Charging activation and desulfurization of MnS unlock the active sites and electrochemical reactivity for Zn-ion batteries

Chen, Xiujuan; Li, Wei; Xu, Yaobin; Zeng, Zhipeng; Tian, Hanchen; Velayutham, Murugesan; Shi, Wangying; Li, Wenyuan; Wang, Chongmin; Reed, David; Khramtsov, Valery V.; Li, Xiaolin; Liu, Xingbo

doi:10.1016/j.nanoen.2020.104869

Title: Charging activation and desulfurization of MnS unlock the active sites and electrochemical reactivity for Zn-ion batteries

Authors:

; Li, Wei; Xu, Yaobin; Zeng, Zhipeng;

; Velayutham, Murugesan; Shi, Wangying; Li, Wenyuan; Wang, Chongmin; Reed, David; Khramtsov, Valery V.; Li, Xiaolin;

Publication Date:: 2020-09-01

Sponsoring Org.:: USDOE

OSTI Identifier:: 1637367

Resource Type:: Publisher's Accepted Manuscript

Journal Name:: Nano Energy

Additional Journal Information:: Journal Name: Nano Energy Journal Volume: 75 Journal Issue: C; Journal ID: ISSN 2211-2855

Publisher:: Elsevier

Country of Publication:: Netherlands

Language:: English

Citation Formats


                    Chen, Xiujuan, Li, Wei, Xu, Yaobin, Zeng, Zhipeng, Tian, Hanchen, Velayutham, Murugesan, Shi, Wangying, Li, Wenyuan, Wang, Chongmin, Reed, David, Khramtsov, Valery V., Li, Xiaolin, and Liu, Xingbo. Charging activation and desulfurization of MnS unlock the active sites and electrochemical reactivity for Zn-ion batteries.  Netherlands: N. p., 2020. 
Web.  doi:10.1016/j.nanoen.2020.104869.

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                    Chen, Xiujuan, Li, Wei, Xu, Yaobin, Zeng, Zhipeng, Tian, Hanchen, Velayutham, Murugesan, Shi, Wangying, Li, Wenyuan, Wang, Chongmin, Reed, David, Khramtsov, Valery V., Li, Xiaolin, & Liu, Xingbo. Charging activation and desulfurization of MnS unlock the active sites and electrochemical reactivity for Zn-ion batteries.  Netherlands.  https://doi.org/10.1016/j.nanoen.2020.104869

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                    Chen, Xiujuan, Li, Wei, Xu, Yaobin, Zeng, Zhipeng, Tian, Hanchen, Velayutham, Murugesan, Shi, Wangying, Li, Wenyuan, Wang, Chongmin, Reed, David, Khramtsov, Valery V., Li, Xiaolin, and Liu, Xingbo. Tue .  
"Charging activation and desulfurization of MnS unlock the active sites and electrochemical reactivity for Zn-ion batteries".  Netherlands.  https://doi.org/10.1016/j.nanoen.2020.104869.

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@article{osti_1637367,

  title        = {Charging activation and desulfurization of MnS unlock the active sites and electrochemical reactivity for Zn-ion batteries},

  author       = {Chen, Xiujuan and Li, Wei and Xu, Yaobin and Zeng, Zhipeng and Tian, Hanchen and Velayutham, Murugesan and Shi, Wangying and Li, Wenyuan and Wang, Chongmin and Reed, David and Khramtsov, Valery V. and Li, Xiaolin and Liu, Xingbo},

  abstractNote = {},

  doi          = {10.1016/j.nanoen.2020.104869},

  journal      = {Nano Energy},

  number       = C,

  volume       = 75,

  place        = {Netherlands},

  year         = {2020},

  month        = {9}

}

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DOI: 10.1149/1.1362539

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Citation Formats

The Manganese Dioxide Electrode in Alkaline Electrolyte; The Electron-Proton Mechanism for the Discharge Process from MnO[sub 2] to MnO[sub 1.5] journal, January 1966

