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Title: Molecular beam epitaxy of the magnetic Kagome metal FeSn on LaAlO3 (111)

Abstract

Materials with Kagome layers are expected to give rise to rich physics arising from band structures with topological properties, spin liquid behavior, and the formation of Skyrmions. Until now, most work on Kagome materials has been performed on bulk samples due to difficulties in thin film synthesis. Here, by using molecular beam epitaxy, layered Kagome-structured FeSn films are synthesized on the (111) oriented LaAlO3 substrate. Both in situ and ex situ characterizations indicate that these films are highly crystalline and c-axis oriented, with atomically smooth surfaces. The films grow as disconnected islands, with lateral dimensions on the micron meter scale. By patterning Pt electrodes using a focused electron beam, the longitudinal and transverse resistance of single islands have been measured in magnetic fields. Our work opens a pathway for exploring mesoscale transport properties in thin films of Kagome materials and related devices.

Authors:
 [1];  [1];  [2];  [3];  [1];  [2]; ORCiD logo [1]
  1. Argonne National Lab. (ANL), Argonne, IL (United States)
  2. Univ. of Illinois at Urbana-Champaign, IL (United States)
  3. Argonne National Lab. (ANL), Argonne, IL (United States). Center for Nanoscale Materials
Publication Date:
Research Org.:
Argonne National Lab. (ANL), Argonne, IL (United States). Center for Nanoscale Materials; Energy Frontier Research Centers (EFRC) (United States). Center for the Advancement of Topological Semimetals (CATS)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
OSTI Identifier:
1671751
Alternate Identifier(s):
OSTI ID: 1671848
Grant/Contract Number:  
AC02-06CH11357
Resource Type:
Accepted Manuscript
Journal Name:
AIP Advances
Additional Journal Information:
Journal Volume: 10; Journal Issue: 10; Journal ID: ISSN 2158-3226
Publisher:
American Institute of Physics (AIP)
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE; Epitaxy; Topological properties; Ferromagnetism; Kagome lattices

Citation Formats

Hong, Deshun, Liu, Changjiang, Hsiao, Haw-Wen, Jin, Dafei, Pearson, John E., Zuo, Jian-Min, and Bhattacharya, Anand. Molecular beam epitaxy of the magnetic Kagome metal FeSn on LaAlO3 (111). United States: N. p., 2020. Web. doi:10.1063/5.0001909.
Hong, Deshun, Liu, Changjiang, Hsiao, Haw-Wen, Jin, Dafei, Pearson, John E., Zuo, Jian-Min, & Bhattacharya, Anand. Molecular beam epitaxy of the magnetic Kagome metal FeSn on LaAlO3 (111). United States. https://doi.org/10.1063/5.0001909
Hong, Deshun, Liu, Changjiang, Hsiao, Haw-Wen, Jin, Dafei, Pearson, John E., Zuo, Jian-Min, and Bhattacharya, Anand. Mon . "Molecular beam epitaxy of the magnetic Kagome metal FeSn on LaAlO3 (111)". United States. https://doi.org/10.1063/5.0001909. https://www.osti.gov/servlets/purl/1671751.
@article{osti_1671751,
title = {Molecular beam epitaxy of the magnetic Kagome metal FeSn on LaAlO3 (111)},
author = {Hong, Deshun and Liu, Changjiang and Hsiao, Haw-Wen and Jin, Dafei and Pearson, John E. and Zuo, Jian-Min and Bhattacharya, Anand},
abstractNote = {Materials with Kagome layers are expected to give rise to rich physics arising from band structures with topological properties, spin liquid behavior, and the formation of Skyrmions. Until now, most work on Kagome materials has been performed on bulk samples due to difficulties in thin film synthesis. Here, by using molecular beam epitaxy, layered Kagome-structured FeSn films are synthesized on the (111) oriented LaAlO3 substrate. Both in situ and ex situ characterizations indicate that these films are highly crystalline and c-axis oriented, with atomically smooth surfaces. The films grow as disconnected islands, with lateral dimensions on the micron meter scale. By patterning Pt electrodes using a focused electron beam, the longitudinal and transverse resistance of single islands have been measured in magnetic fields. Our work opens a pathway for exploring mesoscale transport properties in thin films of Kagome materials and related devices.},
doi = {10.1063/5.0001909},
journal = {AIP Advances},
number = 10,
volume = 10,
place = {United States},
year = {Mon Oct 12 00:00:00 EDT 2020},
month = {Mon Oct 12 00:00:00 EDT 2020}
}

