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Title: High-speed photographic study of vaporclouds from wet droplets and the subsequent solid particles in an inductively coupled plasma

Abstract

Movies of an inductively coupled plasma (ICP) while nebulizing a concentrated sample of yttrium were recorded using a high-speed camera with short exposure time (10 μs) and fast framing rate (5000 frames per s). Clouds from large droplets can be seen in several successive frames as they travel downstream in the axial channel of the ICP. These droplet clouds are superimposed on the usual spatial structure of red YO, neutral Y atom and blue Y+ emission. As a particular large droplet moves downstream, its red emission cloud evolves into a faint white streak with a surrounding cloud of blue Y+ emission. The streak is attributed to a solid residue from the droplet. The velocity of the droplet and subsequent particle is measured to be 28 m s-1. The general characteristics of the droplet and particle clouds agree well with previous photographic measurements and those by other methods such as laser induced-fluorescence or scattering.

Publication Date:
Research Org.:
Ames Lab., Ames, IA (United States)
Sponsoring Org.:
USDOE National Nuclear Security Administration (NNSA), Office of Defense Nuclear Nonproliferation
OSTI Identifier:
1634871
Alternate Identifier(s):
OSTI ID: 1633767
Report Number(s):
IS-J-10,244
Journal ID: ISSN 0267-9477; JASPE2
Grant/Contract Number:  
AC02-07CH11358
Resource Type:
Published Article
Journal Name:
Journal of Analytical Atomic Spectrometry
Additional Journal Information:
Journal Name: Journal of Analytical Atomic Spectrometry; Journal ID: ISSN 0267-9477
Publisher:
Royal Society of Chemistry
Country of Publication:
United Kingdom
Language:
English
Subject:
37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY

Citation Formats

High-speed photographic study of vaporclouds from wet droplets and the subsequent solid particles in an inductively coupled plasma. United Kingdom: N. p., 2020. Web. https://doi.org/10.1039/D0JA00210K.
High-speed photographic study of vaporclouds from wet droplets and the subsequent solid particles in an inductively coupled plasma. United Kingdom. https://doi.org/10.1039/D0JA00210K
Wed . "High-speed photographic study of vaporclouds from wet droplets and the subsequent solid particles in an inductively coupled plasma". United Kingdom. https://doi.org/10.1039/D0JA00210K.
@article{osti_1634871,
title = {High-speed photographic study of vaporclouds from wet droplets and the subsequent solid particles in an inductively coupled plasma},
author = {None, None},
abstractNote = {Movies of an inductively coupled plasma (ICP) while nebulizing a concentrated sample of yttrium were recorded using a high-speed camera with short exposure time (10 μs) and fast framing rate (5000 frames per s). Clouds from large droplets can be seen in several successive frames as they travel downstream in the axial channel of the ICP. These droplet clouds are superimposed on the usual spatial structure of red YO, neutral Y atom and blue Y+ emission. As a particular large droplet moves downstream, its red emission cloud evolves into a faint white streak with a surrounding cloud of blue Y+ emission. The streak is attributed to a solid residue from the droplet. The velocity of the droplet and subsequent particle is measured to be 28 m s-1. The general characteristics of the droplet and particle clouds agree well with previous photographic measurements and those by other methods such as laser induced-fluorescence or scattering.},
doi = {10.1039/D0JA00210K},
journal = {Journal of Analytical Atomic Spectrometry},
number = ,
volume = ,
place = {United Kingdom},
year = {2020},
month = {1}
}

Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record
https://doi.org/10.1039/D0JA00210K

Figures / Tables:

Fig. 1 Fig. 1: Successive frames from a small section of Video 1. Frame 690 is the first image from this clip. Alternate frames are numbered in the order they were measured. The time interval between frames was 200 μs. A white arrow pointing right denotes the first droplet cloud under discussion.more » The yellow arrow pointing left denotes the second such droplet.« less

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    Figures / Tables found in this record:

      Figures/Tables have been extracted from DOE-funded journal article accepted manuscripts.