Characterization of the Bismuth-Modified Manganese Dioxide Cathodes in Rechargeable Alkaline Cells journal, January 2002

Rechargeability and economic aspects of alkaline zinc–manganese dioxide cells for electrical storage and load leveling journal, February 2015

Nanostructured Mn-based oxides for electrochemical energy storage and conversion journal, January 2015

Manganese Sesquioxide as Cathode Material for Multivalent Zinc Ion Battery with High Capacity and Long Cycle Life journal, March 2017

Electro-Deposition and Dissolution of MnO 2 on a Graphene Composite Electrode for Its Utilization in an Aqueous Based Hybrid Supercapacitor journal, January 2012

Rechargeable Zn∣ZnSO4∣MnO2-type cells journal, July 1986

Recent Advances in Zn-Ion Batteries journal, August 2018

The oxygen evolution reaction enabled by transition metal phosphide and chalcogenide pre-catalysts with dynamic changes journal, January 2019

Low-cost and large-scale synthesis of alkaline earth metal germanate nanowires as a new class of lithium ion battery anode material journal, January 2012

Energetic Zinc Ion Chemistry: The Rechargeable Zinc Ion Battery journal, December 2011

Electrochemically Induced Structural Transformation in a γ-MnO 2 Cathode of a High Capacity Zinc-Ion Battery System journal, May 2015

High-Performance Reversible Aqueous Zn-Ion Battery Based on Porous MnO x Nanorods Coated by MOF-Derived N-Doped Carbon journal, August 2018

Zinc ion stabilized MnO 2 nanospheres for high capacity and long lifespan aqueous zinc-ion batteries journal, January 2019

Zn/MnO 2 Battery Chemistry With H + and Zn 2+ Coinsertion journal, July 2017

Built-in oriented electric field facilitating durable Zn MnO2 battery journal, August 2019

Potassium vanadates with stable structure and fast ion diffusion channel as cathode for rechargeable aqueous zinc-ion batteries journal, September 2018

Transition metal ion-preintercalated V2O5 as high-performance aqueous zinc-ion battery cathode with broad temperature adaptability journal, July 2019

Adsorption energy engineering of nickel oxide hybrid nanosheets for high areal capacity flexible lithium-ion batteries journal, March 2020

Hierarchical Co 3 O 4 @N-Doped Carbon Composite as an Advanced Anode Material for Ultrastable Potassium Storage journal, March 2020

Chemical extraction of Zn from ZnMn 2 O 4 -based spinels journal, January 2015

Interfacing nickel nitride and nickel boosts both electrocatalytic hydrogen evolution and oxidation reactions journal, October 2018

Elucidating the intercalation mechanism of zinc ions into α-MnO 2 for rechargeable zinc batteries journal, January 2015

Manganese Oxide Thin Film Preparation by Potentiostatic Electrolyses and Electrochromism journal, January 2000

Size effects and nanostructured materials for energy applications journal, January 2008

Issues and opportunities facing aqueous zinc-ion batteries journal, January 2019

Zinc-manganese dioxide galvanic cell using zinc sulphate as electrolyte. Rechargeability of the cell journal, July 1988

Orderly integration of porous TiO 2 (B) nanosheets into bunchy hierarchical structure for high-rate and ultralong-lifespan lithium-ion batteries journal, January 2017

Advanced rechargeable zinc-based batteries: Recent progress and future perspectives journal, August 2019

Understanding the Low-Voltage Hysteresis of Anionic Redox in Na 2 Mn 3 O 7 journal, May 2019

The Cathodic Reduction Mechanism of Electrolytic Manganese Dioxide in Alkaline Electrolyte journal, January 1965

Nitrogen-Doped Perovskite as a Bifunctional Cathode Catalyst for Rechargeable Lithium–Oxygen Batteries journal, January 2018

Initiating a mild aqueous electrolyte Co 3 O 4 /Zn battery with 2.2 V-high voltage and 5000-cycle lifespan by a Co( iii ) rich-electrode journal, January 2018

