Challenges and Strategies to Advance High-Energy Nickel-Rich Layered Lithium Transition Metal Oxide Cathodes for Harsh Operation

Xu, Gui‐Liang; Liu, Xiang; Daali, Amine; Amine, Rachid; Chen, Zonghai; Amine, Khalil

doi:10.1002/adfm.202004748

Title: Challenges and Strategies to Advance High-Energy Nickel-Rich Layered Lithium Transition Metal Oxide Cathodes for Harsh Operation

Abstract

Abstract Nickel‐rich layered lithium transition metal oxides (LiNi ₁₋ _x ₋ _y Co _x Mn _y O ₂ and LiNi ₁₋ _x ₋ _y Co _x Al _y O ₂ , x + y ≤ 0.2) are the most attractive cathode materials for the next generation lithium‐ion batteries for automotive application. However, they suffer from structural/interfacial instability during repeated charge/discharge, resulting in severe performance degradation and serious safety concerns. This work provides a comprehensive review about challenges and strategies to advance nickel‐rich layered cathodes specifically for harsh (high‐voltage, high‐temperature, and fast charging) operations. Firstly, the degradation pathways of nickel‐rich cathodes including surface/interface degradation, undesired cathode–electrolytes parasitic reactions, gas evolution, inter/intragranular cracking, and electrical/ionic isolation are discussed. Then, recent achievements in stabilizing the structure/interface of nickel‐rich cathodes via surface coating, cation/anion doping, composition tailoring, morphology engineering, and electrolytes optimization are summarized. Moreover, challenges and strategies to improve the performance of Ni‐rich cathodes at the electrode level are discussed. Outlook and perspectives to promote the practical application of nickel‐rich layered cathodes toward automotive application are provided as well.

Authors:

Xu, Gui‐Liang ^[1]; Liu, Xiang ^[1]; Daali, Amine ^[2]; Amine, Rachid ^[1]; Chen, Zonghai ^[1];

^[3]

Argonne National Lab. (ANL), Argonne, IL (United States)
Argonne National Lab. (ANL), Argonne, IL (United States); Univ. of Wisconsin, Milwaukee, WI (United States)
Argonne National Lab. (ANL), Argonne, IL (United States); Stanford Univ., CA (United States)

Publication Date:: Wed Sep 09 00:00:00 EDT 2020

Research Org.:: Argonne National Laboratory (ANL), Argonne, IL (United States)

Sponsoring Org.:: USDOE Office of Energy Efficiency and Renewable Energy (EERE), Transportation Office. Vehicle Technologies Office; USDOE

OSTI Identifier:: 1756623

Alternate Identifier(s):: OSTI ID: 1804188

Grant/Contract Number:: AC02-06CH11357

Resource Type:: Accepted Manuscript

Journal Name:: Advanced Functional Materials

Additional Journal Information:: Journal Volume: 30; Journal Issue: 46; Journal ID: ISSN 1616-301X

Publisher:: Wiley

Country of Publication:: United States

Language:: English

Subject:: 25 ENERGY STORAGE; Ni-rich cathode; degradation; electrolytes; lithium-ion batteries; structures

Citation Formats


                    Xu, Gui‐Liang, Liu, Xiang, Daali, Amine, Amine, Rachid, Chen, Zonghai, and Amine, Khalil. Challenges and Strategies to Advance High-Energy Nickel-Rich Layered Lithium Transition Metal Oxide Cathodes for Harsh Operation.  United States: N. p., 2020. 
Web.  doi:10.1002/adfm.202004748.

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                    Xu, Gui‐Liang, Liu, Xiang, Daali, Amine, Amine, Rachid, Chen, Zonghai, & Amine, Khalil. Challenges and Strategies to Advance High-Energy Nickel-Rich Layered Lithium Transition Metal Oxide Cathodes for Harsh Operation.  United States.  https://doi.org/10.1002/adfm.202004748

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                    Xu, Gui‐Liang, Liu, Xiang, Daali, Amine, Amine, Rachid, Chen, Zonghai, and Amine, Khalil. Wed .  
"Challenges and Strategies to Advance High-Energy Nickel-Rich Layered Lithium Transition Metal Oxide Cathodes for Harsh Operation".  United States.  https://doi.org/10.1002/adfm.202004748.  https://www.osti.gov/servlets/purl/1756623.

