High-resolution neutron spectroscopy using backscattering and neutron spin-echo spectrometers in soft and hard condensed matter

Gardner, Jason S.; Ehlers, Georg; Faraone, Antonio; Garcia-Sakai, Victoria

doi:10.1038/s42254-019-0128-1

Title: High-resolution neutron spectroscopy using backscattering and neutron spin-echo spectrometers in soft and hard condensed matter

Journal Article · 01 January 2020 · Nature Reviews Physics

DOI: https://doi.org/10.1038/s42254-019-0128-1 · OSTI ID:1649600

Gardner, Jason S. ^[1];

^[2]; Faraone, Antonio ^[3]; Garcia-Sakai, Victoria ^[4]

Songshan Lake Materials Lab., Dongguan (China)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
National Inst. of Standards and Technology (NIST), Gaithersburg, MD (United States)
Rutherford Appleton Lab., Didcot (United Kingdom)

The instruments best suited to performing high-energy-resolution neutron spectroscopy are spin-echo spectrometers and backscattering spectrometers. The development of these experimental techniques dates back almost half a century, and most major neutron scattering facilities operate mature spectrometers of one or both classes. Recent advances in instrumentation and neutron sources are enhancing their performance and expanding their capabilities, with the objective of enabling researchers to tackle new and more complex problems. Finally, in this Technical Review, we assess the current state of the art in high-energy-resolution neutron spectrometers, showcasing their role in the study of nanoscale dynamics in soft and biological materials, as well as disordered magnets.

View Accepted Manuscript (DOE)

Cite

Export

Save

Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: National Science Foundation (NSF); USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 1649600

Journal Information:: Nature Reviews Physics, Journal Name: Nature Reviews Physics Journal Issue: 1 Vol. 2; ISSN 2522-5820

Publisher:: Springer NatureCopyright Statement

Country of Publication:: United States

Language:: English

References (148)

