LaMer's 1950 model of particle formation: a review and critical analysis of its classical nucleation and fluctuation theory basis, of competing models and mechanisms for phase-changes and particle formation, and then of its application to silver halide, semiconductor, metal, and metal-oxide nanoparticles

Whitehead, Christopher B.; Özkar, Saim; Finke, Richard G.

doi:10.1039/D0MA00439A

Title: LaMer's 1950 model of particle formation: a review and critical analysis of its classical nucleation and fluctuation theory basis, of competing models and mechanisms for phase-changes and particle formation, and then of its application to silver halide, semiconductor, metal, and metal-oxide nanoparticles

Abstract

Are classical nucleation theory and the 1950 LaMer model of particle formation supported for a wide range of particle formations, or do competing models in the form of chemical reaction mechanisms have better experimental support? Read on to find out.

Authors:

^[1];

^[2];

^[1]

Department of Chemistry, Colorado State University, Fort Collins, USA
Department of Chemistry, Middle East Technical University, 06800 Ankara, Turkey

Publication Date:: Mon Jan 18 00:00:00 EST 2021

Sponsoring Org.:: USDOE

OSTI Identifier:: 1742062

Grant/Contract Number:: SE-FG402-02ER15453

Resource Type:: Published Article

Journal Name:: Materials Advances

Additional Journal Information:: Journal Name: Materials Advances Journal Volume: 2 Journal Issue: 1; Journal ID: ISSN 2633-5409

Publisher:: Royal Society of Chemistry (RSC)

Country of Publication:: United Kingdom

Language:: English

Citation Formats


                    Whitehead, Christopher B., Özkar, Saim, and Finke, Richard G. LaMer's 1950 model of particle formation: a review and critical analysis of its classical nucleation and fluctuation theory basis, of competing models and mechanisms for phase-changes and particle formation, and then of its application to silver halide, semiconductor, metal, and metal-oxide nanoparticles.  United Kingdom: N. p., 2021. 
Web.  doi:10.1039/D0MA00439A.

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                    Whitehead, Christopher B., Özkar, Saim, & Finke, Richard G. LaMer's 1950 model of particle formation: a review and critical analysis of its classical nucleation and fluctuation theory basis, of competing models and mechanisms for phase-changes and particle formation, and then of its application to silver halide, semiconductor, metal, and metal-oxide nanoparticles.  United Kingdom.  https://doi.org/10.1039/D0MA00439A

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                    Whitehead, Christopher B., Özkar, Saim, and Finke, Richard G. Mon .  
"LaMer's 1950 model of particle formation: a review and critical analysis of its classical nucleation and fluctuation theory basis, of competing models and mechanisms for phase-changes and particle formation, and then of its application to silver halide, semiconductor, metal, and metal-oxide nanoparticles".  United Kingdom.  https://doi.org/10.1039/D0MA00439A.

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@article{osti_1742062,

  title        = {LaMer's 1950 model of particle formation: a review and critical analysis of its classical nucleation and fluctuation theory basis, of competing models and mechanisms for phase-changes and particle formation, and then of its application to silver halide, semiconductor, metal, and metal-oxide nanoparticles},

  author       = {Whitehead, Christopher B. and Özkar, Saim and Finke, Richard G.},

  abstractNote = {Are classical nucleation theory and the 1950 LaMer model of particle formation supported for a wide range of particle formations, or do competing models in the form of chemical reaction mechanisms have better experimental support? Read on to find out.},

