Record-Breaking Magnetoresistance at the Edge of a Microflake of Natural Graphite

Precker, Christian E.; Barzola-Quiquia, José; Esquinazi, Pablo D.; Stiller, Markus; Chan, Mun K.; Jaime, Marcelo; Zhang, Zhipeng; Grundmann, Marius

doi:10.1002/adem.201900991

Title: Record-Breaking Magnetoresistance at the Edge of a Microflake of Natural Graphite

Abstract

Placing several electrodes at the edge of a micrometer-size Sri Lankan natural graphite sample at distances comparable to the size of the internal crystalline regions, we found record values for the change of the resistance with magnetic field. At low temperatures and at B ~ 21 T the magnetoresistance (MR) reaches ≈ 10⁷%. The MR values exceed by far all earlier reported ones for graphite and they are comparable or even larger (at T > 50 K) than the largest reported in solids including the Weyl semimetals. The origin of this large MR lies in the existence of highly conducting 2D interfaces aligned parallel to the graphene planes.

Authors:

Precker, Christian E. ^[1]; Barzola-Quiquia, José ^[1]; Esquinazi, Pablo D. ^[1]; Stiller, Markus ^[1]; Chan, Mun K. ^[2];

^[2]; Zhang, Zhipeng ^[3]; Grundmann, Marius ^[3]

Univ. of Leipzig (Germany). Felix Bloch Institute, Div. of Superconductivity and Magnetism
Los Alamos National Lab. (LANL), Los Alamos, NM (United States). National High Magnetic Field Lab. (MagLab), Pulsed Field Facility
Univ. of Leipzig (Germany). Felix Bloch Institute, Semiconductor Physics Group

Publication Date:: 2019-11-11

Research Org.:: Los Alamos National Lab. (LANL), Los Alamos, NM (United States)

Sponsoring Org.:: USDOE Office of Science (SC). Basic Energy Sciences (BES) (SC-22)

OSTI Identifier:: 1660594

Report Number(s):: LA-UR-19-25219
Journal ID: ISSN 1438-1656

Grant/Contract Number:: 89233218CNA000001

Resource Type:: Accepted Manuscript

Journal Name:: Advanced Engineering Materials

Additional Journal Information:: Journal Volume: 21; Journal Issue: 12; Journal ID: ISSN 1438-1656

Publisher:: Wiley

Country of Publication:: United States

Language:: English

Subject:: 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; Natural Graphite; Internal Interfaces; Magnetoresistance; High Magnetic Field

Citation Formats


                    Precker, Christian E., Barzola-Quiquia, José, Esquinazi, Pablo D., Stiller, Markus, Chan, Mun K., Jaime, Marcelo, Zhang, Zhipeng, and Grundmann, Marius. Record-Breaking Magnetoresistance at the Edge of a Microflake of Natural Graphite.  United States: N. p., 2019. 
Web.  https://doi.org/10.1002/adem.201900991.

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                    Precker, Christian E., Barzola-Quiquia, José, Esquinazi, Pablo D., Stiller, Markus, Chan, Mun K., Jaime, Marcelo, Zhang, Zhipeng, & Grundmann, Marius. Record-Breaking Magnetoresistance at the Edge of a Microflake of Natural Graphite.  United States.  https://doi.org/10.1002/adem.201900991

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                    Precker, Christian E., Barzola-Quiquia, José, Esquinazi, Pablo D., Stiller, Markus, Chan, Mun K., Jaime, Marcelo, Zhang, Zhipeng, and Grundmann, Marius. Mon .  
"Record-Breaking Magnetoresistance at the Edge of a Microflake of Natural Graphite".  United States.  https://doi.org/10.1002/adem.201900991.  https://www.osti.gov/servlets/purl/1660594.