Observation of Protein Domain Motions by Neutron Spectroscopy Monkenbusch, Michael; Richter, Dieter; Biehl, Ralf ChemPhysChem, Vol. 11, Issue 6 https://doi.org/10.1002/cphc.200900514	journal	April 2010
Neutron Spin Echo Spectroscopy Mezei, Ferenc; Pappas, Catherine; Gutberlet, Thomas Lecture Notes in Physics https://doi.org/10.1007/3-540-45823-9	book	December 2002
Hyperfine interaction in amorphous ferromagnetic cobalt-phosphorous-alloys measured by inelastic scattering of neutrons Heidemann, A. Zeitschrift f�r Physik B Condensed Matter and Quanta, Vol. 20, Issue 4 https://doi.org/10.1007/BF01313208	journal	December 1975
Neutron Spin Echo in Polymer Systems Richter, Dieter; Monkenbusch, Michael; Arbe, Arantxa https://doi.org/10.1007/b106578	book	January 2005
Neutrons for the study of dynamics in soft matter systems Hoffmann, Ingo Colloid and Polymer Science, Vol. 292, Issue 9 https://doi.org/10.1007/s00396-014-3330-9	journal	August 2014
Wide angle NSE:the spectrometer SPAN at BENSC Pappas, C.; Kischnik, R.; Mezei, F. Physica B: Condensed Matter, Vol. 297, Issue 1-4 https://doi.org/10.1016/S0921-4526(00)00845-0	journal	March 2001
IN11C, medium-resolution multidetector extension of the IN11 NSE spectrometer at the ILL Farago, B. Physica B: Condensed Matter, Vol. 241-243 https://doi.org/10.1016/S0921-4526(97)00526-7	journal	December 1997
Inelastic and quasi-elastic neutron scattering spectrometers in J-PARC Seto, H.; Itoh, S.; Yokoo, T. Biochimica et Biophysica Acta (BBA) - General Subjects, Vol. 1861, Issue 1 https://doi.org/10.1016/j.bbagen.2016.04.025	journal	January 2017
Bilayer undulation dynamics in unilamellar phospholipid vesicles: Effect of temperature, cholesterol and trehalose Brüning, Beate-Annette; Prévost, Sylvain; Stehle, Ralf Biochimica et Biophysica Acta (BBA) - Biomembranes, Vol. 1838, Issue 10 https://doi.org/10.1016/j.bbamem.2014.06.006	journal	October 2014
The helix-to-sheet transition of an HIV-1 fusion peptide derivative changes the mechanical properties of lipid bilayer membranes Heller, William T.; Zolnierczuk, Piotr A. Biochimica et Biophysica Acta (BBA) - Biomembranes, Vol. 1861, Issue 3 https://doi.org/10.1016/j.bbamem.2018.12.004	journal	March 2019
Effect of charged lidocaine on static and dynamic properties of model bio-membranes Yi, Zheng; Nagao, Michihiro; Bossev, Dobrin P. Biophysical Chemistry, Vol. 160, Issue 1 https://doi.org/10.1016/j.bpc.2011.08.007	journal	January 2012
Interpreting Membrane Scattering Experiments at the Mesoscale: The Contribution of Dissipation within the Bilayer Watson, Max C.; Brown, Frank L. H. Biophysical Journal, Vol. 98, Issue 6 https://doi.org/10.1016/j.bpj.2009.11.026	journal	March 2010
Structure and Dynamics of a Compact State of a Multidomain Protein, the Mercuric Ion Reductase Hong, Liang; Sharp, Melissa A.; Poblete, Simón Biophysical Journal, Vol. 107, Issue 2 https://doi.org/10.1016/j.bpj.2014.06.013	journal	July 2014
Tuning Membrane Thickness Fluctuations in Model Lipid Bilayers Ashkar, Rana; Nagao, Michihiro; Butler, Paul D. Biophysical Journal, Vol. 109, Issue 1 https://doi.org/10.1016/j.bpj.2015.05.033	journal	July 2015
Dynamic processes in biological membrane mimics revealed by quasielastic neutron scattering Lautner, Lisa; Pluhackova, Kristyna; Barth, Nicolai K. H. Chemistry and Physics of Lipids, Vol. 206 https://doi.org/10.1016/j.chemphyslip.2017.05.009	journal	August 2017
Quasielastic neutron scattering in soft matter Sakai, Victoria García; Arbe, Arantxa Current Opinion in Colloid & Interface Science, Vol. 14, Issue 6 https://doi.org/10.1016/j.cocis.2009.04.002	journal	December 2009
The spin-echo spectrometer at the Spallation Neutron Source (SNS) Ohl, M.; Monkenbusch, M.; Arend, N. Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 696 https://doi.org/10.1016/j.nima.2012.08.059	journal	December 2012
Nuclear spin excitations in NdCu2 Chatterji, Tapan; Frick, Bernhard Physica B: Condensed Matter, Vol. 350, Issue 1-3 https://doi.org/10.1016/j.physb.2004.03.030	journal	July 2004
Relocation and upgrade of neutron spin echo spectrometer, iNSE Nagao, Michihiro; Yamada, Norifumi L.; Kawabata, Youhei Physica B: Condensed Matter, Vol. 385-386 https://doi.org/10.1016/j.physb.2006.05.383	journal	November 2006
Recent developments in fusion and direct reactions with weakly bound nuclei Canto, L. F.; Gomes, P. R. S.; Donangelo, R. Physics Reports, Vol. 596 https://doi.org/10.1016/j.physrep.2015.08.001	journal	September 2015
Visualizing the nanoscale: protein internal dynamics and neutron spin echo spectroscopy Callaway, David JE; Bu, Zimei Current Opinion in Structural Biology, Vol. 42 https://doi.org/10.1016/j.sbi.2016.10.001	journal	February 2017
Effect of Hierarchical Cluster Formation on the Viscosity of Concentrated Monoclonal Antibody Formulations Studied by Neutron Scattering Godfrin, P. Douglas; Zarraga, Isidro E.; Zarzar, Jonathan The Journal of Physical Chemistry B, Vol. 120, Issue 2 https://doi.org/10.1021/acs.jpcb.5b07260	journal	January 2016
