Superconducting Dome in Nd1-xSrxNiO2 Infinite Layer Films

Li, Danfeng; Wang, Bai Yang; Lee, Kyuho; Harvey, Shannon P.; Osada, Motoki; Goodge, Berit H.; Kourkoutis, Lena F.; Hwang, Harold Y.

doi:10.1103/physrevlett.125.027001

Title: Superconducting Dome in Nd_1-xSr_xNiO₂ Infinite Layer Films

Abstract

We show the phase diagram of Nd_1-xSr_xNiO₂ infinite layer thin films grown on SrTiO₃. A superconducting dome spanning 0.125 < x < 0.25 is found, remarkably similar to cuprates, albeit over a narrower doping window. However, while cuprate superconductivity is bounded by an insulator for underdoping and a metal for overdoping, here we observe weakly insulating behavior on either side of the dome. Furthermore, the normal state Hall coefficient is always small and proximate to a continuous zero crossing in doping and in temperature, in contrast to the ~ 1/x dependence observed for cuprates. This suggests the presence of both electronlike and holelike bands, consistent with band structure calculations.

Authors:

^[1]; Wang, Bai Yang ^[1];

^[1];

^[2];

^[1]

SLAC National Accelerator Lab., Menlo Park, CA (United States); Stanford Univ., CA (United States)
Cornell Univ., Ithaca, NY (United States); Kavli Inst. at Cornell for Nanoscale Science, Ithaca, NY (United States)

Publication Date:: 2020-07-07

Research Org.:: SLAC National Accelerator Lab., Menlo Park, CA (United States)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

OSTI Identifier:: 1646809

Grant/Contract Number:: AC02-76SF00515; GBMF4415; FA 9550-16-1-0305; DMR-1539918; MRI-1429155; DMR-1719875

Resource Type:: Accepted Manuscript

Journal Name:: Physical Review Letters

Additional Journal Information:: Journal Volume: 125; Journal Issue: 2

Publisher:: American Physical Society (APS)

Country of Publication:: United States

Language:: English

Subject:: 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; Electrical conductivity; Hall effect; Phase diagrams; Superconductivity; Superconductors

Citation Formats


                    Li, Danfeng, Wang, Bai Yang, Lee, Kyuho, Harvey, Shannon P., Osada, Motoki, Goodge, Berit H., Kourkoutis, Lena F., and Hwang, Harold Y.. Superconducting Dome in Nd1-xSrxNiO2 Infinite Layer Films.  United States: N. p., 2020. 
Web.  doi:10.1103/physrevlett.125.027001.

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                    Li, Danfeng, Wang, Bai Yang, Lee, Kyuho, Harvey, Shannon P., Osada, Motoki, Goodge, Berit H., Kourkoutis, Lena F., & Hwang, Harold Y.. Superconducting Dome in Nd1-xSrxNiO2 Infinite Layer Films.  United States.  https://doi.org/10.1103/physrevlett.125.027001

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                    Li, Danfeng, Wang, Bai Yang, Lee, Kyuho, Harvey, Shannon P., Osada, Motoki, Goodge, Berit H., Kourkoutis, Lena F., and Hwang, Harold Y.. Tue .  
"Superconducting Dome in Nd1-xSrxNiO2 Infinite Layer Films".  United States.  https://doi.org/10.1103/physrevlett.125.027001.  https://www.osti.gov/servlets/purl/1646809.

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@article{osti_1646809,

  title        = {Superconducting Dome in Nd1-xSrxNiO2 Infinite Layer Films},

  author       = {Li, Danfeng and Wang, Bai Yang and Lee, Kyuho and Harvey, Shannon P. and Osada, Motoki and Goodge, Berit H. and Kourkoutis, Lena F. and Hwang, Harold Y.},

  abstractNote = {We show the phase diagram of Nd1-xSrxNiO2 infinite layer thin films grown on SrTiO3. A superconducting dome spanning 0.125 < x < 0.25 is found, remarkably similar to cuprates, albeit over a narrower doping window. However, while cuprate superconductivity is bounded by an insulator for underdoping and a metal for overdoping, here we observe weakly insulating behavior on either side of the dome. Furthermore, the normal state Hall coefficient is always small and proximate to a continuous zero crossing in doping and in temperature, in contrast to the ~ 1/x dependence observed for cuprates. This suggests the presence of both electronlike and holelike bands, consistent with band structure calculations.},

  doi          = {10.1103/physrevlett.125.027001},

  journal      = {Physical Review Letters},

  number       = 2,

  volume       = 125,

  place        = {United States},

  year         = {2020},

  month        = {7}

}

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Title: Superconducting Dome in Nd1-xSrxNiO2 Infinite Layer Films

Abstract

Citation Formats

Electronic structure of possible nickelate analogs to the cuprates journal, March 1999

Role of 4 f states in infinite-layer NdNiO 2 journal, January 2020

Critical Nature of the Ni Spin State in Doped NdNiO 2 journal, May 2020

Aspects of the synthesis of thin film superconducting infinite-layer nickelates journal, April 2020

Hall effect of La 2 − x Sr x CuO 4 : Implications for the electronic structure in the normal state journal, June 1987

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Complexity in Strongly Correlated Electronic Systems journal, July 2005

Nickelate superconductors: Multiorbital nature and spin freezing journal, January 2020

Type-II t − J model in superconducting nickelate Nd 1 − x Sr x NiO 2 journal, May 2020

Scaling of the temperature dependent Hall effect in La 2 − x Sr x CuO 4 journal, April 1994

