Determination of the Raman polarizability tensor in the optically anisotropic crystal potassium dihydrogen phosphate and its deuterated analog
Abstract
Here, the Raman tensor of the dominant A1 modes of the nonlinear optical crystalline material potassium dihydrogen phosphate and its 70% deuterated analog have been ascertained. Challenges in determining the A1 mode tensor element values based on previous reports have been resolved using a specially designed experimental setup that makes use of spherical crystal samples. This novel experimental design enabled the determination of measurement artifacts, including polarization rotation of the pump and/or scattered light propagating through the sample and the contribution of additional overlapping phonon modes, which have hindered previous efforts. Results confirmed that the polarization tensor is diagonal, and matrix elements were determined with high accuracy.
- Authors:
- Publication Date:
- Research Org.:
- Univ. of Rochester, NY (United States). Lab. for Laser Energetics; Lawrence Livermore National Laboratory (LLNL), Livermore, CA (United States)
- Sponsoring Org.:
- USDOE National Nuclear Security Administration (NNSA)
- Contributing Org.:
- Laboratory for Laser Energetics, University of Rochester
- OSTI Identifier:
- 1669168
- Alternate Identifier(s):
- OSTI ID: 1669222; OSTI ID: 1675369
- Report Number(s):
- LLNL-JRNL-812283; 2020-161, 1587, 2542
Journal ID: ISSN 2045-2322; 16283; PII: 73163
- Grant/Contract Number:
- NA0003856; AC52-07NA27344
- Resource Type:
- Published Article
- Journal Name:
- Scientific Reports
- Additional Journal Information:
- Journal Name: Scientific Reports Journal Volume: 10 Journal Issue: 1; Journal ID: ISSN 2045-2322
- Publisher:
- Nature Publishing Group
- Country of Publication:
- United Kingdom
- Language:
- English
- Subject:
- characterization and analytical techniques; nonlinear optics; Raman spectroscopy; 36 MATERIALS SCIENCE
Citation Formats
Kosc, T. Z., Huang, H., Kessler, T. J., Negres, R. A., and Demos, S. G. Determination of the Raman polarizability tensor in the optically anisotropic crystal potassium dihydrogen phosphate and its deuterated analog. United Kingdom: N. p., 2020.
Web. doi:10.1038/s41598-020-73163-4.
Kosc, T. Z., Huang, H., Kessler, T. J., Negres, R. A., & Demos, S. G. Determination of the Raman polarizability tensor in the optically anisotropic crystal potassium dihydrogen phosphate and its deuterated analog. United Kingdom. https://doi.org/10.1038/s41598-020-73163-4
Kosc, T. Z., Huang, H., Kessler, T. J., Negres, R. A., and Demos, S. G. Thu .
"Determination of the Raman polarizability tensor in the optically anisotropic crystal potassium dihydrogen phosphate and its deuterated analog". United Kingdom. https://doi.org/10.1038/s41598-020-73163-4.
@article{osti_1669168,
title = {Determination of the Raman polarizability tensor in the optically anisotropic crystal potassium dihydrogen phosphate and its deuterated analog},
author = {Kosc, T. Z. and Huang, H. and Kessler, T. J. and Negres, R. A. and Demos, S. G.},
abstractNote = {Here, the Raman tensor of the dominant A1 modes of the nonlinear optical crystalline material potassium dihydrogen phosphate and its 70% deuterated analog have been ascertained. Challenges in determining the A1 mode tensor element values based on previous reports have been resolved using a specially designed experimental setup that makes use of spherical crystal samples. This novel experimental design enabled the determination of measurement artifacts, including polarization rotation of the pump and/or scattered light propagating through the sample and the contribution of additional overlapping phonon modes, which have hindered previous efforts. Results confirmed that the polarization tensor is diagonal, and matrix elements were determined with high accuracy.},
doi = {10.1038/s41598-020-73163-4},
journal = {Scientific Reports},
number = 1,
volume = 10,
place = {United Kingdom},
year = {Thu Oct 01 00:00:00 EDT 2020},
month = {Thu Oct 01 00:00:00 EDT 2020}
}
Free Publicly Available Full Text
Publisher's Version of Record
https://doi.org/10.1038/s41598-020-73163-4
https://doi.org/10.1038/s41598-020-73163-4
Other availability
Search WorldCat to find libraries that may hold this journalFigures / Tables:
Figure 1: Experimental geometry for a Raman scattering measurement based on a spherical sample.
All figures and tables
(5 total)
Save to My Library
You must Sign In or Create an Account in order to save documents to your library.
Works referenced in this record:
High-power tunable IR Raman lasers
journal, November 1978
- Grasiuk, A. Z.; Zubarev, I. G.
- Applied Physics, Vol. 17, Issue 3
Elucidation of “phase difference” in Raman tensor formalism
journal, January 2018
- Zheng, Wei; Yan, Jingshen; Li, Fadi
- Photonics Research, Vol. 6, Issue 7
Measurement of the Raman scattering cross section of the breathing mode in KDP and DKDP crystals
journal, January 2011
- Demos, Stavros G.; Raman, Rajesh N.; Yang, Steven T.
