Organic Cathode Materials for Lithium–Ion Batteries: Past, Present, and Future

Lyu, Hailong; Sun, Xiao-Guang; Dai, Sheng

doi:10.1002/aesr.202000044

Title: Organic Cathode Materials for Lithium–Ion Batteries: Past, Present, and Future

Abstract

With the rapid development of energy storage systems in power supplies and electrical vehicles, the search for sustainable cathode materials to enhance the energy density of lithium‐ion batteries (LIBs) has become the focus in both academic and industrial studies. Currently, the widely utilized inorganic cathode materials suffer from drawbacks such as limited capacity, high energy consumption in production, safety hazards, and high‐cost raw materials. Therefore, it is necessary to develop green and sustainable cathode materials with higher specific capacity, better safety properties, and more abundant natural resources. As alternatives, organic cathode materials possess the advantages of high theoretical capacity, environmental friendliness, flexible structure design, systemic safety, and natural abundance, making them a promising class of energy storage materials. Herein, the development history of the organic cathode materials and recent research developments are reviewed, introducing several categories of typical organic compounds as cathode materials for LIBs, including conductive polymers, organosulfur compounds, radical compounds, carbonyl compounds, and imine compounds. The electrochemical performance, electrode reaction mechanism, and pros and cons of different organic cathode materials are comparatively analyzed to identify the challenges to be addressed. Finally, the future research and improvement directions of the organic cathode materials are also proposed.

Authors:

^[1]; Sun, Xiao-Guang ^[2]; Dai, Sheng ^[1]

Chemical Sciences Division Oak Ridge National Laboratory Oak Ridge TN 37831 USA, Department of Chemistry University of Tennessee Knoxville TN 37996 USA
Chemical Sciences Division Oak Ridge National Laboratory Oak Ridge TN 37831 USA

Publication Date:: 2020-11-11

Research Org.:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

OSTI Identifier:: 1712496

Alternate Identifier(s):: OSTI ID: 1763470; OSTI ID: 1786084

Grant/Contract Number:: AC05-00OR22725

Resource Type:: Published Article

Journal Name:: Advanced Energy and Sustainability Research

Additional Journal Information:: Journal Name: Advanced Energy and Sustainability Research; Journal ID: ISSN 2699-9412

Publisher:: Wiley

Country of Publication:: Germany

Language:: English

Subject:: 25 ENERGY STORAGE; energy storage; lithium-ion batteries; organic cathode materials; sustainability

Citation Formats


                    Lyu, Hailong, Sun, Xiao-Guang, and Dai, Sheng. Organic Cathode Materials for Lithium–Ion Batteries: Past, Present, and Future.  Germany: N. p., 2020. 
Web.  doi:10.1002/aesr.202000044.

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                    Lyu, Hailong, Sun, Xiao-Guang, & Dai, Sheng. Organic Cathode Materials for Lithium–Ion Batteries: Past, Present, and Future.  Germany.  https://doi.org/10.1002/aesr.202000044

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                    Lyu, Hailong, Sun, Xiao-Guang, and Dai, Sheng. Wed .  
"Organic Cathode Materials for Lithium–Ion Batteries: Past, Present, and Future".  Germany.  https://doi.org/10.1002/aesr.202000044.

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@article{osti_1712496,

  title        = {Organic Cathode Materials for Lithium–Ion Batteries: Past, Present, and Future},

  author       = {Lyu, Hailong and Sun, Xiao-Guang and Dai, Sheng},

  abstractNote = {With the rapid development of energy storage systems in power supplies and electrical vehicles, the search for sustainable cathode materials to enhance the energy density of lithium‐ion batteries (LIBs) has become the focus in both academic and industrial studies. Currently, the widely utilized inorganic cathode materials suffer from drawbacks such as limited capacity, high energy consumption in production, safety hazards, and high‐cost raw materials. Therefore, it is necessary to develop green and sustainable cathode materials with higher specific capacity, better safety properties, and more abundant natural resources. As alternatives, organic cathode materials possess the advantages of high theoretical capacity, environmental friendliness, flexible structure design, systemic safety, and natural abundance, making them a promising class of energy storage materials. Herein, the development history of the organic cathode materials and recent research developments are reviewed, introducing several categories of typical organic compounds as cathode materials for LIBs, including conductive polymers, organosulfur compounds, radical compounds, carbonyl compounds, and imine compounds. The electrochemical performance, electrode reaction mechanism, and pros and cons of different organic cathode materials are comparatively analyzed to identify the challenges to be addressed. Finally, the future research and improvement directions of the organic cathode materials are also proposed.},

  doi          = {10.1002/aesr.202000044},

  journal      = {Advanced Energy and Sustainability Research},

  number       = ,

  volume       = ,

  place        = {Germany},

  year         = {2020},

  month        = {11}

}

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Publisher Correction: Advances and issues in developing salt-concentrated battery electrolytes
journal, March 2019