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@article{osti_1660594,

  title        = {Record-Breaking Magnetoresistance at the Edge of a Microflake of Natural Graphite},

  author       = {Precker, Christian E. and Barzola-Quiquia, José and Esquinazi, Pablo D. and Stiller, Markus and Chan, Mun K. and Jaime, Marcelo and Zhang, Zhipeng and Grundmann, Marius},

  abstractNote = {Placing several electrodes at the edge of a micrometer-size Sri Lankan natural graphite sample at distances comparable to the size of the internal crystalline regions, we found record values for the change of the resistance with magnetic field. At low temperatures and at B ~ 21 T the magnetoresistance (MR) reaches ≈ 107%. The MR values exceed by far all earlier reported ones for graphite and they are comparable or even larger (at T > 50 K) than the largest reported in solids including the Weyl semimetals. The origin of this large MR lies in the existence of highly conducting 2D interfaces aligned parallel to the graphene planes.},

  doi          = {10.1002/adem.201900991},

  journal      = {Advanced Engineering Materials},

  number       = 12,

  volume       = 21,

  place        = {United States},

  year         = {2019},

  month        = {11}

}

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Similar Records

Title: Record-Breaking Magnetoresistance at the Edge of a Microflake of Natural Graphite

Abstract

Citation Formats

Extremely high magnetoresistance and conductivity in the type-II Weyl semimetals WP2 and MoP2 journal, November 2017

Thickness-dependent phase transition in graphite under high magnetic field journal, March 2018

Large magnetoresistance and superconductivity in α-gallium single crystals journal, August 2018

Graphite, Graphene, and the Flat Band Superconductivity journal, April 2018

Dissipation Effects on the Superconductor-Insulator Transition in 2D Superconductors journal, June 1999

Identification of a possible superconducting transition above room temperature in natural graphite crystals journal, November 2016

Unconventional superconductivity in magic-angle graphene superlattices journal, March 2018

Sample-Size Effects in the Magnetoresistance of Graphite journal, November 2007

Local Magnetic Measurements of Trapped Flux Through a Permanent Current Path in Graphite journal, February 2018

Ballistic transport at room temperature in micrometer-size graphite flakes journal, March 2011

High-field magnetoresistance of graphite revised journal, May 2019

Negative c-axis magnetoresistance in graphite journal, October 2010

Optimization of graphene dry etching conditions via combined microscopic and spectroscopic analysis journal, May 2013

Granular superconductivity below 5 K in SPI-II pyrolytic graphite journal, January 2015

Large networks of vertical multi-layer graphenes with morphology-tunable magnetoresistance journal, January 2013

A decade of graphene research: production, applications and outlook journal, November 2014

Positive and negative linear magnetoresistance of graphite journal, January 2004

Tunable magnetoresistance in thin-film graphite field-effect transistor by gate voltage journal, October 2018

Evidence for room temperature superconductivity at graphite interfaces: Room temperature superconductivity journal, September 2017

Influence of rhombohedral stacking order in the electrical resistance of bulk and mesoscopic graphite journal, January 2017

Absence of metal–insulator transition and coherent interlayer transport in oriented graphite in parallel magnetic fields journal, January 2003

Josephson-coupled superconducting regions embedded at the interfaces of highly oriented pyrolytic graphite journal, February 2013

Extremely large magnetoresistance and ultrahigh mobility in the topological Weyl semimetal candidate NbP journal, June 2015

Quantum phase transitions in two dimensions: Experiments in Josephson-junction arrays journal, October 1996

Influence of interfaces on the transport properties of graphite revealed by nanometer thickness reduction journal, November 2018

Giant magnetoresistance in single-layer graphene flakes with a gate-voltage-tunable weak antilocalization journal, November 2013

Extremely large magnetoresistance in few-layer graphene/boron–nitride heterostructures journal, September 2015

Field-induced metal-insulator transition in the c -axis resistivity of graphite journal, May 2002

Room Temperature Giant and Linear Magnetoresistance in Topological Insulator Bi 2 Te 3 Nanosheets journal, June 2012

Two Phase Transitions Induced by a Magnetic Field in Graphite journal, June 2013

Reentrant Metallic Behavior of Graphite in the Quantum Limit journal, April 2003

Electric carrier concentration in graphite: Dependence of electrical resistivity and magnetoresistance on defect concentration journal, November 2009

Dimensional reduction, quantum Hall effect and layer parity in graphite films journal, February 2019

Taming the magnetoresistance anomaly in graphite journal, November 2018

Evidence for semiconducting behavior with a narrow band gap of Bernal graphite journal, May 2012

Millikelvin de Haas–van Alphen and magnetotransport studies of graphite journal, January 2011

