},
author = {Huh, S. S. and Kim, Y. S. and Kyung, W. S. and Jung, J. K. and Kappenberger, R. and Aswartham, S. and Büchner, B. and Ok, J. M. and Kim, J. S. and Dong, C. and Hu, J. P. and Cho, S. H. and Shen, D. W. and Denlinger, J. D. and Kim, Y. K. and Kim, C.},
abstractNote = {The nematic phase in iron based superconductors (IBSs) has attracted attention with a notion that it may provide important clue to the superconductivity. A series of angle-resolved photoemission spectroscopy (ARPES) studies were performed to understand the origin of the nematic phase. However, there is lack of ARPES study on LaFeAsO nematic phase. Here, we report the results of ARPES studies of the nematic phase in LaFeAsO. Degeneracy breaking between the dxz and dyz hole bands near the Γ and M point is observed in the nematic phase. Different temperature dependent band splitting behaviors are observed at the Γ and M points. The energy of the band splitting near the M point decreases as the temperature decreases while it has little temperature dependence near the Γ point. The nematic nature of the band shift near the M point is confirmed through a detwin experiment using a piezo device. Since a momentum dependent splitting behavior has been observed in other iron based superconductors, our observation confirms that the behavior is a universal one among iron based superconductors.},
doi = {10.1038/s41598-020-75600-w},
journal = {Scientific Reports},
number = 1,
volume = 10,
place = {United States},
year = {Mon Nov 09 00:00:00 EST 2020},
month = {Mon Nov 09 00:00:00 EST 2020}
}

Works referenced in this record:

Symmetry-breaking orbital anisotropy observed for detwinned Ba(Fe1-xCox)2As2 above the spin density wave transition
journal, April 2011

  • Yi, M.; Lu, D.; Chu, J. -H.
  • Proceedings of the National Academy of Sciences, Vol. 108, Issue 17
  • DOI: 10.1073/pnas.1015572108

Momentum Dependence of the Nematic Order Parameter in Iron-Based Superconductors
journal, August 2019


Phase transitions and iron-ordered moment form factor in LaFeAsO
journal, August 2010


Nematicity and quantum paramagnetism in FeSe
journal, September 2015

  • Wang, Fa; Kivelson, Steven A.; Lee, Dung-Hai
  • Nature Physics, Vol. 11, Issue 11
  • DOI: 10.1038/nphys3456

Electronic reconstruction through the structural and magnetic transitions in detwinned NaFeAs
journal, July 2012


Momentum-dependent sign inversion of orbital order in superconducting FeSe
journal, November 2015


Orbital-dependent Fermi surface shrinking as a fingerprint of nematicity in FeSe
journal, October 2016


Iron-Based Layered Superconductor La[O 1- x F x ]FeAs ( x = 0.05−0.12) with T c = 26 K
journal, March 2008

  • Kamihara, Yoichi; Watanabe, Takumi; Hirano, Masahiro
  • Journal of the American Chemical Society, Vol. 130, Issue 11
  • DOI: 10.1021/ja800073m

Disentangling the surface and bulk electronic structures of LaOFeAs
journal, September 2016


Divergent Nematic Susceptibility in an Iron Arsenide Superconductor
journal, August 2012


Observation of two distinct d x z / d y z band splittings in FeSe
journal, June 2015


Surface and bulk electronic structures of LaFeAsO studied by angle-resolved photoemission spectroscopy
journal, September 2010


High-temperature superconductivity in iron-based materials
journal, August 2010

  • Paglione, Johnpierre; Greene, Richard L.
  • Nature Physics, Vol. 6, Issue 9
  • DOI: 10.1038/nphys1759

Solid state single crystal growth of three-dimensional faceted LaFeAsO crystals
journal, February 2018


Interaction-induced singular Fermi surface in a high-temperature oxypnictide superconductor
journal, May 2015

  • Charnukha, A.; Thirupathaiah, S.; Zabolotnyy, V. B.
  • Scientific Reports, Vol. 5, Issue 1
  • DOI: 10.1038/srep10392

Sign-Reversing Orbital Polarization in the Nematic Phase of FeSe due to the C 2 Symmetry Breaking in the Self-Energy
journal, June 2016


What drives nematic order in iron-based superconductors?
journal, January 2014

  • Fernandes, R. M.; Chubukov, A. V.; Schmalian, J.
  • Nature Physics, Vol. 10, Issue 2
  • DOI: 10.1038/nphys2877

Theory of electron nematic order in LaFeAsO
journal, June 2008


Evidence for unidirectional nematic bond ordering in FeSe
journal, November 2016


Effects of Nematic Fluctuations on the Elastic Properties of Iron Arsenide Superconductors
journal, October 2010


Ubiquitous signatures of nematic quantum criticality in optimally doped Fe-based superconductors
journal, May 2016


Driving force of the orbital-relevant electronic nematicity in Fe-based superconductors
journal, September 2017


Electronic structure of the iron-based superconductor LaOFeP
journal, September 2008


Absence of Y-pocket in 1-Fe Brillouin zone and reversed orbital occupation imbalance in FeSe
journal, March 2020