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@article{osti_1756623,

  title        = {Challenges and Strategies to Advance High-Energy Nickel-Rich Layered Lithium Transition Metal Oxide Cathodes for Harsh Operation},

  author       = {Xu, Gui‐Liang and Liu, Xiang and Daali, Amine and Amine, Rachid and Chen, Zonghai and Amine, Khalil},

  abstractNote = {Abstract Nickel‐rich layered lithium transition metal oxides (LiNi 1− x − y Co x Mn y O 2 and LiNi 1− x − y Co x Al y O 2 , x  + y  ≤ 0.2) are the most attractive cathode materials for the next generation lithium‐ion batteries for automotive application. However, they suffer from structural/interfacial instability during repeated charge/discharge, resulting in severe performance degradation and serious safety concerns. This work provides a comprehensive review about challenges and strategies to advance nickel‐rich layered cathodes specifically for harsh (high‐voltage, high‐temperature, and fast charging) operations. Firstly, the degradation pathways of nickel‐rich cathodes including surface/interface degradation, undesired cathode–electrolytes parasitic reactions, gas evolution, inter/intragranular cracking, and electrical/ionic isolation are discussed. Then, recent achievements in stabilizing the structure/interface of nickel‐rich cathodes via surface coating, cation/anion doping, composition tailoring, morphology engineering, and electrolytes optimization are summarized. Moreover, challenges and strategies to improve the performance of Ni‐rich cathodes at the electrode level are discussed. Outlook and perspectives to promote the practical application of nickel‐rich layered cathodes toward automotive application are provided as well.},

  doi          = {10.1002/adfm.202004748},

  journal      = {Advanced Functional Materials},

  number       = 46,

  volume       = 30,

  place        = {United States},

  year         = {Wed Sep 09 00:00:00 EDT 2020},

  month        = {Wed Sep 09 00:00:00 EDT 2020}

}

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Improving the reversibility of the H2-H3 phase transitions for layered Ni-rich oxide cathode towards retarded structural transition and enhanced cycle stability journal, May 2019

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Synthetic Control of Kinetic Reaction Pathway and Cationic Ordering in High-Ni Layered Oxide Cathodes journal, August 2017

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In Situ Probing and Synthetic Control of Cationic Ordering in Ni-Rich Layered Oxide Cathodes journal, October 2016

Suppressed oxygen extraction and degradation of LiNi x Mn y Co z O2 cathodes at high charge cut-off voltages journal, September 2017

Temperature Dependence of Oxygen Release from LiNi 0.6 Mn 0.2 Co 0.2 O 2 (NMC622) Cathode Materials for Li-Ion Batteries journal, January 2018

Controlled synthesis of nickel-rich layered oxide cathodes with preferentially exposed {010} active facets for high rate and long cycling stable lithium-ion batteries journal, February 2019

Solid–Liquid Interfacial Reaction Trigged Propagation of Phase Transition from Surface into Bulk Lattice of Ni-Rich Layered Cathode journal, September 2018

Charge Transport in Single NCM Cathode Active Material Particles for Lithium-Ion Batteries Studied under Well-Defined Contact Conditions journal, August 2019

Microstructure‐Controlled Ni‐Rich Cathode Material by Microscale Compositional Partition for Next‐Generation Electric Vehicles journal, February 2019

Oxygen Release Induced Chemomechanical Breakdown of Layered Cathode Materials journal, April 2018

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Fluorinated Polyimide as a Novel High-Voltage Binder for High-Capacity Cathode of Lithium-Ion Batteries journal, November 2017

Intrinsic Origins of Crack Generation in Ni-rich LiNi0.8Co0.1Mn0.1O2 Layered Oxide Cathode Material journal, January 2017

