Elucidating the G″ overshoot in soft materials with a yield transition via a time-resolved experimental strain decomposition

Donley, Gavin J.; Singh, Piyush K.; Shetty, Abhishek; Rogers, Simon A.

doi:10.1073/pnas.2003869117

Title: Elucidating the G″ overshoot in soft materials with a yield transition via a time-resolved experimental strain decomposition

Journal Article · 23 August 2020 · Proceedings of the National Academy of Sciences of the United States of America

DOI: https://doi.org/10.1073/pnas.2003869117 · OSTI ID:1650387

Donley, Gavin J. ^[1]; Singh, Piyush K. ^[1]; Shetty, Abhishek ^[2];

^[1]

Department of Chemical and Biomolecular Engineering, University of Illinois at Urbana–Champaign, Urbana, IL 61801-3602,
Rheology Division, Anton Paar USA, Ashland, VA 23005

Significance The yielding transition in soft materials manifests macroscopically as a reversible transition from solid-like deformation to liquid-like flow under sufficiently large loading or deformation. Despite the ubiquity of materials that exhibit yielding, an understanding of the transition has remained elusive due to experimental limitations of the simple rheological tests typically used to study it. We present here a more thorough understanding of yielding, obtained via an iterative test protocol and analysis that allow for the separation of solid-like and liquid-like behaviors in the response of these materials. We show that yielding is a gradual transition, occurring to an increased extent as the deformation increases.

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Sponsoring Organization:: USDOE

OSTI ID:: 1650387

Journal Information:: Proceedings of the National Academy of Sciences of the United States of America, Journal Name: Proceedings of the National Academy of Sciences of the United States of America Journal Issue: 36 Vol. 117; ISSN 0027-8424

Publisher:: Proceedings of the National Academy of SciencesCopyright Statement

Country of Publication:: United States

Language:: English

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