Ligation-Dependent Picosecond Dynamics in Human Hemoglobin As Revealed by Quasielastic Neutron Scattering Fujiwara, Satoru; Chatake, Toshiyuki; Matsuo, Tatsuhito The Journal of Physical Chemistry B, Vol. 121, Issue 34 https://doi.org/10.1021/acs.jpcb.7b05182	journal	August 2017
Lipid Rafts: Buffers of Cell Membrane Physical Properties Nickels, Jonathan D.; Smith, Micholas Dean; Alsop, Richard J. The Journal of Physical Chemistry B, Vol. 123, Issue 9 https://doi.org/10.1021/acs.jpcb.8b12126	journal	January 2019
Chemotherapeutic Targets in Osteosarcoma: Insights from Synchrotron-MicroFTIR and Quasi-Elastic Neutron Scattering Marques, Maria Paula M.; Batista de Carvalho, Ana L. M.; Mamede, Adriana P. The Journal of Physical Chemistry B, Vol. 123, Issue 32 https://doi.org/10.1021/acs.jpcb.9b05596	journal	July 2019
Lithium Conductivity and Ions Dynamics in LiBH ₄ /SiO ₂ Solid Electrolytes Studied by Solid-State NMR and Quasi-Elastic Neutron Scattering and Applied in Lithium–Sulfur Batteries Lefevr, Jessica; Cervini, Luca; Griffin, John M. The Journal of Physical Chemistry C, Vol. 122, Issue 27 https://doi.org/10.1021/acs.jpcc.8b01507	journal	June 2018
In Vivo Protein Dynamics on the Nanometer Length Scale and Nanosecond Time Scale Anunciado, Divina B.; Nyugen, Vyncent P.; Hurst, Gregory B. The Journal of Physical Chemistry Letters, Vol. 8, Issue 8 https://doi.org/10.1021/acs.jpclett.7b00399	journal	April 2017
Crowding-Controlled Cluster Size in Concentrated Aqueous Protein Solutions: Structure, Self- and Collective Diffusion Braun, Michal K.; Grimaldo, Marco; Roosen-Runge, Felix The Journal of Physical Chemistry Letters, Vol. 8, Issue 12 https://doi.org/10.1021/acs.jpclett.7b00658	journal	May 2017
Probing Elastic and Viscous Properties of Phospholipid Bilayers Using Neutron Spin Echo Spectroscopy Nagao, Michihiro; Kelley, Elizabeth G.; Ashkar, Rana The Journal of Physical Chemistry Letters, Vol. 8, Issue 19 https://doi.org/10.1021/acs.jpclett.7b01830	journal	September 2017
Bacillus subtilis Lipid Extract, A Branched-Chain Fatty Acid Model Membrane Nickels, Jonathan D.; Chatterjee, Sneha; Mostofian, Barmak The Journal of Physical Chemistry Letters, Vol. 8, Issue 17 https://doi.org/10.1021/acs.jpclett.7b01877	journal	August 2017
Low-Temperature Decoupling of Water and Protein Dynamics Measured by Neutron Scattering Benedetto, Antonio The Journal of Physical Chemistry Letters, Vol. 8, Issue 19 https://doi.org/10.1021/acs.jpclett.7b02273	journal	September 2017
Relevance of Internal Friction and Structural Constraints for the Dynamics of Denatured Bovine Serum Albumin Ameseder, Felix; Radulescu, Aurel; Holderer, Olaf The Journal of Physical Chemistry Letters, Vol. 9, Issue 10 https://doi.org/10.1021/acs.jpclett.8b00825	journal	April 2018
Phospholipid Bilayer Softening Due to Hydrophobic Gold Nanoparticle Inclusions Chakraborty, Saptarshi; Abbasi, Akram; Bothun, Geoffrey D. Langmuir, Vol. 34, Issue 44 https://doi.org/10.1021/acs.langmuir.8b02553	journal	September 2018
Single Chain Dynamic Structure Factor of Linear Polymers in an All-Polymer Nano-Composite Arbe, Arantxa; Pomposo, José A.; Asenjo-Sanz, Isabel Macromolecules, Vol. 49, Issue 6 https://doi.org/10.1021/acs.macromol.5b02519	journal	March 2016
Relationship between Segmental Dynamics Measured by Quasi-Elastic Neutron Scattering and Conductivity in Polymer Electrolytes Mongcopa, Katrina Irene S.; Tyagi, Madhusudan; Mailoa, Jonathan P. ACS Macro Letters, Vol. 7, Issue 4 https://doi.org/10.1021/acsmacrolett.8b00159	journal	March 2018
Dynamics of Architecturally Engineered All-Polymer Nanocomposites Senses, Erkan; Tyagi, Madhusudan; Pasco, Madeleine ACS Nano, Vol. 12, Issue 11 https://doi.org/10.1021/acsnano.8b02514	journal	October 2018
Using Neutron Spin−Echo To Investigate Proton Dynamics in Proton-Conducting Perovskites ^† Karlsson, Maths; Engberg, Dennis; Björketun, Mårten E. Chemistry of Materials, Vol. 22, Issue 3 https://doi.org/10.1021/cm901624v	journal	February 2010
Internal Nanosecond Dynamics in the Intrinsically Disordered Myelin Basic Protein Stadler, Andreas M.; Stingaciu, Laura; Radulescu, Aurel Journal of the American Chemical Society, Vol. 136, Issue 19 https://doi.org/10.1021/ja502343b	journal	May 2014
Mechanical Properties of Nanoscopic Lipid Domains Nickels, Jonathan D.; Cheng, Xiaolin; Mostofian, Barmak Journal of the American Chemical Society, Vol. 137, Issue 50 https://doi.org/10.1021/jacs.5b08894	journal	October 2015
Formation of the Dynamic Clusters in Concentrated Lysozyme Protein Solutions Porcar, Lionel; Falus, Peter; Chen, Wei-Ren The Journal of Physical Chemistry Letters, Vol. 1, Issue 1 https://doi.org/10.1021/jz900127c	journal	November 2009
Dynamics of Entangled Chains in Polymer Nanocomposites Schneider, G. J.; Nusser, K.; Willner, L. Macromolecules, Vol. 44, Issue 15 https://doi.org/10.1021/ma200899y	journal	August 2011