- Optics Express, Vol. 19, Issue 21
Transverse stimulated Raman scattering in KDP
conference, December 1995
- Barker, Charles E.; Sacks, Richard A.; Van Wonterghem, Bruno M.
- Solid State Lasers for Application to Inertial Confinement Fusion (ICF), SPIE Proceedings
Raman Effect in Zinc Oxide
journal, February 1966
- Damen, T. C.; Porto, S. P. S.; Tell, B.
- Physical Review, Vol. 142, Issue 2
Accurate measurements of the Raman scattering coefficient and the depolarization ratio in liquid water
journal, January 2013
- Bray, Andrew; Chapman, Robert; Plakhotnik, Taras
- Applied Optics, Vol. 52, Issue 11
The Laser Mégajoule (LMJ) Project dedicated to inertial confinement fusion: Development and construction status
journal, November 2005
- Fleurot, Noël; Cavailler, Claude; Bourgade, J. L.
- Fusion Engineering and Design, Vol. 74, Issue 1-4
Demonstration of high efficiency third harmonic conversion of high power Nd-glass laser radiation
journal, September 1980
- Seka, W.; Jacobs, S. D.; Rizzo, J. E.
- Optics Communications, Vol. 34, Issue 3
Reduction of laser imprinting using polarization smoothing on a solid-state fusion laser
journal, April 1999
- Boehly, T. R.; Smalyuk, V. A.; Meyerhofer, D. D.
- Journal of Applied Physics, Vol. 85, Issue 7
The Raman effect in crystals
journal, October 1964
- Loudon, R.
- Advances in Physics, Vol. 13, Issue 52
Raman Tensor Formalism for Optically Anisotropic Crystals
journal, March 2016
- Kranert, Christian; Sturm, Chris; Schmidt-Grund, Rüdiger
- Physical Review Letters, Vol. 116, Issue 12
Hydrogen modes in KDP/DKDP mixed crystals
journal, February 2003
- Tominaga, Yasunori; Kawahata, Yoshimi; Amo, Yuko
- Solid State Communications, Vol. 125, Issue 7-8
Experimental progress of inertial confinement fusion based at the ShenGuang-III laser facility in China
journal, December 2018
- Jiang, Shaoen; Wang, Feng; Ding, Yongkun
- Nuclear Fusion, Vol. 59, Issue 3
Depolarization of Raman Scattering in La
journal, April 1968
- Asawa, C. K.; Satten, R. A.; Stafsudd, O. M.
- Physical Review, Vol. 168, Issue 3
The physics basis for ignition using indirect-drive targets on the National Ignition Facility
journal, February 2004
- Lindl, John D.; Amendt, Peter; Berger, Richard L.
- Physics of Plasmas, Vol. 11, Issue 2
Damage Mechanisms Avoided or Managed for NIF Large Optics
journal, February 2016
- Manes, K. R.; Spaeth, M. L.; Adams, J. J.
- Fusion Science and Technology, Vol. 69, Issue 1
Breakdown of selection rules in the Raman spectra of KDP
journal, January 1975
- Srivastava, M. K.
- The Journal of Chemical Physics, Vol. 62, Issue 9
Raman scattering and in-water ocean optical properties
journal, January 1990
- Marshall, Bruce R.; Smith, Raymond C.
- Applied Optics, Vol. 29, Issue 1
Measurement of the angular dependence of the spontaneous Raman scattering in anisotropic crystalline materials using spherical samples: Potassium dihydrogen phosphate as a case example
journal, January 2020
- Kosc, T. Z.; Huang, H.; Kessler, T. J.
- Review of Scientific Instruments, Vol. 91, Issue 1
Theory of Stimulated Brillouin and Raman Scattering
journal, March 1965
- Shen, Y. R.; Bloembergen, N.
- Physical Review, Vol. 137, Issue 6A
Depolarization of Raman Scattering in Calcite
journal, July 1966
- Porto, S. P. S.; Giordmaine, J. A.; Damen, T. C.
- Physical Review, Vol. 147, Issue 2
Internal modes and local symmetry of PO4 tetrahedrons in KH2PO4 by Raman scattering
journal, October 1983
- Tominaga, Y.; Urabe, H.; Tokunaga, M.
- Solid State Communications, Vol. 48, Issue 3
Polarization smoothing on the national ignition facility
journal, June 2006
- Dixit, S. N.; Munro, D.; Murray, J. R.
- Journal de Physique IV (Proceedings), Vol. 133
Angular Dependence and Depolarization Ratio of the Raman Effect
journal, January 1966
- Porto, S. P. S.
- Journal of the Optical Society of America, Vol. 56, Issue 11
Figures / Tables found in this record:
Figures/Tables have been extracted from DOE-funded journal article accepted manuscripts.