Collapse of LiNi 1– x – y Co x Mn y O 2 Lattice at Deep Charge Irrespective of Nickel Content in Lithium-Ion Batteries journal, March 2019

Altering Surface Contaminants and Defects Influences the First-Cycle Outgassing and Irreversible Transformations of LiNi 0.6 Mn 0.2 Co 0.2 O 2 journal, June 2019

New Insight into Ni-Rich Layered Structure for Next-Generation Li Rechargeable Batteries journal, October 2017

Extending the Service Life of High-Ni Layered Oxides by Tuning the Electrode-Electrolyte Interphase journal, September 2018

Cation Ordering of Zr-Doped LiNiO 2 Cathode for Lithium-Ion Batteries journal, February 2018

Nickel-Rich Layered Lithium Transition-Metal Oxide for High-Energy Lithium-Ion Batteries journal, March 2015

Anisotropic Lattice Strain and Mechanical Degradation of High- and Low-Nickel NCM Cathode Materials for Li-Ion Batteries journal, February 2017

Mn versus Al in Layered Oxide Cathodes in Lithium-Ion Batteries: A Comprehensive Evaluation on Long-Term Cyclability journal, February 2018

Suppressing the Structure Deterioration of Ni-Rich LiNi 0.8 Co 0.1 Mn 0.1 O 2 through Atom-Scale Interfacial Integration of Self-Forming Hierarchical Spinel Layer with Ni Gradient Concentration journal, August 2017

Probing the Complexities of Structural Changes in Layered Oxide Cathode Materials for Li-Ion Batteries during Fast Charge–Discharge Cycling and Heating journal, January 2018

Thermal Runaway of Lithium-Ion Batteries without Internal Short Circuit journal, October 2018

Tailoring grain boundary structures and chemistry of Ni-rich layered cathodes for enhanced cycle stability of lithium-ion batteries journal, June 2018

Ni-Rich LiNi 0.8 Co 0.1 Mn 0.1 O 2 Oxide Coated by Dual-Conductive Layers as High Performance Cathode Material for Lithium-Ion Batteries journal, August 2017

Optimized preparation of LiNi0.6Mn0.2Co0.2O2 with single crystal morphology cathode material for lithium-ion batteries journal, January 2020

Self-Terminated Artificial SEI Layer for Nickel-Rich Layered Cathode Material via Mixed Gas Chemical Vapor Deposition journal, October 2015

Electrode–electrolyte interfaces in lithium-based batteries journal, January 2018

Role of Mn Content on the Electrochemical Properties of Nickel-Rich Layered LiNi 0.8– x Co 0.1 Mn 0.1+ x O 2 (0.0 ≤ x ≤ 0.08) Cathodes for Lithium-Ion Batteries journal, March 2015

Enhanced electrochemical performance and storage property of LiNi0.815Co0.15Al0.035O2 via Al gradient doping journal, September 2016

Revisiting Primary Particles in Layered Lithium Transition‐Metal Oxides and Their Impact on Structural Degradation journal, January 2019

Exposing the {010} Planes by Oriented Self-Assembly with Nanosheets To Improve the Electrochemical Performances of Ni-Rich Li[Ni 0.8 Co 0.1 Mn 0.1 ]O 2 Microspheres journal, February 2018

Long-Life Nickel-Rich Layered Oxide Cathodes with a Uniform Li 2 ZrO 3 Surface Coating for Lithium-Ion Batteries journal, March 2017

Pseudo-ischaemic ECG in a patient with amyotrophic lateral sclerosis surviving for a decade journal, February 2012

Combining In Situ Synchrotron X-Ray Diffraction and Absorption Techniques with Transmission Electron Microscopy to Study the Origin of Thermal Instability in Overcharged Cathode Materials for Lithium-Ion Batteries journal, June 2012

Al 2 O 3 , SiO 2 and TiO 2 as Coatings for Safer LiNi 0.8 Co 0.15 Al 0.05 O 2 Cathodes: Electrochemical Performance and Thermal Analysis by Accelerating Rate Calorimetry journal, January 2017

Intragranular cracking as a critical barrier for high-voltage usage of layer-structured cathode for lithium-ion batteries journal, January 2017

