Stress‐Induced Domain Wall Motion in a Ferroelastic Mn 3+ Spin Crossover Complex

Jakobsen, Vibe B.; Trzop, Elzbieta; Gavin, Laurence C.; Dobbelaar, Emiel; Chikara, Shalinee; Ding, Xiaxin; Esien, Kane; Müller‐Bunz, Helge; Felton, Solveig; Zapf, Vivien S.; Collet, Eric; Carpenter, Michael A.; Morgan, Grace G.

doi:10.1002/ange.202003041

Title: Stress‐Induced Domain Wall Motion in a Ferroelastic Mn ³⁺ Spin Crossover Complex

Journal Article · 08 June 2020 · Angewandte Chemie

DOI: https://doi.org/10.1002/ange.202003041 · OSTI ID:1632251

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^[2]; Gavin, Laurence C. ^[1];

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^[5]; Esien, Kane ^[6]; Müller‐Bunz, Helge ^[1];

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School of Chemistry University College Dublin Belfield Dublin 4 Ireland
Univ Rennes CNRS, IPR (Institut de Physique de Rennes)—UMR 6251 35000 Rennes France
School of Chemistry University College Dublin Belfield Dublin 4 Ireland, Current address: Technische Universität Kaiserslautern Kaiserslautern Germany
Department of Physics Auburn University Auburn AL 36849 USA, Current address: National High Magnetic Field Lab at Florida State University Tallahassee FL USA
National High Magnetic Field Laboratory Los Alamos National Laboratory Los Alamos NM 87545 USA, Current address: Idaho National Laboratory Idaho Falls ID USA
Centre for Nanostructured Media School of Mathematics and Physics Queen's University of Belfast Belfast BT7 1NN, Northern Ireland UK
National High Magnetic Field Laboratory Los Alamos National Laboratory Los Alamos NM 87545 USA
Department of Earth Sciences University of Cambridge Downing Street Cambridge CB2 3EQ UK

Abstract Domain wall motion is detected for the first time during the transition to a ferroelastic and spin state ordered phase of a spin crossover complex. Single‐crystal X‐ray diffraction and resonant ultrasound spectroscopy (RUS) revealed two distinct symmetry‐breaking phase transitions in the mononuclear Mn ³⁺ compound [Mn(3,5‐diBr‐sal ₂ (323))]BPh ₄ , 1. The first at 250 K, involves the space group change Cc → Pc and is thermodynamically continuous, while the second, Pc → P 1 at 85 K, is discontinuous and related to spin crossover and spin state ordering. Stress‐induced domain wall mobility was interpreted on the basis of a steep increase in acoustic loss immediately below the the Pc ‐ P 1 transition

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Sponsoring Organization:: USDOE

Grant/Contract Number:: SC0019330

OSTI ID:: 1632251

Journal Information:: Angewandte Chemie, Journal Name: Angewandte Chemie Journal Issue: 32 Vol. 132; ISSN 0044-8249

Publisher:: Wiley Blackwell (John Wiley & Sons)Copyright Statement

Country of Publication:: Germany

Language:: English

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