Chain Dynamics and Viscoelastic Properties of Poly(ethylene oxide) Niedzwiedz, K.; Wischnewski, A.; Pyckhout-Hintzen, W. Macromolecules, Vol. 41, Issue 13 https://doi.org/10.1021/ma800446n	journal	July 2008
Dynamical transition of myoglobin revealed by inelastic neutron scattering Doster, Wolfgang; Cusack, Stephen; Petry, Winfried Nature, Vol. 337, Issue 6209 https://doi.org/10.1038/337754a0	journal	February 1989
Jamming phase diagram for attractive particles Trappe, V.; Prasad, V.; Cipelletti, Luca Nature, Vol. 411, Issue 6839 https://doi.org/10.1038/35081021	journal	June 2001
Emergent excitations in a geometrically frustrated magnet Lee, S. -H.; Broholm, C.; Ratcliff, W. Nature, Vol. 418, Issue 6900 https://doi.org/10.1038/nature00964	journal	August 2002
Measurement of the charge and current of magnetic monopoles in spin ice Bramwell, S. T.; Giblin, S. R.; Calder, S. Nature, Vol. 461, Issue 7266 https://doi.org/10.1038/nature08500	journal	October 2009
Spin liquids in frustrated magnets Balents, Leon Nature, Vol. 464, Issue 7286 https://doi.org/10.1038/nature08917	journal	March 2010
Absence of Pauling’s residual entropy in thermally equilibrated Dy2Ti2O7 Pomaranski, D.; Yaraskavitch, L. R.; Meng, S. Nature Physics, Vol. 9, Issue 6 https://doi.org/10.1038/nphys2591	journal	April 2013
Far-from-equilibrium monopole dynamics in spin ice Paulsen, C.; Jackson, M. J.; Lhotel, E. Nature Physics, Vol. 10, Issue 2 https://doi.org/10.1038/nphys2847	journal	January 2014
Observation of magnetic fragmentation in spin ice Petit, S.; Lhotel, E.; Canals, B. Nature Physics, Vol. 12, Issue 8 https://doi.org/10.1038/nphys3710	journal	April 2016
Continuous excitations of the triangular-lattice quantum spin liquid YbMgGaO4 Paddison, Joseph A. M.; Daum, Marcus; Dun, Zhiling Nature Physics, Vol. 13, Issue 2 https://doi.org/10.1038/nphys3971	journal	December 2016
Hemoglobin diffusion and the dynamics of oxygen capture by red blood cells Longeville, Stéphane; Stingaciu, Laura-Roxana Scientific Reports, Vol. 7, Issue 1 https://doi.org/10.1038/s41598-017-09146-9	journal	September 2017
Scaling of Memories and Crossover in Glassy Magnets Samarakoon, A. M.; Takahashi, M.; Zhang, D. Scientific Reports, Vol. 7, Issue 1 https://doi.org/10.1038/s41598-017-12187-9	journal	September 2017
The effects of pressure on the energy landscape of proteins Librizzi, Fabio; Carrotta, Rita; Peters, Judith Scientific Reports, Vol. 8, Issue 1 https://doi.org/10.1038/s41598-018-20417-x	journal	February 2018
Microscopic diffusion processes measured in living planarians Mamontov, Eugene Scientific Reports, Vol. 8, Issue 1 https://doi.org/10.1038/s41598-018-22643-9	journal	March 2018
A flexible high speed pulse chopper system for an inverted neutron time-of-flight option on backscattering spectrometers Appel, Markus; Frick, Bernhard; Magerl, Andreas Scientific Reports, Vol. 8, Issue 1 https://doi.org/10.1038/s41598-018-31774-y	journal	September 2018
Adaptation to extreme environments: macromolecular dynamics in bacteria compared in vivo by neutron scattering Tehei, Moeava; Franzetti, Bruno; Madern, Dominique EMBO reports, Vol. 5, Issue 1 https://doi.org/10.1038/sj.embor.7400049	journal	January 2004
Microscopic Chain Motion in Polymer Nanocomposites with Dynamically Asymmetric Interphases Senses, Erkan; Faraone, Antonio; Akcora, Pinar Scientific Reports, Vol. 6, Issue 1 https://doi.org/10.1038/srep29326	journal	July 2016
Spectroscopic characteristics of the OSIRIS near-backscattering crystal analyser spectrometer on the ISIS pulsed neutron source Telling, Mark. T. F.; Andersen, Ken. H. Phys. Chem. Chem. Phys., Vol. 7, Issue 6 https://doi.org/10.1039/B413934H	journal	January 2005
Exploring internal protein dynamics by neutron spin echo spectroscopy Biehl, Ralf; Monkenbusch, Michael; Richter, Dieter Soft Matter, Vol. 7, Issue 4 https://doi.org/10.1039/C0SM00683A	journal	January 2011
Perspectives of neutron scattering on proton conducting oxides Karlsson, Maths Dalton Trans., Vol. 42, Issue 2 https://doi.org/10.1039/C2DT31891A	journal	January 2013
Softening of phospholipid membranes by the adhesion of silica nanoparticles – as seen by neutron spin-echo (NSE) Hoffmann, Ingo; Michel, Raphael; Sharp, Melissa Nanoscale, Vol. 6, Issue 12 https://doi.org/10.1039/C4NR00774C	journal	January 2014
Structural and mechanical properties of cardiolipin lipid bilayers determined using neutron spin echo, small angle neutron and X-ray scattering, and molecular dynamics simulations Pan, Jianjun; Cheng, Xiaolin; Sharp, Melissa Soft Matter, Vol. 11, Issue 1 https://doi.org/10.1039/C4SM02227K	journal	January 2015
Effect of antimicrobial peptide on the dynamics of phosphocholine membrane: role of cholesterol and physical state of bilayer Sharma, V. K.; Mamontov, E.; Anunciado, D. B. Soft Matter, Vol. 11, Issue 34 https://doi.org/10.1039/C5SM01562F	journal	January 2015
