Tunable anomalous Hall conductivity through volume-wise magnetic competition in a topological kagome magnet

Guguchia, Z.; Verezhak, J. A. T.; Gawryluk, D. J.; Tsirkin, S. S.; Yin, J.-X.; Belopolski, I.; Zhou, H.; Simutis, G.; Zhang, S.-S.; Cochran, T. A.; Chang, G.; Pomjakushina, E.; Keller, L.; Skrzeczkowska, Z.; Wang, Q.; Lei, H. C.; Khasanov, R.; Amato, A.; Jia, S.; Neupert, T.; Luetkens, H.; Hasan, M. Z.

doi:10.1038/s41467-020-14325-w

Title: Tunable anomalous Hall conductivity through volume-wise magnetic competition in a topological kagome magnet

Abstract

Magnetic topological phases of quantum matter are an emerging frontier in physics and material science. Along these lines, several kagome magnets have appeared as the most promising platforms. Here, we explore magnetic correlations in the kagome magnet Co₃Sn₂S₂. Using muon spin-rotation, we present evidence for competing magnetic orders in the kagome lattice of this compound. Our results show that while the sample exhibits an out-of-plane ferromagnetic ground state, an in-plane antiferromagnetic state appears at temperatures above 90 K, eventually attaining a volume fraction of 80% around 170 K, before reaching a non-magnetic state. Strikingly, the reduction of the anomalous Hall conductivity (AHC) above 90 K linearly follows the disappearance of the volume fraction of the ferromagnetic state. We further show that the competition of these magnetic phases is tunable through applying either an external magnetic field or hydrostatic pressure. Our results taken together suggest the thermal and quantum tuning of Berry curvature induced AHC via external tuning of magnetic order.

Authors:

^[1]; Verezhak, J. A. T. ^[2];

^[3];

^[4]; Yin, J.-X. ^[5]; Belopolski, I. ^[5]; Zhou, H. ^[6]; Simutis, G. ^[2];

^[5]; Cochran, T. A. ^[5];

^[5];

^[3]; Keller, L. ^[7]; Skrzeczkowska, Z. ^[3]; Wang, Q. ^[8];

^[8]; Khasanov, R. ^[2];

^[2]; Jia, S. ^[6];

^[4] more »

Paul Scherrer Inst. (PSI), Villigen (Switzerland). Lab. for Muon Spin Spectroscopy; Princeton Univ., NJ (United States). Dept. of Physics
Paul Scherrer Inst. (PSI), Villigen (Switzerland). Lab. for Muon Spin Spectroscopy
Paul Scherrer Inst. (PSI), Villigen (Switzerland). Lab. for Multiscale Materials Experiments
Univ. of Zurich (Switzerland). Dept. of Physics
Princeton Univ., NJ (United States). Dept. of Physics
Peking Univ., Beijing (China). School of Physics; Univ. of Chinese Academy of Sciences, Beijing (China). CAS Center for Excellence in Topological Quantum Computation
Paul Scherrer Inst., Villigen (Switzerland). Lab. for Neutron Scattering
Renmin Univ. of China, Beijing (China). Dept. of Physics

Publication Date:: 2020-01-28

Research Org.:: Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES); National Key Research and Development Program of China; National Natural Science Foundation of China (NSFC); European Research Council (ERC); Swiss National Science Foundation (SNSF); Gordon and Betty Moore Foundation

OSTI Identifier:: 1632135

Grant/Contract Number:: AC02-05CH11231; FG-02-05ER46200; 2016YFA0300504; 11574394; 11774423; 11822412; ERC-StG-Neupert-757867-PARATOP; 206021_139082; GBMF4547

Resource Type:: Accepted Manuscript

Journal Name:: Nature Communications

Additional Journal Information:: Journal Volume: 11; Journal Issue: 1; Journal ID: ISSN 2041-1723

Publisher:: Nature Publishing Group

Country of Publication:: United States

Language:: English

Subject:: 71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS; magnetic properties and materials; topological insulators

Citation Formats


                    Guguchia, Z., Verezhak, J. A. T., Gawryluk, D. J., Tsirkin, S. S., Yin, J.-X., Belopolski, I., Zhou, H., Simutis, G., Zhang, S.-S., Cochran, T. A., Chang, G., Pomjakushina, E., Keller, L., Skrzeczkowska, Z., Wang, Q., Lei, H. C., Khasanov, R., Amato, A., Jia, S., Neupert, T., Luetkens, H., and Hasan, M. Z. Tunable anomalous Hall conductivity through volume-wise magnetic competition in a topological kagome magnet.  United States: N. p., 2020. 
Web.  doi:10.1038/s41467-020-14325-w.

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                    Guguchia, Z., Verezhak, J. A. T., Gawryluk, D. J., Tsirkin, S. S., Yin, J.-X., Belopolski, I., Zhou, H., Simutis, G., Zhang, S.-S., Cochran, T. A., Chang, G., Pomjakushina, E., Keller, L., Skrzeczkowska, Z., Wang, Q., Lei, H. C., Khasanov, R., Amato, A., Jia, S., Neupert, T., Luetkens, H., & Hasan, M. Z. Tunable anomalous Hall conductivity through volume-wise magnetic competition in a topological kagome magnet.  United States.  https://doi.org/10.1038/s41467-020-14325-w

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                    Guguchia, Z., Verezhak, J. A. T., Gawryluk, D. J., Tsirkin, S. S., Yin, J.-X., Belopolski, I., Zhou, H., Simutis, G., Zhang, S.-S., Cochran, T. A., Chang, G., Pomjakushina, E., Keller, L., Skrzeczkowska, Z., Wang, Q., Lei, H. C., Khasanov, R., Amato, A., Jia, S., Neupert, T., Luetkens, H., and Hasan, M. Z. Tue .  
"Tunable anomalous Hall conductivity through volume-wise magnetic competition in a topological kagome magnet".  United States.  https://doi.org/10.1038/s41467-020-14325-w.  https://www.osti.gov/servlets/purl/1632135.