Atomic layer deposition of solid-state electrolyte coated cathode materials with superior high-voltage cycling behavior for lithium ion battery application journal, January 2014

High-performance battery electrodes via magnetic templating journal, July 2016

High-energy cathode material for long-life and safe lithium batteries journal, March 2009

Dynamic behaviour of interphases and its implication on high-energy-density cathode materials in lithium-ion batteries journal, April 2017

Fluorinated electrolyte for 4.5 V Li(Ni0.4Mn0.4Co0.2)O2/graphite Li-ion cells journal, March 2016

Improvement of long-term cycling performance of Li[Ni0.8Co0.15Al0.05]O2 by AlF3 coating journal, July 2013

Hierarchical LiNi 0.8 Co 0.15 Al 0.05 O 2 plates with exposed {010} active planes as a high performance cathode material for Li-ion batteries journal, January 2016

Non-flammable LiNi0.8Co0.1Mn0.1O2 cathode via functional binder; stabilizing high-voltage interface and performance for safer and high-energy lithium rechargeable batteries journal, September 2019

Flux-free synthesis of single-crystal LiNi0.8Co0.1Mn0.1O2 boosts its electrochemical performance in lithium batteries journal, July 2020

Enhancing structural stability unto 4.5 V of Ni-rich cathodes by tungsten-doping for lithium storage journal, May 2019

Structural Changes and Thermal Stability of Charged LiNi x Mn y Co z O 2 Cathode Materials Studied by Combined In Situ Time-Resolved XRD and Mass Spectroscopy journal, December 2014

Polyanion and cation co-doping stabilized Ni-rich Ni–Co–Al material as cathode with enhanced electrochemical performance for Li-ion battery journal, September 2019

Synthesis of single crystalline hexagonal nanobricks of LiNi1/3Co1/3Mn1/3O2 with high percentage of exposed {010} active facets as high rate performance cathode material for lithium-ion battery journal, January 2013

High-Performance and Industrially Feasible Ni-Rich Layered Cathode Materials by Integrating Coherent Interphase journal, May 2018

Lattice doping regulated interfacial reactions in cathode for enhanced cycling stability journal, August 2019

Enhancement on structural stability of Ni-rich cathode materials by in-situ fabricating dual-modified layer for lithium-ion batteries journal, November 2019

Towards Understanding of Cracking during Drying of Thick Aqueous-Processed LiNi 0.8 Mn 0.1 Co 0.1 O 2 Cathodes journal, February 2020

Surface reconstruction and chemical evolution of stoichiometric layered cathode materials for lithium-ion batteries journal, March 2014

Mechanisms of Degradation and Strategies for the Stabilization of Cathode–Electrolyte Interfaces in Li-Ion Batteries journal, January 2018

A New Coating Method for Alleviating Surface Degradation of LiNi 0.6 Co 0.2 Mn 0.2 O 2 Cathode Material: Nanoscale Surface Treatment of Primary Particles journal, February 2015

Origin of Carbon Dioxide Evolved during Cycling of Nickel-Rich Layered NCM Cathodes journal, October 2018

Oxidatively stable fluorinated sulfone electrolytes for high voltage high energy lithium-ion batteries journal, January 2017

Effect of Residual Lithium Compounds on Layer Ni-Rich Li[Ni 0.7 Mn 0.3 ]O 2 journal, January 2014

Pushing the limit of layered transition metal oxide cathodes for high-energy density rechargeable Li ion batteries journal, January 2018

Enhanced Stability of LiCoO2 Cathodes in Lithium-Ion Batteries Using Surface Modification by Atomic Layer Deposition journal, January 2010

Improving the reversibility of the H2-H3 phase transitions for layered Ni-rich oxide cathode towards retarded structural transition and enhanced cycle stability
journal, May 2019

Revealing Cycling Rate-Dependent Structure Evolution in Ni-Rich Layered Cathode Materials
journal, September 2018

Synthetic Control of Kinetic Reaction Pathway and Cationic Ordering in High-Ni Layered Oxide Cathodes
journal, August 2017

