Direct determination of mode-projected electron-phonon coupling in the time domain

Na, M. X.; Mills, A. K.; Boschini, F.; Michiardi, M.; Nosarzewski, B.; Day, R. P.; Razzoli, E.; Sheyerman, A.; Schneider, M.; Levy, G.; Zhdanovich, S.; Devereaux, T. P.; Kemper, A. F.; Jones, D. J.; Damascelli, A.

doi:10.1126/science.aaw1662

Title: Direct determination of mode-projected electron-phonon coupling in the time domain

Journal Article · 05 December 2019 · Science

DOI: https://doi.org/10.1126/science.aaw1662 · OSTI ID:1660443

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Univ. of British Columbia, Vancouver, BC (Canada); Quantum Matter Inst., Vancouver, BC (Canada)
Univ. of British Columbia, Vancouver, BC (Canada); Quantum Matter Inst., Vancouver, BC (Canada); Max Planck Inst. for Chemical Physics of Solids, Dresden (Germany)
Stanford Univ., CA (United States)
North Carolina State Univ., Raleigh, NC (United States)

Ultrafast spectroscopies have become an important tool for elucidating the microscopic description and dynamical properties of quantum materials. In particular, by tracking the dynamics of nonthermal electrons, a material’s dominant scattering processes can be revealed. In this paper, we present a method for extracting the electron-phonon coupling strength in the time domain, using time- and angle-resolved photoemission spectroscopy (TR-ARPES). This method is demonstrated in graphite, where we investigate the dynamics of photoinjected electrons at the $$\overline{K}$$ point, detecting quantized energy-loss processes that correspond to the emission of strongly coupled optical phonons. We show that the observed characteristic time scale for spectral weight transfer mediated by phonon-scattering processes allows for the direct quantitative extraction of electron-phonon matrix elements for specific modes.

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Research Organization:: SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)

Sponsoring Organization:: Gordon and Betty Moore Foundation; National Science Foundation (NSF); Swiss National Science Foundation (SNSF); USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division

Grant/Contract Number:: AC02-76SF00515

OSTI ID:: 1660443

Journal Information:: Science, Journal Name: Science Journal Issue: 6470 Vol. 366; ISSN 0036-8075

Publisher:: AAASCopyright Statement

Country of Publication:: United States

Language:: English

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