From quantum matter to high-temperature superconductivity in copper oxides journal, February 2015

Superconductivity produced by electron doping in CuO 2 -layered compounds journal, March 1989

Superconductor-to-nonsuperconductor transition in ( La 1 − x Sr x ) 2 CuO 4 as investigated by transport and magnetic measurements journal, August 1989

Sodium Hydride as a Powerful Reducing Agent for Topotactic Oxide Deintercalation: Synthesis and Characterization of the Nickel(I) Oxide LaNiO 2 journal, September 1999

Lifshitz transition and frustration of magnetic moments in infinite-layer NdNiO 2 upon hole doping journal, June 2020

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Superconductivity in an infinite-layer nickelate journal, August 2019

Infinite-layer La Ni O 2 : Ni 1 + is not Cu 2 + journal, October 2004

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Stacked charge stripes in the quasi-2D trilayer nickelate La 4 Ni 3 O 8 journal, July 2016

Charge modulations in La 2 − x Sr x NiO 4 + y : Ordering of polarons journal, October 1993

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Anomalous electron transport in epitaxial NdNiO 3 films journal, June 2019

Charge-ordered states in (La,Sr ) 2 NiO 4 for hole concentrations n h =1/3 and 1/2 journal, March 1994

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Scattering and Pairing in Cuprate Superconductors journal, August 2010

Simultaneous Ordering of Holes and Spins in La 2 Ni O 4.125 journal, August 1994

Progress and perspectives on electron-doped cuprates journal, September 2010

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Similarities and Differences between LaNiO 2 and CaCuO 2 and Implications for Superconductivity journal, February 2020

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Title: Superconducting Dome in Nd_1-xSr_xNiO₂ Infinite Layer Films

Electronic structure of possible nickelate analogs to the cuprates
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Role of $4 f$ states in infinite-layer ${NdNiO}_{2}$
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Critical Nature of the Ni Spin State in Doped ${NdNiO}_{2}$
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Aspects of the synthesis of thin film superconducting infinite-layer nickelates
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Hall effect of ${La}_{2 - x}$ ${Sr}_{x}$ ${CuO}_{4}$ : Implications for the electronic structure in the normal state
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journal, January 2020

Complexity in Strongly Correlated Electronic Systems
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Type-II $t − J$ model in superconducting nickelate ${Nd}_{1 - x} {Sr}_{x} {NiO}_{2}$
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Scaling of the temperature dependent Hall effect in ${La}_{2 - x}$ ${Sr}_{x}$ ${CuO}_{4}$
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From quantum matter to high-temperature superconductivity in copper oxides
journal, February 2015

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journal, March 1989

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Sodium Hydride as a Powerful Reducing Agent for Topotactic Oxide Deintercalation: Synthesis and Characterization of the Nickel(I) Oxide LaNiO ₂
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Lifshitz transition and frustration of magnetic moments in infinite-layer ${NdNiO}_{2}$ upon hole doping
journal, June 2020

Similarity of Scattering Rates in Metals Showing T-Linear Resistivity
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Two-band model for magnetism and superconductivity in nickelates
journal, December 2019

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Superconductivity in an infinite-layer nickelate
journal, August 2019

Infinite-layer $La Ni O_{2}$ : ${Ni}^{1 +}$ is not ${Cu}^{2 +}$
journal, October 2004

Superconductivity seen in a non-magnetic nickel oxide
journal, August 2019

Superconducting properties of ${La}_{2 - x}$ ${Ba}_{x}$ ${CuO}_{4}$
journal, September 1988

Formation of a two-dimensional single-component correlated electron system and band engineering in the nickelate superconductor ${NdNiO}_{2}$
journal, November 2019

Many-Body Electronic Structure of ${NdNiO}_{2}$ and ${CaCuO}_{2}$
journal, June 2020

Positive Hall coefficient observed in single-crystal ${Nd}_{2 - x}$ ${Ce}_{x}$ ${CuO}_{4 - δ}$ at low temperatures
journal, February 1991

Stacked charge stripes in the quasi-2D trilayer nickelate La ₄ Ni ₃ O ₈
journal, July 2016

Charge modulations in ${La}_{2 - x}$ ${Sr}_{x}$ ${NiO}_{4 + y}$ : Ordering of polarons
journal, October 1993

Synthesis of the infinite layer Ni(I) phase NdNiO2+x by low temperature reduction of NdNiO3 with sodium hydride
journal, June 2003

Anomalous electron transport in epitaxial ${NdNiO}_{3}$ films
journal, June 2019

Charge-ordered states in (La,Sr $)_{2}$ ${NiO}_{4}$ for hole concentrations $n_{h}$ =1/3 and 1/2
journal, March 1994

Tunable resistivity exponents in the metallic phase of epitaxial nickelates
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Scattering and Pairing in Cuprate Superconductors
journal, August 2010

Simultaneous Ordering of Holes and Spins in ${La}_{2}$ Ni $O_{4.125}$
journal, August 1994

Progress and perspectives on electron-doped cuprates
journal, September 2010

Electronic structure of the parent compound of superconducting infinite-layer nickelates
journal, January 2020

Similarities and Differences between ${LaNiO}_{2}$ and ${CaCuO}_{2}$ and Implications for Superconductivity
journal, February 2020

Violation of the isotropic mean free path approximation for overdoped ${La}_{2 - x} {Sr}_{x} {CuO}_{4}$
journal, June 2008

Effective-field theory of local-moment formation in disordered metals
journal, July 1989