Crystal structural design of exposed planes: express channels, high-rate capability cathodes for lithium-ion batteries
journal, January 2018

Pathways for practical high-energy long-cycling lithium metal batteries
journal, February 2019

High-Capacity Concentration Gradient Li[Ni _0.865 Co _0.120 Al _0.015 ]O ₂ Cathode for Lithium-Ion Batteries
journal, March 2018

Ni‐Rich/Co‐Poor Layered Cathode for Automotive Li‐Ion Batteries: Promises and Challenges
journal, March 2020

In Situ Probing and Synthetic Control of Cationic Ordering in Ni-Rich Layered Oxide Cathodes
journal, October 2016

Suppressed oxygen extraction and degradation of LiNi x Mn y Co z O2 cathodes at high charge cut-off voltages
journal, September 2017

Temperature Dependence of Oxygen Release from LiNi _0.6 Mn _0.2 Co _0.2 O ₂ (NMC622) Cathode Materials for Li-Ion Batteries
journal, January 2018

Controlled synthesis of nickel-rich layered oxide cathodes with preferentially exposed {010} active facets for high rate and long cycling stable lithium-ion batteries
journal, February 2019

Solid–Liquid Interfacial Reaction Trigged Propagation of Phase Transition from Surface into Bulk Lattice of Ni-Rich Layered Cathode
journal, September 2018

Charge Transport in Single NCM Cathode Active Material Particles for Lithium-Ion Batteries Studied under Well-Defined Contact Conditions
journal, August 2019

Microstructure‐Controlled Ni‐Rich Cathode Material by Microscale Compositional Partition for Next‐Generation Electric Vehicles
journal, February 2019

Oxygen Release Induced Chemomechanical Breakdown of Layered Cathode Materials
journal, April 2018

Role of surface coating on cathode materials for lithium-ion batteries
journal, January 2010

Low temperature and roll-to-roll spatial atomic layer deposition for flexible electronics
journal, January 2012

Conflicting Roles of Anion Doping on the Electrochemical Performance of Li-Ion Battery Cathode Materials
journal, September 2016

Persistent State-of-Charge Heterogeneity in Relaxed, Partially Charged Li ₁₋ _x Ni _1/3 Co _1/3 Mn _1/3 O ₂ Secondary Particles
journal, May 2016

A Wide Range of Testing Results on an Excellent Lithium-Ion Cell Chemistry to be used as Benchmarks for New Battery Technologies
journal, January 2019

Stabilizing the Electrode/Electrolyte Interface of LiNi _0.8 Co _0.15 Al _0.05 O ₂ through Tailoring Aluminum Distribution in Microspheres as Long-Life, High-Rate, and Safe Cathode for Lithium-Ion Batteries
journal, August 2017

Building ultraconformal protective layers on both secondary and primary particles of layered lithium transition metal oxide cathodes
journal, May 2019

Understanding thickness and porosity effects on the electrochemical performance of LiNi0.6Co0.2Mn0.2O2-based cathodes for high energy Li-ion batteries
journal, April 2019

Dissolution, migration, and deposition of transition metal ions in Li-ion batteries exemplified by Mn-based cathodes – a critical review
journal, January 2018

Design of Battery Electrodes with Dual-Scale Porosity to Minimize Tortuosity and Maximize Performance
journal, December 2012

Fluorinated Polyimide as a Novel High-Voltage Binder for High-Capacity Cathode of Lithium-Ion Batteries
journal, November 2017

Intrinsic Origins of Crack Generation in Ni-rich LiNi0.8Co0.1Mn0.1O2 Layered Oxide Cathode Material
journal, January 2017

Collapse of LiNi _{1– x – y} Co _x Mn _y O ₂ Lattice at Deep Charge Irrespective of Nickel Content in Lithium-Ion Batteries
journal, March 2019

Altering Surface Contaminants and Defects Influences the First-Cycle Outgassing and Irreversible Transformations of LiNi _0.6 Mn _0.2 Co _0.2 O ₂
journal, June 2019

