The importance of anode protection towards lithium oxygen batteries
Abstract
Developing lithium oxygen (Li–O2) batteries is critical to achieve high energy density in energy storage devices. Benefiting from the low weight of the cathode reagent, oxygen, Li–O2 batteries possess a high theoretical energy density of 3500 W h kg-1 based on the formation of Li2O2. However, they face several challenges from the metal anode, the air electrode, and the unstable electrolyte. Although most studies have focused on the air electrode, the importance of the anode protection should not be neglected. Here, we aim to understand the challenges on the lithium anode in Li–O2 batteries, which include Li dendrite growth, parasitic reactions between Li and active species in the electrolyte, and the oxygen crossover effect. Also, recent advances on the Li protection in Li–O2 batteries will be introduced. This review emphasizes the importance of anode protection especially in an oxygen rich environment and could provide guidance for future development of Li–O2 batteries.
- Authors:
-
- Argonne National Lab. (ANL), Argonne, IL (United States). Chemical Sciences and Engineering Division
- Argonne National Lab. (ANL), Argonne, IL (United States). Chemical Sciences and Engineering Division; Stanford Univ., CA (United States); Imam Abdulrahman Bin Faisal Univ. (IAU), Dammam (Saudi Arabia)
- Publication Date:
- Research Org.:
- Argonne National Laboratory (ANL), Argonne, IL (United States)
- Sponsoring Org.:
- USDOE Office of Energy Efficiency and Renewable Energy (EERE), Transportation Office. Vehicle Technologies Office
- OSTI Identifier:
- 1633066
- Alternate Identifier(s):
- OSTI ID: 1595861
- Grant/Contract Number:
- AC02-06CH11357
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Journal of Materials Chemistry. A
- Additional Journal Information:
- Journal Volume: 8; Journal Issue: 7; Journal ID: ISSN 2050-7488
- Publisher:
- Royal Society of Chemistry
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 25 ENERGY STORAGE
Citation Formats
Bi, Xuanxuan, Amine, Khalil, and Lu, Jun. The importance of anode protection towards lithium oxygen batteries. United States: N. p., 2020.
Web. doi:10.1039/c9ta12414d.
Bi, Xuanxuan, Amine, Khalil, & Lu, Jun. The importance of anode protection towards lithium oxygen batteries. United States. https://doi.org/10.1039/c9ta12414d
Bi, Xuanxuan, Amine, Khalil, and Lu, Jun. Thu .
"The importance of anode protection towards lithium oxygen batteries". United States. https://doi.org/10.1039/c9ta12414d. https://www.osti.gov/servlets/purl/1633066.
@article{osti_1633066,
title = {The importance of anode protection towards lithium oxygen batteries},
author = {Bi, Xuanxuan and Amine, Khalil and Lu, Jun},
abstractNote = {Developing lithium oxygen (Li–O2) batteries is critical to achieve high energy density in energy storage devices. Benefiting from the low weight of the cathode reagent, oxygen, Li–O2 batteries possess a high theoretical energy density of 3500 W h kg-1 based on the formation of Li2O2. However, they face several challenges from the metal anode, the air electrode, and the unstable electrolyte. Although most studies have focused on the air electrode, the importance of the anode protection should not be neglected. Here, we aim to understand the challenges on the lithium anode in Li–O2 batteries, which include Li dendrite growth, parasitic reactions between Li and active species in the electrolyte, and the oxygen crossover effect. Also, recent advances on the Li protection in Li–O2 batteries will be introduced. This review emphasizes the importance of anode protection especially in an oxygen rich environment and could provide guidance for future development of Li–O2 batteries.},
doi = {10.1039/c9ta12414d},
journal = {Journal of Materials Chemistry. A},
number = 7,
volume = 8,
place = {United States},
year = {Thu Jan 09 00:00:00 EST 2020},
month = {Thu Jan 09 00:00:00 EST 2020}
}
Web of Science
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