Works referenced in this record:

Evidence for magnetic Weyl fermions in a correlated metal
journal, September 2017

  • Kuroda, K.; Tomita, T.; Suzuki, M. -T.
  • Nature Materials, Vol. 16, Issue 11
  • DOI: 10.1038/nmat4987

Unconventional superconductivity in magic-angle graphene superlattices
journal, March 2018


Large anomalous Hall effect in a non-collinear antiferromagnet at room temperature
journal, October 2015

  • Nakatsuji, Satoru; Kiyohara, Naoki; Higo, Tomoya
  • Nature, Vol. 527, Issue 7577
  • DOI: 10.1038/nature15723

Gate-tunable negative longitudinal magnetoresistance in the predicted type-II Weyl semimetal WTe2
journal, October 2016

  • Wang, Yaojia; Liu, Erfu; Liu, Huimei
  • Nature Communications, Vol. 7, Issue 1
  • DOI: 10.1038/ncomms13142

Electronics and optoelectronics of two-dimensional transition metal dichalcogenides
journal, November 2012

  • Wang, Qing Hua; Kalantar-Zadeh, Kourosh; Kis, Andras
  • Nature Nanotechnology, Vol. 7, Issue 11, p. 699-712
  • DOI: 10.1038/nnano.2012.193

Epitaxial growth of ultraflat stanene with topological band inversion
journal, November 2018


Observation of a three-dimensional topological Dirac semimetal phase in high-mobility Cd3As2
journal, May 2014

  • Neupane, Madhab; Xu, Su-Yang; Sankar, Raman
  • Nature Communications, Vol. 5, Issue 1
  • DOI: 10.1038/ncomms4786

Massive Dirac fermions in a ferromagnetic kagome metal
journal, March 2018


Epitaxial growth of Bi 2 Se 3 topological insulator thin films on Si (111)
journal, May 2011

  • He, Liang; Xiu, Faxian; Wang, Yong
  • Journal of Applied Physics, Vol. 109, Issue 10
  • DOI: 10.1063/1.3585673

Large anomalous Hall effect driven by a nonvanishing Berry curvature in the noncolinear antiferromagnet Mn 3 Ge
journal, April 2016

  • Nayak, Ajaya K.; Fischer, Julia Erika; Sun, Yan
  • Science Advances, Vol. 2, Issue 4
  • DOI: 10.1126/sciadv.1501870

Dirac fermions and flat bands in the ideal kagome metal FeSn
journal, December 2019


Correlated insulator behaviour at half-filling in magic-angle graphene superlattices
journal, March 2018


Topological metal at the surface of an ultrathin Bi 1 x Sb x alloy film
journal, April 2010


Topological Insulator Thin Films of Bi2Te3 with Controlled Electronic Structure
journal, May 2011


Topological Weyl semimetals in the chiral antiferromagnetic materials Mn 3 Ge and Mn 3 Sn
journal, January 2017


Molecular beam epitaxy growth of antiferromagnetic Kagome metal FeSn
journal, August 2019

  • Inoue, Hisashi; Han, Minyong; Ye, Linda
  • Applied Physics Letters, Vol. 115, Issue 7
  • DOI: 10.1063/1.5111792

Giant and anisotropic many-body spin–orbit tunability in a strongly correlated kagome magnet
journal, September 2018