Reversible anion intercalation in a layered aromatic amine: a high-voltage host structure for organic batteries
journal, January 2016

Recent Progress in Multivalent Metal (Mg, Zn, Ca, and Al) and Metal‐Ion Rechargeable Batteries with Organic Materials as Promising Electrodes
journal, March 2019

High-voltage performance of LiCoO2/graphite batteries with methylene methanedisulfonate as electrolyte additive
journal, December 2012

Electrochromic and electrochemical capacitive properties of tungsten oxide and its polyaniline nanocomposite films obtained by chemical bath deposition method
journal, May 2014

Concentration-controlled morphology of LiFePO4 crystals with an exposed (100) facet and their enhanced performance for use in lithium-ion batteries
journal, April 2018

Organosulfides: An Emerging Class of Cathode Materials for Rechargeable Lithium Batteries
journal, July 2019

Lithium Salt of Tetrahydroxybenzoquinone: Toward the Development of a Sustainable Li-Ion Battery
journal, July 2009

Azo compounds as a family of organic electrode materials for alkali-ion batteries
journal, February 2018

Conductive nonconjugated radical polymer as high capacity organic cathode material for high-energy Li/Na ion batteries
journal, December 2020

Binding Zinc Ions by Carboxyl Groups from Adjacent Molecules toward Long‐Life Aqueous Zinc–Organic Batteries
journal, March 2020

Superior performance for lithium-ion battery with organic cathode and ionic liquid electrolyte
journal, January 2021

Safe and recyclable lithium-ion capacitors using sacrificial organic lithium salt
journal, December 2017

Ortho-di-sodium salts of tetrahydroxyquinone as a novel electrode for lithium-ion and potassium-ion batteries
journal, January 2019

Introduction of two lithiooxycarbonyl groups enhances cyclability of lithium batteries with organic cathode materials
journal, August 2014

Rapid gas-assisted exfoliation promises V2O5 nanosheets for high performance lithium-sulfur batteries
journal, January 2020

"Water-in-salt" electrolyte enables high-voltage aqueous lithium-ion chemistries
journal, November 2015

Rechargeable Lithium–Sulfur Batteries
journal, July 2014

Polyphenyl polysulfide: a new polymer cathode material for Li–S batteries
journal, January 2019

A Carbonyl Compound-Based Flexible Cathode with Superior Rate Performance and Cyclic Stability for Flexible Lithium-Ion Batteries
journal, December 2017

5,7,12,14-Pentacenetetrone as a High-Capacity Organic Positive-Electrode Material for Use in Rechargeable Lithium Batteries
journal, July 2011

A MC/AQ Parasitic Composite as Cathode Material for Lithium Battery
journal, January 2011

A 3D cross-linked graphene-based honeycomb carbon composite with excellent confinement effect of organic cathode material for lithium-ion batteries
journal, February 2020

Microwave-assisted optimization of the manganese redox states for enhanced capacity and capacity retention of LiAl _x Mn _2−x O ₄ (x = 0 and 0.3) spinel materials
journal, January 2015

Redox polymers for rechargeable metal-ion batteries
journal, May 2020

Characterization of PEDOT-Quinone Conducting Redox Polymers for Water Based Secondary Batteries
journal, May 2017

A 2D covalent organic framework as a high-performance cathode material for lithium-ion batteries
journal, April 2020

New Naphthalene‐Based Polyimide as an Environment‐Friendly Organic Cathode Material for Lithium Batteries
journal, April 2019

An All-Organic Aqueous Battery Powered by Adsorbed Quinone
journal, June 2019

Li-Ion Storage Performance of MnO Nanoparticles Coated with Nitrogen-Doped Carbon Derived from Different Carbon Sources
journal, November 2014

Simultaneously Boosting the Ionic Conductivity and Mechanical Strength of Polymer Gel Electrolyte Membranes by Confining Ionic Liquids into Hollow Silica Nanocavities
journal, September 2019

Enhanced electrochemical performance of barium hexaferrite nanoplates by Zn ²⁺ doping serving as anode materials
journal, January 2015

Ten years left to redesign lithium-ion batteries
journal, July 2018

Significantly stable organic cathode for lithium-ion battery based on nanoconfined poly(anthraquinonyl sulfide)@MOF-derived microporous carbon
journal, March 2020

Microwave Irradiation Controls the Manganese Oxidation States of Nanostructured (Li[Li _0.2 Mn _0.52 Ni _0.13 Co _0.13 Al _0.02 ]O ₂ ) Layered Cathode Materials for High-Performance Lithium Ion Batteries
journal, January 2015

