Instability and evolution of the magnetic ground state in metallic perovskites GdRh3C1-xBx
Abstract
In this paper, we report investigations of the structural, magnetic, electrical transport and thermal properties of five compositions of the metallic perovskite GdRh3C1–xBx (0.00 ≤ x ≤ 1.00). Our results show that all the five compositions undergo magnetic ordering at low temperatures, but the nature of the ordered state is significantly different in the carbon- and the boron-rich compositions, where the former shows signatures of an amplitude-modulated magnetic structure and the latter exhibits evidences of an equal-moment incommensurate antiferromagnetic ordering. We also observe a remarkable field-dependent evolution of conduction carrier polarization in the compositionally disordered compounds. The outcomes indicate that this system is energetically situated in proximity to a magnetic instability where small variations in the control parameter(s), such as lattice constant and/or electron density, lead to considerably different ground states.
- Authors:
-
[1];
[2];
[3];
[2];
[7];
- Univ. of the Witwatersrand, Johannesburg (South Africa)
- Indian Inst. of Technology (IIT), Varanasi (India)
- Univ. of Burdwan, Bengal (India)
- P. C. Vigyan College, Bihar (India)
- Saha Inst. of Nuclear Physics, Bengal (Indian)
- National Inst. of Technology, Jharkhand (India)
- Ames Lab., and Iowa State Univ., Ames, IA (United States)
- Publication Date:
- Research Org.:
- Ames Laboratory (AMES), Ames, IA (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division; Wits University Research Committee; Wits University Faculty Research Committee
- OSTI Identifier:
- 1663151
- Report Number(s):
- IS-J-10,316
Journal ID: ISSN 2475-9953; TRN: US2203779
- Grant/Contract Number:
- AC02-07CH11358; 001.254.87581018503; 001.000.8758101.3113101
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Physical Review Materials
- Additional Journal Information:
- Journal Volume: 4; Journal Issue: 8; Journal ID: ISSN 2475-9953
- Publisher:
- American Physical Society (APS)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE
Citation Formats
Pandey, Abhishek, Singh, A. K., Dan, Shovan, Ghosh, K., Das, I., Tripathi, S., Kumar, U., Ranganathan, R., Johnston, D. C., and Mazumdar, Chandan. Instability and evolution of the magnetic ground state in metallic perovskites GdRh3C1-xBx. United States: N. p., 2020.
Web. doi:10.1103/physrevmaterials.4.084411.
Pandey, Abhishek, Singh, A. K., Dan, Shovan, Ghosh, K., Das, I., Tripathi, S., Kumar, U., Ranganathan, R., Johnston, D. C., & Mazumdar, Chandan. Instability and evolution of the magnetic ground state in metallic perovskites GdRh3C1-xBx. United States. https://doi.org/10.1103/physrevmaterials.4.084411
Pandey, Abhishek, Singh, A. K., Dan, Shovan, Ghosh, K., Das, I., Tripathi, S., Kumar, U., Ranganathan, R., Johnston, D. C., and Mazumdar, Chandan. Mon .
"Instability and evolution of the magnetic ground state in metallic perovskites GdRh3C1-xBx". United States. https://doi.org/10.1103/physrevmaterials.4.084411. https://www.osti.gov/servlets/purl/1663151.
@article{osti_1663151,
title = {Instability and evolution of the magnetic ground state in metallic perovskites GdRh3C1-xBx},
author = {Pandey, Abhishek and Singh, A. K. and Dan, Shovan and Ghosh, K. and Das, I. and Tripathi, S. and Kumar, U. and Ranganathan, R. and Johnston, D. C. and Mazumdar, Chandan},
abstractNote = {In this paper, we report investigations of the structural, magnetic, electrical transport and thermal properties of five compositions of the metallic perovskite GdRh3C1–xBx (0.00 ≤ x ≤ 1.00). Our results show that all the five compositions undergo magnetic ordering at low temperatures, but the nature of the ordered state is significantly different in the carbon- and the boron-rich compositions, where the former shows signatures of an amplitude-modulated magnetic structure and the latter exhibits evidences of an equal-moment incommensurate antiferromagnetic ordering. We also observe a remarkable field-dependent evolution of conduction carrier polarization in the compositionally disordered compounds. The outcomes indicate that this system is energetically situated in proximity to a magnetic instability where small variations in the control parameter(s), such as lattice constant and/or electron density, lead to considerably different ground states.},
doi = {10.1103/physrevmaterials.4.084411},
journal = {Physical Review Materials},
number = 8,
volume = 4,
place = {United States},
year = {Mon Aug 31 00:00:00 EDT 2020},
month = {Mon Aug 31 00:00:00 EDT 2020}
}
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