Intracellular water – an overlooked drug target? Cisplatin impact in cancer cells probed by neutrons Marques, M. P. M.; Batista de Carvalho, A. L. M.; Sakai, V. Garcia Physical Chemistry Chemical Physics, Vol. 19, Issue 4 https://doi.org/10.1039/C6CP05198G	journal	January 2017
DMPC vesicle structure and dynamics in the presence of low amounts of the saponin aescin Sreij, Ramsia; Dargel, Carina; Geisler, Philippe Physical Chemistry Chemical Physics, Vol. 20, Issue 14 https://doi.org/10.1039/C7CP08027A	journal	January 2018
Relaxation dynamics of saturated and unsaturated oriented lipid bilayers Nanda, Hirsh; García Sakai, Victoria; Khodadadi, Sheila Soft Matter, Vol. 14, Issue 29 https://doi.org/10.1039/C7SM01720K	journal	January 2018
Temperature-dependent structure and dynamics of highly-branched poly( N -isopropylacrylamide) in aqueous solution AL-Baradi, Ateyyah M.; Rimmer, Stephen; Carter, Steven R. Soft Matter, Vol. 14, Issue 8 https://doi.org/10.1039/C7SM02330H	journal	January 2018
A quasielastic and inelastic neutron scattering study of the alkaline and alkaline-earth borohydrides LiBH ₄ and Mg(BH ₄ ) ₂ and the mixture LiBH ₄ + Mg(BH ₄ ) ₂ Silvi, Luca; Zhao-Karger, Zhirong; Röhm, Eva Physical Chemistry Chemical Physics, Vol. 21, Issue 2 https://doi.org/10.1039/C8CP04316G	journal	January 2019
Dynamic properties of different liquid states in systems with competing interactions studied with lysozyme solutions Godfrin, P. D.; Falus, P.; Porcar, L. Soft Matter, Vol. 14, Issue 42 https://doi.org/10.1039/C8SM01678J	journal	January 2018
Partitioning of ethanol into lipid membranes and its effect on fluidity and permeability as seen by X-ray and neutron scattering Toppozini, Laura; Armstrong, Clare L.; Barrett, Matthew A. Soft Matter, Vol. 8, Issue 47 https://doi.org/10.1039/c2sm26546j	journal	January 2012
From BASIS to MIRACLES: Benchmarking and perspectives for high-resolution neutron spectroscopy at the ESS Tsapatsaris, Nikolaos; Willendrup, Peter K.; Lechner, Ruep E. EPJ Web of Conferences, Vol. 83 https://doi.org/10.1051/epjconf/20158303015	journal	January 2015
Neutron Spin Echo Spectroscopy Mezei, F. Europhysics News, Vol. 16, Issue 4 https://doi.org/10.1051/epn/19851604001	journal	January 1985
Neutron Spin Echo Spectroscopy: Applications in Magnetism Mezei, F. Europhysics News, Vol. 17, Issue 11-12 https://doi.org/10.1051/epn/19861711129	journal	January 1986
The high-flux backscattering spectrometer at the NIST Center for Neutron Research Meyer, A.; Dimeo, R. M.; Gehring, P. M. Review of Scientific Instruments, Vol. 74, Issue 5 https://doi.org/10.1063/1.1568557	journal	May 2003
Reptation of a Polymer Chain in the Presence of Fixed Obstacles de Gennes, P. G. The Journal of Chemical Physics, Vol. 55, Issue 2 https://doi.org/10.1063/1.1675789	journal	July 1971
A time-of-flight backscattering spectrometer at the Spallation Neutron Source, BASIS Mamontov, E.; Herwig, K. W. Review of Scientific Instruments, Vol. 82, Issue 8 https://doi.org/10.1063/1.3626214	journal	August 2011
SPHERES, Jülich's high-flux neutron backscattering spectrometer at FRM II Wuttke, Joachim; Budwig, Alfred; Drochner, Matthias Review of Scientific Instruments, Vol. 83, Issue 7 https://doi.org/10.1063/1.4732806	journal	July 2012
New physics in frustrated magnets: Spin ices, monopoles, etc. (Review Article) Zvyagin, A. A. Low Temperature Physics, Vol. 39, Issue 11 https://doi.org/10.1063/1.4826079	journal	November 2013
Rheology of clustering protein solutions Dharmaraj, Vishnu L.; Godfrin, P. Douglas; Liu, Yun Biomicrofluidics, Vol. 10, Issue 4 https://doi.org/10.1063/1.4955162	journal	July 2016
Polymer dynamics under cylindrical confinement featuring a locally repulsive surface: A quasielastic neutron scattering study Krutyeva, M.; Pasini, S.; Monkenbusch, M. The Journal of Chemical Physics, Vol. 146, Issue 20 https://doi.org/10.1063/1.4974836	journal	May 2017
Short-time dynamics of lysozyme solutions with competing short-range attraction and long-range repulsion: Experiment and theory Riest, Jonas; Nägele, Gerhard; Liu, Yun The Journal of Chemical Physics, Vol. 148, Issue 6 https://doi.org/10.1063/1.5016517	journal	February 2018
Neutron scattering studies on short- and long-range layer structures and related dynamics in imidazolium-based ionic liquids Nemoto, Fumiya; Kofu, Maiko; Nagao, Michihiro The Journal of Chemical Physics, Vol. 149, Issue 5 https://doi.org/10.1063/1.5037217	journal	August 2018
Aging, memory, and nonhierarchical energy landscape of spin jam Samarakoon, Anjana; Sato, Taku J.; Chen, Tianran Proceedings of the National Academy of Sciences, Vol. 113, Issue 42 https://doi.org/10.1073/pnas.1608057113	journal	October 2016
Entropic contribution to enhanced thermal stability in the thermostable P450 CYP119 Liu, Zhuo; Lemmonds, Sara; Huang, Juan Proceedings of the National Academy of Sciences, Vol. 115, Issue 43 https://doi.org/10.1073/pnas.1807473115	journal	October 2018