Aqueous vs. nonaqueous Zn-ion batteries: consequences of the desolvation penalty at the interface journal, January 2018

In Situ Electrochemical Oxidation Tuning of Transition Metal Disulfides to Oxides for Enhanced Water Oxidation journal, July 2015

Joint Charge Storage for High‐Rate Aqueous Zinc–Manganese Dioxide Batteries journal, May 2019

The Effect of Electrode-Electrolyte Interface on the Electrochemical Impedance Spectra for Positive Electrode in Li-Ion Battery journal, November 2018

Novel Insights into Energy Storage Mechanism of Aqueous Rechargeable Zn/MnO2 Batteries with Participation of Mn2+ journal, June 2019

Selective sodium intercalation into sodium nickel–manganese sulfate for dual Na–Li-ion batteries journal, January 2018

An Electrolytic Zn–MnO 2 Battery for High‐Voltage and Scalable Energy Storage journal, June 2019

Electrolyzer Design for Flexible Decoupled Water Splitting and Organic Upgrading with Electron Reservoirs journal, March 2018

Programmed Design of a Lithium–Sulfur Battery Cathode by Integrating Functional Units journal, July 2019

Nanostructured anode materials for lithium ion batteries journal, January 2015

A high-capacity and long-life aqueous rechargeable zinc battery using a metal oxide intercalation cathode journal, August 2016

Inverse opal manganese dioxide constructed by few-layered ultrathin nanosheets as high-performance cathodes for aqueous zinc-ion batteries journal, May 2019

Crystal Structure Modeling of a Highly Disordered Potassium Birnessite journal, January 1996

TiC supported amorphous MnOx as highly efficient bifunctional electrocatalyst for corrosion resistant oxygen electrode of Zn-air batteries journal, January 2020

Polyaniline-intercalated manganese dioxide nanolayers as a high-performance cathode material for an aqueous zinc-ion battery journal, July 2018

A zinc battery with ultra-flat discharge plateau through phase transition mechanism journal, May 2020

Cation-Deficient Spinel ZnMn 2 O 4 Cathode in Zn(CF 3 SO 3 ) 2 Electrolyte for Rechargeable Aqueous Zn-Ion Battery journal, September 2016

Nano active materials for lithium-ion batteries journal, January 2010

Reactive oxygen species scavenging with a biodegradable, thermally responsive hydrogel compatible with soft tissue injection journal, September 2018

Pursuing the stabilisation of crystalline nanostructured magnetic manganites through a green low temperature hydrothermal synthesis journal, January 2017

Charging and discharging behavior of zinc—manganese dioxide galvanic cells using zinc sulfate as electrolyte journal, December 1993

Rapid electrochemical synthesis of δ-MnO2 from γ-MnO2 and unleashing its performance as an energy dense electrode journal, December 2017

Suppressing Ion Transfer Enables Versatile Measurements of Electrochemical Surface Area for Intrinsic Activity Comparisons journal, February 2018

A General Thermodynamic Theory of the Potential of Passive Electrodes and Its Influence on Passive Corrosion journal, January 1963

Synthesis, structure, and magnetic behavior of nanoparticles of cubic ZnMnO 3 journal, June 2012

Crystal water for high performance layered manganese oxide cathodes in aqueous rechargeable zinc batteries journal, January 2019

Surface functionalized 3D carbon fiber boosts the lithium storage behaviour of transition metal oxide nanowires via strong electronic interaction and tunable adsorption energy journal, January 2019

Dehydration behaviors of interlayer water in systhetic Buserites journal, September 2004

Achieving Ultrahigh Energy Density and Long Durability in a Flexible Rechargeable Quasi-Solid-State Zn-MnO 2 Battery journal, April 2017

Rechargeable aqueous zinc-manganese dioxide batteries with high energy and power densities journal, September 2017

Cathodic Reduction Mechanism of MnOOH to Mn(OH)[sub 2] in Alkaline Electrolyte journal, January 1968

Rechargeability of aqueous sulfate Zn/MnO2 batteries enhanced by accessible Mn2+ ions journal, November 2018

