Magnetoelastic distortion of multiferroic BiFeO3 in the canted antiferromagnetic state

Rõõm, T.; Viirok, J.; Peedu, L.; Nagel, U.; Farkas, D. G.; Szaller, D.; Kocsis, V.; Bordács, S.; Kézsmárki, I.; Kamenskyi, D. L.; Engelkamp, H.; Ozerov, M.; Smirnov, D.; Krzystek, J.; Thirunavukkuarasu, K.; Ozaki, Y.; Tomioka, Y.; Ito, T.; Datta, T.; Fishman, R. S.

doi:10.1103/physrevb.102.214410

Title: Magnetoelastic distortion of multiferroic BiFeO₃ in the canted antiferromagnetic state

Journal Article · 08 December 2020 · Physical Review. B

DOI: https://doi.org/10.1103/physrevb.102.214410 · OSTI ID:1755293

^[1]; Viirok, J. ^[1]; Peedu, L. ^[1];

^[1]; Farkas, D. G. ^[2];

^[3]; Kocsis, V. ^[4]; Bordács, S. ^[2]; Kézsmárki, I. ^[5]; Kamenskyi, D. L. ^[6];

^[6]; Ozerov, M. ^[7]; Smirnov, D. ^[7];

^[7]; Thirunavukkuarasu, K. ^[8]; Ozaki, Y. ^[9]; Tomioka, Y. ^[9]; Ito, T. ^[9];

^[10];

^[11]

National Inst. of Chemical Physics and Biophysics, Tallinn (Estonia)
Budapest Univ. of Technology and Economics (Hungary); Hungarian Academy of Sciences, Budapest (Hungary)
Budapest Univ. of Technology and Economics (Hungary); Vienna Univ. of Technology (Austria)
Budapest Univ. of Technology and Economics (Hungary); RIKEN Center for Emergent Matter Science (CEMS), Wako (Japan)
Budapest Univ. of Technology and Economics (Hungary); Univ. of Augsburg (Germany)
Radboud Univ., Nijmegen (Netherlands)
Florida State Univ., Tallahassee, FL (United States). National High Magnetic Field Lab. (MagLab)
Florida A & M University, Tallahassee, FL (United States)
National Inst. of Advanced Industrial Science and Technology (AIST), Tsukuba (Japan)
Augusta Univ., GA (United States)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Materials Science & Technology Division

Using THz spectroscopy, here we show that the spin-wave spectrum of multiferroic BiFeO₃ in its high-field canted antiferromagnetic state is well described by a spin model that violates rhombohedral symmetry. We demonstrate that the monoclinic distortion of the canted antiferromagnetic state is induced by the single-ion magnetoelastic coupling between the lattice and the two nearly antiparallel spins. The revised spin model for BiFeO₃ contains two new single-ion anisotropy terms that violate rhombohedral symmetry and depend on the direction of the magnetic field.

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Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: Austrian Science Fund (FWF); BME; Estonian Academy of Science; Estonian Ministry of Education and Research Council Grants; European Regional Development Fund; German Research Foundation (DFG); Hungarian Academy of Science; Hungarian Innovation Office (NKFIH); National Science Foundation (NSF); SYSU; USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 1755293

Journal Information:: Physical Review. B, Journal Name: Physical Review. B Journal Issue: 21 Vol. 102; ISSN 2469-9950

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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75 CONDENSED MATTER PHYSICS
SUPERCONDUCTIVITY AND SUPERFLUIDITY
ferroelectricity
ferroelectrics
magnetic anisotropy
magnetic order
magnetoelastic effect
multiferroics
spin dynamics
spin waves
spin-orbit coupling
terahertz spectroscopy

Title: Magnetoelastic distortion of multiferroic BiFeO3 in the canted antiferromagnetic state

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Title: Magnetoelastic distortion of multiferroic BiFeO₃ in the canted antiferromagnetic state