Coherent two-dimensional Fourier transform spectroscopy using a 25 Tesla resistive magnet

Paul, Jagannath; Stevens, Christopher. E.; Smith, Ryan P.; Dey, Prasenjit; Mapara, Varun; Semenov, Dimitry; McGill, Steven A.; Kaindl, Robert A.; Hilton, David J.; Karaiskaj, Denis

doi:10.1063/1.5055891

Title: Coherent two-dimensional Fourier transform spectroscopy using a 25 Tesla resistive magnet

Journal Article · 04 June 2019 · Review of Scientific Instruments

DOI: https://doi.org/10.1063/1.5055891 · OSTI ID:1633234

Paul, Jagannath ^[1]; Stevens, Christopher. E. ^[1];

^[2]; Dey, Prasenjit ^[1]; Mapara, Varun ^[1]; Semenov, Dimitry ^[3];

^[3];

^[4]; Hilton, David J. ^[5];

^[1]

Univ. of South Florida, Tampa, FL (United States)
California State Univ., East Bay, Hayward, CA (United States); Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
Florida State Univ., Tallahassee, FL (United States). National High Magnetic Field Lab. (MagLab)
Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
Univ. of Alabama, Birmingham, AL (United States)

We performed nonlinear optical two-dimensional Fourier transform spectroscopy measurements using an optical resistive high-field magnet on GaAs quantum wells. Magnetic fields up to 25 T can be achieved using the split helix resistive magnet. Two-dimensional spectroscopy measurements based on the coherent four-wave mixing signal require phase stability. Therefore, these measurements are difficult to perform in environments prone to mechanical vibrations. Large resistive magnets use extensive quantities of cooling water, which causes mechanical vibrations, making two-dimensional Fourier transform spectroscopy very challenging. Here, we report on the strategies we used to overcome these challenges and maintain the required phase-stability throughout the measurement. A self-contained portable platform was used to set up the experiments within the time frame provided by a user facility. Furthermore, this platform was floated above the optical table in order to isolate it from vibrations originating from the resistive magnet. Finally, we present two-dimensional Fourier transform spectra obtained from GaAs quantum wells at magnetic fields up to 25 T and demonstrate the utility of this technique in providing important details, which are obscured in one dimensional spectroscopy.

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Research Organization:: Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC)

Grant/Contract Number:: AC02-05CH11231; AC0205CH11231; SC0012635

OSTI ID:: 1633234

Alternate ID(s):: OSTI ID: 1524466

Journal Information:: Review of Scientific Instruments, Vol. 90, Issue 6; ISSN 0034-6748

Publisher:: American Institute of Physics (AIP)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 1 work

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