The wide-angle neutron spin echo spectrometer project WASP Fouquet, Peter; Ehlers, Georg; Farago, Bela Journal of Neutron Research, Vol. 15, Issue 1 https://doi.org/10.1080/10238160601048791	journal	January 2007
IN13 Backscattering Spectrometer at ILL: Looking for Motions in Biological Macromolecules and Organisms Francesca, Natali; Peters, J.; Russo, D. Neutron News, Vol. 19, Issue 4 https://doi.org/10.1080/10448630802474083	journal	November 2008
The IN15 upgrade Farago, B.; Falus, P.; Hoffmann, I. Neutron News, Vol. 26, Issue 3 https://doi.org/10.1080/10448632.2015.1057052	journal	July 2015
Neutron scattering lengths and cross sections Sears, Varley F. Neutron News, Vol. 3, Issue 3 https://doi.org/10.1080/10448639208218770	journal	January 1992
A study of supertransferred hyperfine magnetic fields and relaxation of Dy ³⁺ ions by Mossbauer spectroscopy of ⁵⁷ Fe and ¹¹⁹ Sn ^m in the pyrochlores Dy ₂ Sn ₂ O ₇ and Dy ₂ FeSbO ₇ Snee, T. J.; Meads, R. E.; Parker, W. G. Journal of Physics C: Solid State Physics, Vol. 10, Issue 10 https://doi.org/10.1088/0022-3719/10/10/018	journal	May 1977
Spin glasses: redux: an updated experimental/materials survey Mydosh, J. A. Reports on Progress in Physics, Vol. 78, Issue 5 https://doi.org/10.1088/0034-4885/78/5/052501	journal	April 2015
Unusual ordered phases of highly frustrated magnets: a review Starykh, Oleg A. Reports on Progress in Physics, Vol. 78, Issue 5 https://doi.org/10.1088/0034-4885/78/5/052502	journal	April 2015
Dynamical crossover in hot spin ice Ehlers, G.; Cornelius, A. L.; Orend c., M. Journal of Physics: Condensed Matter, Vol. 15, Issue 2 https://doi.org/10.1088/0953-8984/15/2/102	journal	December 2002
Study of slow dynamic processes in magnetic systems by neutron spin-echo spectroscopy Ehlers, G. Journal of Physics: Condensed Matter, Vol. 18, Issue 13 https://doi.org/10.1088/0953-8984/18/13/R01	journal	March 2006
Frustrated spin correlations in diluted spin ice Ho _{2− x} La _x Ti ₂ O ₇ Ehlers, G.; Mamontov, E.; Zamponi, M. Journal of Physics: Condensed Matter, Vol. 20, Issue 23 https://doi.org/10.1088/0953-8984/20/23/235206	journal	April 2008
Magnetic monopole dynamics in spin ice Jaubert, L. D. C.; Holdsworth, P. C. W. Journal of Physics: Condensed Matter, Vol. 23, Issue 16 https://doi.org/10.1088/0953-8984/23/16/164222	journal	April 2011
Optimized superconducting coils for a high-resolution neutron spin-echo spectrometer at the European Spallation Source, ESS Pasini, S.; Monkenbusch, M. Measurement Science and Technology, Vol. 26, Issue 3 https://doi.org/10.1088/0957-0233/26/3/035501	journal	January 2015
ToF-Backscattering spectroscopy at the ISIS Facility: Status and Perspectives Demmel, F.; McPhail, D.; French, C. Journal of Physics: Conference Series, Vol. 1021 https://doi.org/10.1088/1742-6596/1021/1/012027	journal	May 2018
CASCADE with NRSE: Fast Intensity Modulation Techniques used in Quasielastic Neutron Scattering Schmidt, C. J.; Groitl, F.; Klein, M. Journal of Physics: Conference Series, Vol. 251 https://doi.org/10.1088/1742-6596/251/1/012067	journal	November 2010
The Neutron Beam Expansion Program at the Bragg Institute Klose, F.; Constantine, P.; Kennedy, S. J. Journal of Physics: Conference Series, Vol. 528 https://doi.org/10.1088/1742-6596/528/1/012026	journal	July 2014
Instrument developments and recent scientific highlights at the J-NSE Ivanova, Oxana; Pasini, Stefano; Monkenbusch, Michael Journal of Physics: Conference Series, Vol. 862 https://doi.org/10.1088/1742-6596/862/1/012009	journal	June 2017
Quasielastic Neutron Scattering and Solid State Diffusion Hempelmann, Rolf Oxford University Press https://doi.org/10.1093/acprof:oso/9780198517436.001.0001	book	November 2000
Correlations in Space and Time and Born Approximation Scattering in Systems of Interacting Particles Van Hove, Léon Physical Review, Vol. 95, Issue 1 https://doi.org/10.1103/PhysRev.95.249	journal	July 1954
Dynamics of frustrated magnetic moments in antiferromagnetically ordered TbNiAl probed by neutron time-of-flight and spin-echo spectroscopy Ehlers, G.; Casalta, H.; Lechner, R. E. Physical Review B, Vol. 63, Issue 22 https://doi.org/10.1103/PhysRevB.63.224407	journal	May 2001
Low-temperature spin freezing in the Dy 2 Ti 2 O 7 spin ice Snyder, J.; Ueland, B. G.; Slusky, J. S. Physical Review B, Vol. 69, Issue 6 https://doi.org/10.1103/PhysRevB.69.064414	journal	February 2004
Spin-spin correlations in Yb_{2}Ti_{2}O_{7} : A polarized neutron scattering study Gardner, J. S.; Ehlers, G.; Rosov, N. Physical Review B, Vol. 70, Issue 18 https://doi.org/10.1103/PhysRevB.70.180404	journal	November 2004
Spontaneous spin-lattice coupling in the geometrically frustrated triangular lattice antiferromagnet Cu Fe O 2 Ye, F.; Ren, Y.; Huang, Q. Physical Review B, Vol. 73, Issue 22 https://doi.org/10.1103/PhysRevB.73.220404	journal	June 2006