Synthesis, electrical resistivity, thermo-electric power and magnetization of cubic ZnMnO3 journal, March 2011

Towards High-Voltage Aqueous Metal-Ion Batteries Beyond 1.5 V: The Zinc/Zinc Hexacyanoferrate System journal, September 2014

Zn sorption modifies dynamically the layer and interlayer structure of vernadite journal, May 2012

Reversible aqueous zinc/manganese oxide energy storage from conversion reactions journal, April 2016

Effect of Zn coprecipitation on the structure of layered Mn oxides journal, August 2018

Zinc hydroxide sulphate and its transformation to crystalline zinc oxide journal, January 2013

Interfacial Sites between Cobalt Nitride and Cobalt Act as Bifunctional Catalysts for Hydrogen Electrochemistry journal, June 2019

V2O5 nanopaper as a cathode material with high capacity and long cycle life for rechargeable aqueous zinc-ion battery journal, June 2019

Extracting oxygen anions from ZnMn2O4: Robust cathode for flexible all-solid-state Zn-ion batteries journal, September 2019

Defect Engineering of Oxygen‐Deficient Manganese Oxide to Achieve High‐Performing Aqueous Zinc Ion Battery journal, February 2019

Recent Advances in Flexible Zinc-Based Rechargeable Batteries journal, November 2018

Investigation of zinc ion storage of transition metal oxides, sulfides, and borides in zinc ion battery systems journal, January 2017

Layered VS 2 Nanosheet-Based Aqueous Zn Ion Battery Cathode journal, January 2017

The Manganese Dioxide Electrode in Alkaline Electrolyte; The Electron-Proton Mechanism for the Discharge Process from MnO[sub 2] to MnO[sub 1.5]
journal, January 1966

Characterization of the Bismuth-Modified Manganese Dioxide Cathodes in Rechargeable Alkaline Cells
journal, January 2002

Rechargeability and economic aspects of alkaline zinc–manganese dioxide cells for electrical storage and load leveling
journal, February 2015

Nanostructured Mn-based oxides for electrochemical energy storage and conversion
journal, January 2015

Manganese Sesquioxide as Cathode Material for Multivalent Zinc Ion Battery with High Capacity and Long Cycle Life
journal, March 2017

Electro-Deposition and Dissolution of MnO ₂ on a Graphene Composite Electrode for Its Utilization in an Aqueous Based Hybrid Supercapacitor
journal, January 2012

Rechargeable Zn∣ZnSO4∣MnO2-type cells
journal, July 1986

Recent Advances in Zn-Ion Batteries
journal, August 2018

The oxygen evolution reaction enabled by transition metal phosphide and chalcogenide pre-catalysts with dynamic changes
journal, January 2019

Low-cost and large-scale synthesis of alkaline earth metal germanate nanowires as a new class of lithium ion battery anode material
journal, January 2012

Energetic Zinc Ion Chemistry: The Rechargeable Zinc Ion Battery
journal, December 2011

Electrochemically Induced Structural Transformation in a γ-MnO ₂ Cathode of a High Capacity Zinc-Ion Battery System
journal, May 2015

High-Performance Reversible Aqueous Zn-Ion Battery Based on Porous MnO _x Nanorods Coated by MOF-Derived N-Doped Carbon
journal, August 2018

Zinc ion stabilized MnO 2 nanospheres for high capacity and long lifespan aqueous zinc-ion batteries
journal, January 2019

Zn/MnO ₂ Battery Chemistry With H ⁺ and Zn ²⁺ Coinsertion
journal, July 2017

Built-in oriented electric field facilitating durable Zn MnO2 battery
journal, August 2019

Potassium vanadates with stable structure and fast ion diffusion channel as cathode for rechargeable aqueous zinc-ion batteries
journal, September 2018

Transition metal ion-preintercalated V2O5 as high-performance aqueous zinc-ion battery cathode with broad temperature adaptability
journal, July 2019