Semiconductor-superconductor transition in granular Al-Ge journal, April 1983

Tight-binding description of intrinsic superconducting correlations in multilayer graphene journal, April 2013

Fabrication of graphite nanopillars and nanocones by reactive ion etching journal, August 2006

Sample size effects on the transport characteristics of mesoscopic graphite samples journal, December 2008

Extremely high magnetoresistance and conductivity in the type-II Weyl semimetals WP2 and MoP2
journal, November 2017

Thickness-dependent phase transition in graphite under high magnetic field
journal, March 2018

Large magnetoresistance and superconductivity in α-gallium single crystals
journal, August 2018

Graphite, Graphene, and the Flat Band Superconductivity
journal, April 2018

Dissipation Effects on the Superconductor-Insulator Transition in 2D Superconductors
journal, June 1999

Identification of a possible superconducting transition above room temperature in natural graphite crystals
journal, November 2016

Unconventional superconductivity in magic-angle graphene superlattices
journal, March 2018

Sample-Size Effects in the Magnetoresistance of Graphite
journal, November 2007

Local Magnetic Measurements of Trapped Flux Through a Permanent Current Path in Graphite
journal, February 2018

Ballistic transport at room temperature in micrometer-size graphite flakes
journal, March 2011

High-field magnetoresistance of graphite revised
journal, May 2019

Negative c-axis magnetoresistance in graphite
journal, October 2010

Optimization of graphene dry etching conditions via combined microscopic and spectroscopic analysis
journal, May 2013

Granular superconductivity below 5 K in SPI-II pyrolytic graphite
journal, January 2015

Large networks of vertical multi-layer graphenes with morphology-tunable magnetoresistance
journal, January 2013

A decade of graphene research: production, applications and outlook
journal, November 2014

Positive and negative linear magnetoresistance of graphite
journal, January 2004

Tunable magnetoresistance in thin-film graphite field-effect transistor by gate voltage
journal, October 2018

Evidence for room temperature superconductivity at graphite interfaces: Room temperature superconductivity
journal, September 2017

Influence of rhombohedral stacking order in the electrical resistance of bulk and mesoscopic graphite
journal, January 2017

Absence of metal–insulator transition and coherent interlayer transport in oriented graphite in parallel magnetic fields
journal, January 2003

Josephson-coupled superconducting regions embedded at the interfaces of highly oriented pyrolytic graphite
journal, February 2013

Extremely large magnetoresistance and ultrahigh mobility in the topological Weyl semimetal candidate NbP
journal, June 2015

Quantum phase transitions in two dimensions: Experiments in Josephson-junction arrays
journal, October 1996

Influence of interfaces on the transport properties of graphite revealed by nanometer thickness reduction
journal, November 2018

Giant magnetoresistance in single-layer graphene flakes with a gate-voltage-tunable weak antilocalization
journal, November 2013

Extremely large magnetoresistance in few-layer graphene/boron–nitride heterostructures
journal, September 2015

Field-induced metal-insulator transition in the c -axis resistivity of graphite
journal, May 2002

Room Temperature Giant and Linear Magnetoresistance in Topological Insulator ${Bi}_{2} {Te}_{3}$ Nanosheets
journal, June 2012

Two Phase Transitions Induced by a Magnetic Field in Graphite
journal, June 2013

Reentrant Metallic Behavior of Graphite in the Quantum Limit
journal, April 2003

Electric carrier concentration in graphite: Dependence of electrical resistivity and magnetoresistance on defect concentration
journal, November 2009

Dimensional reduction, quantum Hall effect and layer parity in graphite films
journal, February 2019

Taming the magnetoresistance anomaly in graphite
journal, November 2018

Evidence for semiconducting behavior with a narrow band gap of Bernal graphite
journal, May 2012

Millikelvin de Haas–van Alphen and magnetotransport studies of graphite
journal, January 2011

Semiconductor-superconductor transition in granular Al-Ge
journal, April 1983

Tight-binding description of intrinsic superconducting correlations in multilayer graphene
journal, April 2013

Fabrication of graphite nanopillars and nanocones by reactive ion etching
journal, August 2006

Sample size effects on the transport characteristics of mesoscopic graphite samples
journal, December 2008