New Insight into Ni-Rich Layered Structure for Next-Generation Li Rechargeable Batteries
journal, October 2017

Extending the Service Life of High-Ni Layered Oxides by Tuning the Electrode-Electrolyte Interphase
journal, September 2018

Cation Ordering of Zr-Doped LiNiO ₂ Cathode for Lithium-Ion Batteries
journal, February 2018

Nickel-Rich Layered Lithium Transition-Metal Oxide for High-Energy Lithium-Ion Batteries
journal, March 2015

Anisotropic Lattice Strain and Mechanical Degradation of High- and Low-Nickel NCM Cathode Materials for Li-Ion Batteries
journal, February 2017

Mn versus Al in Layered Oxide Cathodes in Lithium-Ion Batteries: A Comprehensive Evaluation on Long-Term Cyclability
journal, February 2018

Suppressing the Structure Deterioration of Ni-Rich LiNi _0.8 Co _0.1 Mn _0.1 O ₂ through Atom-Scale Interfacial Integration of Self-Forming Hierarchical Spinel Layer with Ni Gradient Concentration
journal, August 2017

Probing the Complexities of Structural Changes in Layered Oxide Cathode Materials for Li-Ion Batteries during Fast Charge–Discharge Cycling and Heating
journal, January 2018

Thermal Runaway of Lithium-Ion Batteries without Internal Short Circuit
journal, October 2018

Tailoring grain boundary structures and chemistry of Ni-rich layered cathodes for enhanced cycle stability of lithium-ion batteries
journal, June 2018

Ni-Rich LiNi _0.8 Co _0.1 Mn _0.1 O ₂ Oxide Coated by Dual-Conductive Layers as High Performance Cathode Material for Lithium-Ion Batteries
journal, August 2017

Optimized preparation of LiNi0.6Mn0.2Co0.2O2 with single crystal morphology cathode material for lithium-ion batteries
journal, January 2020

Self-Terminated Artificial SEI Layer for Nickel-Rich Layered Cathode Material via Mixed Gas Chemical Vapor Deposition
journal, October 2015

Electrode–electrolyte interfaces in lithium-based batteries
journal, January 2018

Role of Mn Content on the Electrochemical Properties of Nickel-Rich Layered LiNi _{0.8– x} Co _0.1 Mn _{0.1+ x} O ₂ (0.0 ≤ x ≤ 0.08) Cathodes for Lithium-Ion Batteries
journal, March 2015

Enhanced electrochemical performance and storage property of LiNi0.815Co0.15Al0.035O2 via Al gradient doping
journal, September 2016

Revisiting Primary Particles in Layered Lithium Transition‐Metal Oxides and Their Impact on Structural Degradation
journal, January 2019

Exposing the {010} Planes by Oriented Self-Assembly with Nanosheets To Improve the Electrochemical Performances of Ni-Rich Li[Ni _0.8 Co _0.1 Mn _0.1 ]O ₂ Microspheres
journal, February 2018

Long-Life Nickel-Rich Layered Oxide Cathodes with a Uniform Li ₂ ZrO ₃ Surface Coating for Lithium-Ion Batteries
journal, March 2017

Pseudo-ischaemic ECG in a patient with amyotrophic lateral sclerosis surviving for a decade
journal, February 2012

Combining In Situ Synchrotron X-Ray Diffraction and Absorption Techniques with Transmission Electron Microscopy to Study the Origin of Thermal Instability in Overcharged Cathode Materials for Lithium-Ion Batteries
journal, June 2012

Al ₂ O ₃ , SiO ₂ and TiO ₂ as Coatings for Safer LiNi _0.8 Co _0.15 Al _0.05 O ₂ Cathodes: Electrochemical Performance and Thermal Analysis by Accelerating Rate Calorimetry
journal, January 2017

Intragranular cracking as a critical barrier for high-voltage usage of layer-structured cathode for lithium-ion batteries
journal, January 2017

Atomic layer deposition of solid-state electrolyte coated cathode materials with superior high-voltage cycling behavior for lithium ion battery application
journal, January 2014