Renewable-Biomolecule-Based Full Lithium-Ion Batteries
journal, March 2016

High-performance Lithium Secondary Batteries Using Cathode Active Materials of Triquinoxalinylenes Exhibiting Six Electron Migration
journal, July 2011

A H-bond stabilized quinone electrode material for Li–organic batteries: the strength of weak bonds
journal, January 2019

Combination of high performance organic cathode Calix[4]quinone and practical biocarbon in sodium-ion batteries
journal, July 2020

Poly(5-amino-1,4-naphthoquinone), a Novel Lithium-Inserting Electroactive Polymer with High Specific Charge
journal, January 1999

Electrodes with High Power and High Capacity for Rechargeable Lithium Batteries
journal, February 2006

Diffusion-Cooperative Model for Charge Transport by Redox-Active Nonconjugated Polymers
journal, January 2018

New Spin on Organic Radical Batteries–An Isoindoline Nitroxide-Based High-Voltage Cathode Material
journal, February 2018

Anthraquinone based polymer as high performance cathode material for rechargeable lithium batteries
journal, January 2009

Towards the selective modification of soft-templated mesoporous carbon materials by elemental fluorine for energy storage devices
journal, January 2013

Symmetric All-Quinone Aqueous Battery
journal, May 2019

Porous Ti ₄ O ₇ Particles with Interconnected-Pore Structure as a High-Efficiency Polysulfide Mediator for Lithium-Sulfur Batteries
journal, May 2017

Single Nickel Atoms on Nitrogen‐Doped Graphene Enabling Enhanced Kinetics of Lithium–Sulfur Batteries
journal, August 2019

Recent progress in metal–organic polymers as promising electrodes for lithium/sodium rechargeable batteries
journal, January 2019

Recent progress in carbonyl-based organic polymers as promising electrode materials for lithium-ion batteries (LIBs)
journal, January 2020

Flexible, aqueous-electrolyte supercapacitors based on water-processable dioxythiophene polymer/carbon nanotube textile electrodes
journal, January 2017

Recent Progress in Polymeric Carbonyl-Based Electrode Materials for Lithium and Sodium Ion Batteries
journal, November 2018

Organic Electrode Materials for Rechargeable Lithium Batteries
journal, May 2012

Molecular Design Strategies for Electrochemical Behavior of Aromatic Carbonyl Compounds in Organic and Aqueous Electrolytes
journal, July 2019

New intercalation compounds for lithium batteries: layered LiMnO2
journal, January 1999

Polysulfurating reagent design for unsymmetrical polysulfide construction
journal, June 2018

Real-time insight into the doping mechanism of redox-active organic radical polymers
journal, November 2018

An Insoluble Benzoquinone-Based Organic Cathode for Use in Rechargeable Lithium-Ion Batteries
journal, August 2017

Graphene wrapped 3,4,9,10-perylenetetracarboxylic dianhydride as a high-performance organic cathode for lithium ion batteries
journal, January 2016

A Novel Conductive Polymer-Sulfur Composite Cathode Material for Rechargeable Lithium Batteries
journal, July 2002

Ionic Conductivity of Organosulfur Melts for Advanced Storage Electrodes
journal, January 1988

Ionic Liquid‐Directed Nanoporous TiNb ₂ O ₇ Anodes with Superior Performance for Fast‐Rechargeable Lithium‐Ion Batteries
journal, June 2020

Rechargeable quasi-solid state lithium battery with organic crystalline cathode
journal, June 2012

Unraveling the storage mechanism in organic carbonyl electrodes for sodium-ion batteries
journal, September 2015

From Biomass to a Renewable LiXC6O6 Organic Electrode for Sustainable Li-Ion Batteries
journal, April 2008

Polyquinoneimines for lithium storage: more than the sum of its parts
journal, January 2016

Utilizing Latent Multi‐Redox Activity of p‐Type Organic Cathode Materials toward High Energy Density Lithium‐Organic Batteries
journal, July 2020

Phenyl Selenosulfides as Cathode Materials for Rechargeable Lithium Batteries
journal, June 2018

Challenges for Rechargeable Li Batteries
journal, February 2010

Proton trap effect on catechol–pyridine redox polymer nanoparticles as organic electrodes for lithium batteries
journal, January 2020

How Many Lithium Ions Can Be Inserted onto Fused C ₆ Aromatic Ring Systems?
journal, April 2012

Lithium Iron Aluminum Nickelate, LiNi _x Fe _y Al _z O ₂ —New Sustainable Cathodes for Next‐Generation Cobalt‐Free Li‐Ion Batteries
journal, July 2020

All-Solid-State Lithium Organic Battery with Composite Polymer Electrolyte and Pillar[5]quinone Cathode
journal, November 2014

Toward Improved Performance of All-Organic Nitroxide Radical Batteries with Ionic Liquids: A Theoretical Perspective
journal, February 2019