Revisiting static and dynamic spin-ice correlations in Ho 2 Ti 2 O 7 with neutron scattering Clancy, J. P.; Ruff, J. P. C.; Dunsiger, S. R. Physical Review B, Vol. 79, Issue 1 https://doi.org/10.1103/PhysRevB.79.014408	journal	January 2009
Lightly stuffed pyrochlore structure of single-crystalline Yb 2 Ti 2 O 7 grown by the optical floating zone technique Ross, K. A.; Proffen, Th.; Dabkowska, H. A. Physical Review B, Vol. 86, Issue 17 https://doi.org/10.1103/PhysRevB.86.174424	journal	November 2012
Magnetic excitations in the ground state of Yb 2 Ti 2 O 7 Peçanha-Antonio, Viviane; Feng, Erxi; Su, Yixi Physical Review B, Vol. 96, Issue 21 https://doi.org/10.1103/PhysRevB.96.214415	journal	December 2017
Direct Observation of a Nuclear Spin Excitation in Ho 2 Ti 2 O 7 Ehlers, G.; Mamontov, E.; Zamponi, M. Physical Review Letters, Vol. 102, Issue 1 https://doi.org/10.1103/PhysRevLett.102.016405	journal	January 2009
Generalized Spin-Glass Relaxation Pickup, R. M.; Cywinski, R.; Pappas, C. Physical Review Letters, Vol. 102, Issue 9 https://doi.org/10.1103/PhysRevLett.102.097202	journal	March 2009
Thermal Fluctuation and Elasticity of Lipid Vesicles Interacting with Pore-Forming Peptides Lee, Ji-Hwan; Choi, Sung-Min; Doe, Changwoo Physical Review Letters, Vol. 105, Issue 3 https://doi.org/10.1103/PhysRevLett.105.038101	journal	July 2010
Spin Ice: Magnetic Excitations without Monopole Signatures Using Muon Spin Rotation Dunsiger, S. R.; Aczel, A. A.; Arguello, C. Physical Review Letters, Vol. 107, Issue 20 https://doi.org/10.1103/PhysRevLett.107.207207	journal	November 2011
Monopoles, Magnetricity, and the Stray Field from Spin Ice Blundell, Stephen J. Physical Review Letters, Vol. 108, Issue 14 https://doi.org/10.1103/PhysRevLett.108.147601	journal	April 2012
Lipid Bilayers and Membrane Dynamics: Insight into Thickness Fluctuations Woodka, Andrea C.; Butler, Paul D.; Porcar, Lionel Physical Review Letters, Vol. 109, Issue 5 https://doi.org/10.1103/PhysRevLett.109.058102	journal	July 2012
Nanoparticle Effect on the Dynamics of Polymer Chains and Their Entanglement Network Li, Ying; Kröger, Martin; Liu, Wing Kam Physical Review Letters, Vol. 109, Issue 11 https://doi.org/10.1103/PhysRevLett.109.118001	journal	September 2012
Effect of Nanoconfinement on Polymer Dynamics: Surface Layers and Interphases Krutyeva, M.; Wischnewski, A.; Monkenbusch, M. Physical Review Letters, Vol. 110, Issue 10 https://doi.org/10.1103/PhysRevLett.110.108303	journal	March 2013
Microscopic Dynamics of Polyethylene Glycol Chains Interacting with Silica Nanoparticles Glomann, T.; Schneider, G. J.; Allgaier, J. Physical Review Letters, Vol. 110, Issue 17 https://doi.org/10.1103/PhysRevLett.110.178001	journal	April 2013
de Gennes Narrowing Describes the Relative Motion of Protein Domains Hong, Liang; Smolin, Nikolai; Smith, Jeremy C. Physical Review Letters, Vol. 112, Issue 15 https://doi.org/10.1103/PhysRevLett.112.158102	journal	April 2014
Spin Fluctuations from Hertz to Terahertz on a Triangular Lattice Nambu, Yusuke; Gardner, Jason S.; MacLaughlin, Douglas E. Physical Review Letters, Vol. 115, Issue 12 https://doi.org/10.1103/PhysRevLett.115.127202	journal	September 2015
Solitary Magnons in the S = 5 2 Antiferromagnet CaFe 2 O 4 Stock, C.; Rodriguez, E. E.; Lee, N. Physical Review Letters, Vol. 117, Issue 1 https://doi.org/10.1103/PhysRevLett.117.017201	journal	June 2016
Molecular View on Supramolecular Chain and Association Dynamics Monkenbusch, M.; Krutyeva, M.; Pyckhout-Hintzen, W. Physical Review Letters, Vol. 117, Issue 14 https://doi.org/10.1103/PhysRevLett.117.147802	journal	September 2016
Small Particle Driven Chain Disentanglements in Polymer Nanocomposites Senses, Erkan; Ansar, Siyam M.; Kitchens, Christopher L. Physical Review Letters, Vol. 118, Issue 14 https://doi.org/10.1103/PhysRevLett.118.147801	journal	April 2017
Magnetic Fluctuations, Precursor Phenomena, and Phase Transition in MnSi under a Magnetic Field Pappas, C.; Bannenberg, L. J.; Lelièvre-Berna, E. Physical Review Letters, Vol. 119, Issue 4 https://doi.org/10.1103/PhysRevLett.119.047203	journal	July 2017
Quasiparticle Breakdown and Spin Hamiltonian of the Frustrated Quantum Pyrochlore Yb 2 Ti 2 O 7 in a Magnetic Field Thompson, J. D.; McClarty, P. A.; Prabhakaran, D. Physical Review Letters, Vol. 119, Issue 5 https://doi.org/10.1103/PhysRevLett.119.057203	journal	August 2017
Undulations and Dynamic Structure Factor of Membranes Zilman, A. G.; Granek, R. Physical Review Letters, Vol. 77, Issue 23 https://doi.org/10.1103/PhysRevLett.77.4788	journal	December 1996
Glassy Statics and Dynamics in the Chemically Ordered Pyrochlore Antiferromagnet Y 2 Mo 2 O 7 Gardner, J. S.; Gaulin, B. D.; Lee, S. -H. Physical Review Letters, Vol. 83, Issue 1 https://doi.org/10.1103/PhysRevLett.83.211	journal	July 1999
