Partially disordered state with short-range spin correlation in classical triangular antiferromagnet
Abstract
A triangular-lattice antiferromagnet of was synthesized under high pressure. Its magnetism was studied in terms of electrical resistivity, magnetic susceptibility, heat capacity, powder neutron scattering, and Mössbauer spectroscopy. The magnetic state of changes successively through a second-order phase transition at K and a crossover at K. A partially disordered (PD) state appears below , in which spins are ordered and the remaining spins fluctuate, which state persists at least down to 5 K. The spin correlation length starts to grow at ; however, it remains very short ( Å) below . This exotic magnetism is concerned with strong frustration in the classic antiferromagnetic triangular lattice.
- Authors:
- Publication Date:
- Research Org.:
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES); Japan Society for the Promotion of Science (JSPS)
- OSTI Identifier:
- 1708977
- Alternate Identifier(s):
- OSTI ID: 1712720
- Grant/Contract Number:
- AC05-00OR22725; 22-10454; 18K03529; 22560676; 22246083
- Resource Type:
- Published Article
- Journal Name:
- Physical Review Research
- Additional Journal Information:
- Journal Name: Physical Review Research Journal Volume: 2 Journal Issue: 4; Journal ID: ISSN 2643-1564
- Publisher:
- American Physical Society (APS)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; Antiferromagnetism; triangular network; Mossbauer spectroscopy; neutron scattering
Citation Formats
Yoshida, H. K., Matsuda, M., Stone, M. B., dela Cruz, C. R., Furubayashi, T., Onoda, M., Takayama-Muromachi, E., and Isobe, M. Partially disordered state with short-range spin correlation in S = 5 / 2 classical triangular antiferromagnet Ag 2 FeO 2. United States: N. p., 2020.
Web. doi:10.1103/PhysRevResearch.2.043211.
Yoshida, H. K., Matsuda, M., Stone, M. B., dela Cruz, C. R., Furubayashi, T., Onoda, M., Takayama-Muromachi, E., & Isobe, M. Partially disordered state with short-range spin correlation in S = 5 / 2 classical triangular antiferromagnet Ag 2 FeO 2. United States. https://doi.org/10.1103/PhysRevResearch.2.043211
Yoshida, H. K., Matsuda, M., Stone, M. B., dela Cruz, C. R., Furubayashi, T., Onoda, M., Takayama-Muromachi, E., and Isobe, M. Tue .
"Partially disordered state with short-range spin correlation in S = 5 / 2 classical triangular antiferromagnet Ag 2 FeO 2". United States. https://doi.org/10.1103/PhysRevResearch.2.043211.
@article{osti_1708977,
title = {Partially disordered state with short-range spin correlation in S = 5 / 2 classical triangular antiferromagnet Ag 2 FeO 2},
author = {Yoshida, H. K. and Matsuda, M. and Stone, M. B. and dela Cruz, C. R. and Furubayashi, T. and Onoda, M. and Takayama-Muromachi, E. and Isobe, M.},
abstractNote = {A triangular-lattice antiferromagnet of Ag2FeO2 was synthesized under high pressure. Its magnetism was studied in terms of electrical resistivity, magnetic susceptibility, heat capacity, powder neutron scattering, and Mössbauer spectroscopy. The magnetic state of Ag2FeO2 changes successively through a second-order phase transition at Tp=36 K and a crossover at Tc=20 K. A partially disordered (PD) state appears below Tp, in which ≈2/3 spins are ordered and the remaining ≈1/3 spins fluctuate, which state persists at least down to 5 K. The spin correlation length starts to grow at Tp; however, it remains very short (≈27 Å) below Tc. This exotic magnetism is concerned with strong frustration in the classic antiferromagnetic triangular lattice.},
doi = {10.1103/PhysRevResearch.2.043211},
journal = {Physical Review Research},
number = 4,
volume = 2,
place = {United States},
year = {Tue Nov 10 00:00:00 EST 2020},
month = {Tue Nov 10 00:00:00 EST 2020}
}
https://doi.org/10.1103/PhysRevResearch.2.043211
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