Adsorption energy engineering of nickel oxide hybrid nanosheets for high areal capacity flexible lithium-ion batteries
journal, March 2020

Hierarchical Co ₃ O ₄ @N-Doped Carbon Composite as an Advanced Anode Material for Ultrastable Potassium Storage
journal, March 2020

Chemical extraction of Zn from ZnMn ₂ O ₄ -based spinels
journal, January 2015

Interfacing nickel nitride and nickel boosts both electrocatalytic hydrogen evolution and oxidation reactions
journal, October 2018

Elucidating the intercalation mechanism of zinc ions into α-MnO ₂ for rechargeable zinc batteries
journal, January 2015

Manganese Oxide Thin Film Preparation by Potentiostatic Electrolyses and Electrochromism
journal, January 2000

Size effects and nanostructured materials for energy applications
journal, January 2008

Issues and opportunities facing aqueous zinc-ion batteries
journal, January 2019

Zinc-manganese dioxide galvanic cell using zinc sulphate as electrolyte. Rechargeability of the cell
journal, July 1988

Orderly integration of porous TiO 2 (B) nanosheets into bunchy hierarchical structure for high-rate and ultralong-lifespan lithium-ion batteries
journal, January 2017

Advanced rechargeable zinc-based batteries: Recent progress and future perspectives
journal, August 2019

Understanding the Low-Voltage Hysteresis of Anionic Redox in Na ₂ Mn ₃ O ₇
journal, May 2019

The Cathodic Reduction Mechanism of Electrolytic Manganese Dioxide in Alkaline Electrolyte
journal, January 1965

Nitrogen-Doped Perovskite as a Bifunctional Cathode Catalyst for Rechargeable Lithium–Oxygen Batteries
journal, January 2018

Initiating a mild aqueous electrolyte Co ₃ O ₄ /Zn battery with 2.2 V-high voltage and 5000-cycle lifespan by a Co( iii ) rich-electrode
journal, January 2018

Aqueous vs. nonaqueous Zn-ion batteries: consequences of the desolvation penalty at the interface
journal, January 2018

In Situ Electrochemical Oxidation Tuning of Transition Metal Disulfides to Oxides for Enhanced Water Oxidation
journal, July 2015

Joint Charge Storage for High‐Rate Aqueous Zinc–Manganese Dioxide Batteries
journal, May 2019

The Effect of Electrode-Electrolyte Interface on the Electrochemical Impedance Spectra for Positive Electrode in Li-Ion Battery
journal, November 2018

Novel Insights into Energy Storage Mechanism of Aqueous Rechargeable Zn/MnO2 Batteries with Participation of Mn2+
journal, June 2019

Selective sodium intercalation into sodium nickel–manganese sulfate for dual Na–Li-ion batteries
journal, January 2018

An Electrolytic Zn–MnO ₂ Battery for High‐Voltage and Scalable Energy Storage
journal, June 2019

Electrolyzer Design for Flexible Decoupled Water Splitting and Organic Upgrading with Electron Reservoirs
journal, March 2018

Programmed Design of a Lithium–Sulfur Battery Cathode by Integrating Functional Units
journal, July 2019

Nanostructured anode materials for lithium ion batteries
journal, January 2015

A high-capacity and long-life aqueous rechargeable zinc battery using a metal oxide intercalation cathode
journal, August 2016

Inverse opal manganese dioxide constructed by few-layered ultrathin nanosheets as high-performance cathodes for aqueous zinc-ion batteries
journal, May 2019

Crystal Structure Modeling of a Highly Disordered Potassium Birnessite
journal, January 1996

TiC supported amorphous MnOx as highly efficient bifunctional electrocatalyst for corrosion resistant oxygen electrode of Zn-air batteries
journal, January 2020

Polyaniline-intercalated manganese dioxide nanolayers as a high-performance cathode material for an aqueous zinc-ion battery
journal, July 2018

A zinc battery with ultra-flat discharge plateau through phase transition mechanism
journal, May 2020