Measurement of Vortex Motion in a Type-II Superconductor: A Novel Use of the Neutron Spin-Echo Technique Forgan, E. M.; Kealey, P. G.; Johnson, S. T. Physical Review Letters, Vol. 85, Issue 16 https://doi.org/10.1103/PhysRevLett.85.3488	journal	October 2000
First-Order Transition in the Spin Dynamics of Geometrically Frustrated Yb 2 Ti 2 O 7 Hodges, J. A.; Bonville, P.; Forget, A. Physical Review Letters, Vol. 88, Issue 7 https://doi.org/10.1103/PhysRevLett.88.077204	journal	February 2002
Fermi Surface Topology and the Superconducting Gap Function in UPd 2 Al 3 : A Neutron Spin-Echo Study Blackburn, E.; Hiess, A.; Bernhoeft, N. Physical Review Letters, Vol. 97, Issue 5 https://doi.org/10.1103/PhysRevLett.97.057002	journal	August 2006
Magnetic pyrochlore oxides Gardner, Jason S.; Gingras, Michel J. P.; Greedan, John E. Reviews of Modern Physics, Vol. 82, Issue 1 https://doi.org/10.1103/RevModPhys.82.53	journal	January 2010
Colloquium : Herbertsmithite and the search for the quantum spin liquid Norman, M. R. Reviews of Modern Physics, Vol. 88, Issue 4 https://doi.org/10.1103/RevModPhys.88.041002	journal	December 2016
Dramatic influence of patchy attractions on short-time protein diffusion under crowded conditions Bucciarelli, Saskia; Myung, Jin Suk; Farago, Bela Science Advances, Vol. 2, Issue 12 https://doi.org/10.1126/sciadv.1601432	journal	December 2016
Spin Ice State in Frustrated Magnetic Pyrochlore Materials Bramwell, S. T. Science, Vol. 294, Issue 5546 https://doi.org/10.1126/science.1064761	journal	November 2001
Hidden order in spin-liquid Gd3Ga5O12 Paddison, J. A. M.; Jacobsen, H.; Petrenko, O. A. Science, Vol. 350, Issue 6257 https://doi.org/10.1126/science.aaa5326	journal	October 2015
Neutron Scattering in Condensed Matter Physics Furrer, Albert; Mesot, Joël; Strässle, Thierry Series on Neutron Techniques and Applications https://doi.org/10.1142/4870	book	May 2009
Ferromagnetic Transition of Pyrochlore Compound Yb ₂ Ti ₂ O ₇ Yasui, Yukio; Soda, Minoru; Iikubo, Satoshi Journal of the Physical Society of Japan, Vol. 72, Issue 11 https://doi.org/10.1143/JPSJ.72.3014	journal	November 2003
Dynamics of an asymmetric bilayer lipid membrane in a viscous solvent Bingham, R. J.; Smye, S. W.; Olmsted, P. D. EPL (Europhysics Letters), Vol. 111, Issue 1 https://doi.org/10.1209/0295-5075/111/18004	journal	July 2015
Effect of melittin on water diffusion and membrane structure in DMPC lipid bilayers Buck, Z. N.; Torres, J.; Miskowiec, A. EPL (Europhysics Letters), Vol. 123, Issue 1 https://doi.org/10.1209/0295-5075/123/18002	journal	July 2018
Elastic Properties of Lipid Bilayers: Theory and Possible Experiments Helfrich, W. Zeitschrift für Naturforschung C, Vol. 28, Issue 11-12 https://doi.org/10.1515/znc-1973-11-1209	journal	December 1973
Recent Backscattering Instrument Developments at the ILL and SNS Frick, Bernhard; Mamontov, Eugene; Eijck, Lambert van Zeitschrift für Physikalische Chemie, Vol. 224, Issue 1-2 https://doi.org/10.1524/zpch.2010.6091	journal	February 2010
Spin Fluctuations from Hertz to Terahertz on a Triangular Lattice Nambu, Yusuke; Gardner, Jason S.; MacLaughlin, Douglas E. arXiv https://doi.org/10.48550/arxiv.1509.04760	text	January 2015
Magnetic Fluctuations, Precursor Phenomena and Phase Transition in MnSi under Magnetic Field Pappas, C.; Bannenberg, L. J.; Lelievre-Berna, E. arXiv https://doi.org/10.48550/arxiv.1606.07962	text	January 2016
Aging, memory, and nonhierarchical energy landscape of spin jam Samarakoon, Anjana; Sato, Taku J.; Chen, Tianran arXiv https://doi.org/10.48550/arxiv.1707.03086	text	January 2017
Scaling of Memories and Crossover in Glassy Magnets Samarakoon, A. M.; Takahashi, M.; Zhang, D. arXiv https://doi.org/10.48550/arxiv.1708.07974	preprint	January 2017
The High-Flux Backscattering Spectrometer at the NIST Center for Neutron Research Meyer, A.; Dimeo, R. M.; Gehring, P. M. arXiv https://doi.org/10.48550/arxiv.cond-mat/0209153	text	January 2002
Water Dynamics in Neural Tissue Natali, Francesca; Dolce, Caterina; Peters, Judith Journal of the Physical Society of Japan, Vol. 82, Issue Suppl.A https://doi.org/10.7566/JPSJS.82SA.SA017	journal	January 2013

Similar Records

Ultra-high resolution inelastic neutron scattering

Technical Report · 1992 · OSTI ID:6575771

Neumann, D A; Hammouda, B

Ultra-high resolution inelastic neutron scattering

Journal Article · · Journal of Research of the National Institute of Standards and Technology; (United States) · OSTI ID:5831094

Neumann, D A; Hammouda, B

Neutron resonance spin-echo upgrade at the three-axis spectrometer FLEXX

Journal Article · 2015 · Review of Scientific Instruments · OSTI ID:22392387

Quintero-Castro, D. L.; Habicht, K.; Keller, T.

Related Subjects

47 OTHER INSTRUMENTATION
biological physics
chemical physics
condensed-matter physics
soft materials

Title: High-resolution neutron spectroscopy using backscattering and neutron spin-echo spectrometers in soft and hard condensed matter

Citation Formats

References (148)

Similar Records

Related Subjects