  doi          = {10.1039/D0MA00439A},

  journal      = {Materials Advances},

  number       = 1,

  volume       = 2,

  place        = {United Kingdom},

  year         = {Mon Jan 18 00:00:00 EST 2021},

  month        = {Mon Jan 18 00:00:00 EST 2021}

}

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Mechanism of Formation of Monodispersed Colloids by Aggregation of Nanosize Precursors
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Heterogeneous nucleation of/on nanoparticles: a density functional study using the phase-field crystal model
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On the Kinetics of Formation of Precipitates of Sparingly Soluble Salts.
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Pathways for Gold Nucleation and Growth over Protein Cages
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Common Features of Extraordinary Rate Theories
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Nucleation of Crystals from Solution: Classical and Two-Step Models
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Mechanism of Gold Nanoparticle Formation in the Classical Citrate Synthesis Method Derived from Coupled In Situ XANES and SAXS Evaluation
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Computer Simulations of Nucleation of Nanoparticle Superclusters from Solution
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Mechanisms of Nucleation and Growth of Nanoparticles in Solution
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The theory of the nucleation of monodisperse particles in open systems and its application to agbr systems
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The Bakerian Lecture: Experimental Relations of Gold (and Other Metals) to Light
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Nucleation Kinetics vs Chemical Kinetics in the Initial Formation of Semiconductor Nanocrystals
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Pathway from a Molecular Precursor to Silver Nanoparticles: The Prominent Role of Aggregative Growth
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Enhanced Nanoparticle Size Control by Extending LaMer’s Mechanism
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Aggregative Growth of Silicalite-1
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Enhancement of Protein Crystal Nucleation by Critical Density Fluctuations
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Precursor Conversion Kinetics and the Nucleation of Cadmium Selenide Nanocrystals
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The Initial Stages of Template-Controlled CaCO₃ Formation Revealed by Cryo-TEM
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The Problem of Measuring Homogeneous Nucleation Rates and the Molecular Contents of Nuclei: Progress in the Form of Nucleation Pulse Measurements
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Tuning Precursor Reactivity toward Nanometer-Size Control in Palladium Nanoparticles Studied by in Situ Small Angle X-ray Scattering
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Morphology development and crystal growth in nanocrystalline aggregates under hydrothermal conditions: insights from titania
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On the Two-Step Mechanism for Synthesis of Transition-Metal Nanoparticles
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Strong Inference: Certain systematic methods of scientific thinking may produce much more rapid progress than others
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Ligand Effects on Synthesis and Post-Synthetic Stability of PbSe Nanocrystals
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Synthesis of monodispersed silica powders I. Particle properties and reaction kinetics
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Analysis of reaction kinetics in the photomechanical molecular crystal 9-methylanthracene using an extended Finke–Watzky model
journal, January 2016

Synthesis and Characterization of [Ir(1,5-Cyclooctadiene)(μ-H)] ₄ : A Tetrametallic Ir ₄ H ₄ -Core, Coordinatively Unsaturated Cluster
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Controlled growth of monodisperse silica spheres in the micron size range
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Surface Ligand Dynamics in Growth of Nanocrystals
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A critical review of the applicability of Avrami fractional kinetic equation in adsorption-based water treatment studies
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Monodisperse mesoporous silica nanoparticles of distinct topology
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The role of pre-nucleation clusters in the crystallization of gold nanoparticles
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Association phenomena. I. The growth of particles of silver chloride and the higher-order tyndall effect
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Toward Rationally Designing Surface Structures of Micro- and Nanocrystallites: Role of Supersaturation
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Seedless Continuous Injection Synthesis of Indium Phosphide Quantum Dots as a Route to Large Size and Low Size Dispersity
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A Four-Step Mechanism for the Formation of Supported-Nanoparticle Heterogenous Catalysts in Contact with Solution: The Conversion of Ir(1,5-COD)Cl/γ-Al ₂ O ₃ to Ir(0) _∼170 /γ-Al ₂ O ₃
journal, January 2014

Hydrothermal Synthesis of Ba-Hexaferrite Nanoparticles
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The Formation of Colloidal Gold
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Pre-nucleation clusters as solute precursors in crystallisation
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Nanocluster Nucleation, Growth, and Then Agglomeration Kinetic and Mechanistic Studies: A More General, Four-Step Mechanism Involving Double Autocatalysis
journal, October 2005

Sigmoidal Nucleation and Growth Curves Across Nature Fit by the Finke–Watzky Model of Slow Continuous Nucleation and Autocatalytic Growth: Explicit Formulas for the Lag and Growth Times Plus Other Key Insights
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On the Mechanism of Metal Nanoparticle Synthesis in the Brust–Schiffrin Method
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I.—On the Number of Dust Particles in the Atmosphere
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The preparation of monodisperse silver bromide and silver iodide sols
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