High-performance battery electrodes via magnetic templating
journal, July 2016

High-energy cathode material for long-life and safe lithium batteries
journal, March 2009

Dynamic behaviour of interphases and its implication on high-energy-density cathode materials in lithium-ion batteries
journal, April 2017

Fluorinated electrolyte for 4.5 V Li(Ni0.4Mn0.4Co0.2)O2/graphite Li-ion cells
journal, March 2016

Improvement of long-term cycling performance of Li[Ni0.8Co0.15Al0.05]O2 by AlF3 coating
journal, July 2013

Hierarchical LiNi _0.8 Co _0.15 Al _0.05 O ₂ plates with exposed {010} active planes as a high performance cathode material for Li-ion batteries
journal, January 2016

Non-flammable LiNi0.8Co0.1Mn0.1O2 cathode via functional binder; stabilizing high-voltage interface and performance for safer and high-energy lithium rechargeable batteries
journal, September 2019

Flux-free synthesis of single-crystal LiNi0.8Co0.1Mn0.1O2 boosts its electrochemical performance in lithium batteries
journal, July 2020

Enhancing structural stability unto 4.5 V of Ni-rich cathodes by tungsten-doping for lithium storage
journal, May 2019

Structural Changes and Thermal Stability of Charged LiNi _x Mn _y Co _z O ₂ Cathode Materials Studied by Combined In Situ Time-Resolved XRD and Mass Spectroscopy
journal, December 2014

Polyanion and cation co-doping stabilized Ni-rich Ni–Co–Al material as cathode with enhanced electrochemical performance for Li-ion battery
journal, September 2019

Synthesis of single crystalline hexagonal nanobricks of LiNi1/3Co1/3Mn1/3O2 with high percentage of exposed {010} active facets as high rate performance cathode material for lithium-ion battery
journal, January 2013

High-Performance and Industrially Feasible Ni-Rich Layered Cathode Materials by Integrating Coherent Interphase
journal, May 2018

Lattice doping regulated interfacial reactions in cathode for enhanced cycling stability
journal, August 2019

Enhancement on structural stability of Ni-rich cathode materials by in-situ fabricating dual-modified layer for lithium-ion batteries
journal, November 2019

Towards Understanding of Cracking during Drying of Thick Aqueous-Processed LiNi _0.8 Mn _0.1 Co _0.1 O ₂ Cathodes
journal, February 2020

Surface reconstruction and chemical evolution of stoichiometric layered cathode materials for lithium-ion batteries
journal, March 2014

Mechanisms of Degradation and Strategies for the Stabilization of Cathode–Electrolyte Interfaces in Li-Ion Batteries
journal, January 2018

A New Coating Method for Alleviating Surface Degradation of LiNi _0.6 Co _0.2 Mn _0.2 O ₂ Cathode Material: Nanoscale Surface Treatment of Primary Particles
journal, February 2015

Origin of Carbon Dioxide Evolved during Cycling of Nickel-Rich Layered NCM Cathodes
journal, October 2018

Oxidatively stable fluorinated sulfone electrolytes for high voltage high energy lithium-ion batteries
journal, January 2017

Effect of Residual Lithium Compounds on Layer Ni-Rich Li[Ni _0.7 Mn _0.3 ]O ₂
journal, January 2014

Pushing the limit of layered transition metal oxide cathodes for high-energy density rechargeable Li ion batteries
journal, January 2018

Enhanced Stability of LiCoO₂ Cathodes in Lithium-Ion Batteries Using Surface Modification by Atomic Layer Deposition
journal, January 2010

Single-crystal LiNi0.6Co0.2Mn0.2O2 as high performance cathode materials for Li-ion batteries
journal, July 2016

High-energy-density lithium-ion battery using a carbon-nanotube–Si composite anode and a compositionally graded Li[Ni _0.85 Co _0.05 Mn _0.10 ]O ₂ cathode
journal, January 2016

The high-temperature and high-humidity storage behaviors and electrochemical degradation mechanism of LiNi0.6Co0.2Mn0.2O2 cathode material for lithium ion batteries
journal, September 2017