Performance of sweeping gas membrane distillation for treating produced water: Modeling and experiments
Abstract
Membrane distillation (MD) has shown promise for desalination of produced water (PW), but there are very few studies reported on the performance of MD with real PW and the characteristics of the fouling and scaling in MD. Among different MD configurations, sweeping gas MD (SGMD) is the least studied configuration. Here we report the application of SGMD for treating high-salinity PW (123 g L-1). The SGMD operating conditions were first carefully optimized through pure water MD experiments by varying operating conditions. The flux evaluation was accompanied by a detailed Aspen Custom Modeler simulation based on the electrolyte-NRTL thermodynamic model to better understand the heat and mass transfer in the feed and permeate channel. Supported by experiments, modeling results confirmed the partial condensation of the vapor in the permeate channel. Furthermore, it was concluded that the saturation of the sweeping gas is controlling the overall mass transfer through the membrane. Selected membranes and optimized conditions were then used to conduct short-term and long-term performance tests with PW. In long-term MD test, the concentration of the PW increased by a factor of two (50% water recovery), while the membrane exhibited small flux decline. Elemental analysis showed that strontium and sodium were themore »
- Authors:
-
- Texas Tech Univ., Lubbock, TX (United States). Dept. of Chemical Engineering
- Publication Date:
- Research Org.:
- American Institute of Chemical Engineers (AIChE), New York, NY (United States)
- Sponsoring Org.:
- USDOE Office of Energy Efficiency and Renewable Energy (EERE)
- OSTI Identifier:
- 1848618
- Alternate Identifier(s):
- OSTI ID: 1642343
- Grant/Contract Number:
- EE0007888
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Desalination
- Additional Journal Information:
- Journal Volume: 492; Journal Issue: C; Journal ID: ISSN 0011-9164
- Publisher:
- Elsevier
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 42 ENGINEERING; 54 ENVIRONMENTAL SCIENCES; Engineering; Water Resources; Membrane Distillation; Sweeping Gas; Produced Water; High Salinity; Scaling; Modeling
Citation Formats
Thakur, Amit K., Hsieh, I-Min, Islam, Md R., Lin, Boson, Chen, Chau-Chyun, and Malmali, Mahdi. Performance of sweeping gas membrane distillation for treating produced water: Modeling and experiments. United States: N. p., 2020.
Web. doi:10.1016/j.desal.2020.114597.
Thakur, Amit K., Hsieh, I-Min, Islam, Md R., Lin, Boson, Chen, Chau-Chyun, & Malmali, Mahdi. Performance of sweeping gas membrane distillation for treating produced water: Modeling and experiments. United States. https://doi.org/10.1016/j.desal.2020.114597
Thakur, Amit K., Hsieh, I-Min, Islam, Md R., Lin, Boson, Chen, Chau-Chyun, and Malmali, Mahdi. Thu .
"Performance of sweeping gas membrane distillation for treating produced water: Modeling and experiments". United States. https://doi.org/10.1016/j.desal.2020.114597. https://www.osti.gov/servlets/purl/1848618.
@article{osti_1848618,
title = {Performance of sweeping gas membrane distillation for treating produced water: Modeling and experiments},
author = {Thakur, Amit K. and Hsieh, I-Min and Islam, Md R. and Lin, Boson and Chen, Chau-Chyun and Malmali, Mahdi},
abstractNote = {Membrane distillation (MD) has shown promise for desalination of produced water (PW), but there are very few studies reported on the performance of MD with real PW and the characteristics of the fouling and scaling in MD. Among different MD configurations, sweeping gas MD (SGMD) is the least studied configuration. Here we report the application of SGMD for treating high-salinity PW (123 g L-1). The SGMD operating conditions were first carefully optimized through pure water MD experiments by varying operating conditions. The flux evaluation was accompanied by a detailed Aspen Custom Modeler simulation based on the electrolyte-NRTL thermodynamic model to better understand the heat and mass transfer in the feed and permeate channel. Supported by experiments, modeling results confirmed the partial condensation of the vapor in the permeate channel. Furthermore, it was concluded that the saturation of the sweeping gas is controlling the overall mass transfer through the membrane. Selected membranes and optimized conditions were then used to conduct short-term and long-term performance tests with PW. In long-term MD test, the concentration of the PW increased by a factor of two (50% water recovery), while the membrane exhibited small flux decline. Elemental analysis showed that strontium and sodium were the major scalant compounds.},
doi = {10.1016/j.desal.2020.114597},
journal = {Desalination},
number = C,
volume = 492,
place = {United States},
year = {Thu Jul 23 00:00:00 EDT 2020},
month = {Thu Jul 23 00:00:00 EDT 2020}
}
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