Cation-Deficient Spinel ZnMn ₂ O ₄ Cathode in Zn(CF ₃ SO ₃ ) ₂ Electrolyte for Rechargeable Aqueous Zn-Ion Battery
journal, September 2016

Nano active materials for lithium-ion batteries
journal, January 2010

Reactive oxygen species scavenging with a biodegradable, thermally responsive hydrogel compatible with soft tissue injection
journal, September 2018

Pursuing the stabilisation of crystalline nanostructured magnetic manganites through a green low temperature hydrothermal synthesis
journal, January 2017

Charging and discharging behavior of zinc—manganese dioxide galvanic cells using zinc sulfate as electrolyte
journal, December 1993

Rapid electrochemical synthesis of δ-MnO2 from γ-MnO2 and unleashing its performance as an energy dense electrode
journal, December 2017

Suppressing Ion Transfer Enables Versatile Measurements of Electrochemical Surface Area for Intrinsic Activity Comparisons
journal, February 2018

A General Thermodynamic Theory of the Potential of Passive Electrodes and Its Influence on Passive Corrosion
journal, January 1963

Synthesis, structure, and magnetic behavior of nanoparticles of cubic ZnMnO ₃
journal, June 2012

Crystal water for high performance layered manganese oxide cathodes in aqueous rechargeable zinc batteries
journal, January 2019

Surface functionalized 3D carbon fiber boosts the lithium storage behaviour of transition metal oxide nanowires via strong electronic interaction and tunable adsorption energy
journal, January 2019

Dehydration behaviors of interlayer water in systhetic Buserites
journal, September 2004

Achieving Ultrahigh Energy Density and Long Durability in a Flexible Rechargeable Quasi-Solid-State Zn-MnO ₂ Battery
journal, April 2017

Rechargeable aqueous zinc-manganese dioxide batteries with high energy and power densities
journal, September 2017

Cathodic Reduction Mechanism of MnOOH to Mn(OH)[sub 2] in Alkaline Electrolyte
journal, January 1968

Rechargeability of aqueous sulfate Zn/MnO2 batteries enhanced by accessible Mn2+ ions
journal, November 2018

Synthesis, electrical resistivity, thermo-electric power and magnetization of cubic ZnMnO3
journal, March 2011

Towards High-Voltage Aqueous Metal-Ion Batteries Beyond 1.5 V: The Zinc/Zinc Hexacyanoferrate System
journal, September 2014

Zn sorption modifies dynamically the layer and interlayer structure of vernadite
journal, May 2012

Reversible aqueous zinc/manganese oxide energy storage from conversion reactions
journal, April 2016

Effect of Zn coprecipitation on the structure of layered Mn oxides
journal, August 2018

Zinc hydroxide sulphate and its transformation to crystalline zinc oxide
journal, January 2013

Interfacial Sites between Cobalt Nitride and Cobalt Act as Bifunctional Catalysts for Hydrogen Electrochemistry
journal, June 2019

V2O5 nanopaper as a cathode material with high capacity and long cycle life for rechargeable aqueous zinc-ion battery
journal, June 2019

Extracting oxygen anions from ZnMn2O4: Robust cathode for flexible all-solid-state Zn-ion batteries
journal, September 2019

Defect Engineering of Oxygen‐Deficient Manganese Oxide to Achieve High‐Performing Aqueous Zinc Ion Battery
journal, February 2019

Recent Advances in Flexible Zinc-Based Rechargeable Batteries
journal, November 2018

Investigation of zinc ion storage of transition metal oxides, sulfides, and borides in zinc ion battery systems
journal, January 2017

Layered VS ₂ Nanosheet-Based Aqueous Zn Ion Battery Cathode
journal, January 2017

Hydrothermal Synthesis of Monolithic Co ₃ Se ₄ Nanowire Electrodes for Oxygen Evolution and Overall Water Splitting with High Efficiency and Extraordinary Catalytic Stability
journal, May 2017

Reaction Mechanisms for Long-Life Rechargeable Zn/MnO ₂ Batteries
journal, June 2018