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@article{osti_1632135,

  title        = {Tunable anomalous Hall conductivity through volume-wise magnetic competition in a topological kagome magnet},

  author       = {Guguchia, Z. and Verezhak, J. A. T. and Gawryluk, D. J. and Tsirkin, S. S. and Yin, J.-X. and Belopolski, I. and Zhou, H. and Simutis, G. and Zhang, S.-S. and Cochran, T. A. and Chang, G. and Pomjakushina, E. and Keller, L. and Skrzeczkowska, Z. and Wang, Q. and Lei, H. C. and Khasanov, R. and Amato, A. and Jia, S. and Neupert, T. and Luetkens, H. and Hasan, M. Z.},

  abstractNote = {Magnetic topological phases of quantum matter are an emerging frontier in physics and material science. Along these lines, several kagome magnets have appeared as the most promising platforms. Here, we explore magnetic correlations in the kagome magnet Co3Sn2S2. Using muon spin-rotation, we present evidence for competing magnetic orders in the kagome lattice of this compound. Our results show that while the sample exhibits an out-of-plane ferromagnetic ground state, an in-plane antiferromagnetic state appears at temperatures above 90 K, eventually attaining a volume fraction of 80% around 170 K, before reaching a non-magnetic state. Strikingly, the reduction of the anomalous Hall conductivity (AHC) above 90 K linearly follows the disappearance of the volume fraction of the ferromagnetic state. We further show that the competition of these magnetic phases is tunable through applying either an external magnetic field or hydrostatic pressure. Our results taken together suggest the thermal and quantum tuning of Berry curvature induced AHC via external tuning of magnetic order.},

  doi          = {10.1038/s41467-020-14325-w},

  journal      = {Nature Communications},

  number       = 1,

  volume       = 11,

  place        = {United States},

  year         = {2020},

  month        = {1}

}

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Fig. 1: Topological ground state of the kagome system Co₃Sn₂S₂. a Magnetic structure of Co₃Sn₂S₂, showing a ferromagnetic ground state with spins on Co atoms aligned along the c-axis. b Kagome lattice structure of the Co₃Sn layer. c Topographic image of the CoSn surface. d A zoom-in image of themore »

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Title: Tunable anomalous Hall conductivity through volume-wise magnetic competition in a topological kagome magnet

Abstract

Citation Formats

Figures / Tables:

Criteria for Directly Detecting Topological Fermi Arcs in Weyl Semimetals journal, February 2016

A versatile double-axis multicounter neutron powder diffractometer journal, March 1990

Generalized Gradient Approximation Made Simple journal, October 1996

Large intrinsic anomalous Hall effect in half-metallic ferromagnet Co3Sn2S2 with magnetic Weyl fermions journal, September 2018

WannierTools: An open-source software package for novel topological materials text, January 2018

Low-field anomalous magnetic phase in the kagome-lattice shandite C o 3 S n 2 S 2 journal, July 2017

Direct evidence for a pressure-induced nodal superconducting gap in the Ba0.65Rb0.35Fe2As2 superconductor journal, November 2015

Giant anomalous Hall effect in a ferromagnetic kagome-lattice semimetal journal, July 2018

Topological surface Fermi arcs in the magnetic Weyl semimetal Co 3 Sn 2 S 2 journal, June 2018

Projector augmented-wave method journal, December 1994

Musrfit: a free platform-independent framework for μSR data analysis text, January 2012

Maximally localized Wannier functions: Theory and applications journal, October 2012

Large anomalous Hall effect in a non-collinear antiferromagnet at room temperature journal, October 2015

An updated version of wannier90: A tool for obtaining maximally-localised Wannier functions journal, August 2014

Negative flat band magnetism in a spin–orbit-coupled correlated kagome magnet text, January 2019

A powder neutron diffraction study of the metallic ferromagnet Co3Sn2S2 journal, February 2009

Ab initio calculation of the anomalous Hall conductivity by Wannier interpolation journal, November 2006

Electronic structure of AlFeN films exhibiting crystallographic orientation change from c- to a-axis with Fe concentrations and annealing effect journal, February 2020

wannier90: A tool for obtaining maximally-localised Wannier functions journal, May 2008

High-resolution powder diffractometer HRPT for thermal neutrons at SINQ journal, March 2000

Ab initio molecular dynamics for open-shell transition metals journal, November 1993

Spin-Liquid Ground State of the S = 1/2 Kagome Heisenberg Antiferromagnet journal, April 2011

Colloquium: Topological insulators journal, November 2010

Recent advances in magnetic structure determination by neutron powder diffraction journal, October 1993

The physics of quantum materials journal, October 2017

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From ultrasoft pseudopotentials to the projector augmented-wave method journal, January 1999

Large anomalous Hall effect driven by a nonvanishing Berry curvature in the noncolinear antiferromagnet Mn 3 Ge journal, April 2016

Photoemission study of electronic structure of the half-metallic ferromagnet Co 3 Sn 2 S 2 journal, May 2009

Musrfit: A Free Platform-Independent Framework for μSR Data Analysis journal, January 2012

Fractionalized excitations in the spin-liquid state of a kagome-lattice antiferromagnet journal, December 2012

WannierTools: An open-source software package for novel topological materials journal, March 2018

Reducing Dzyaloshinskii-Moriya interaction and field-free spin-orbit torque switching in synthetic antiferromagnets journal, May 2021

Negative flat band magnetism in a spin–orbit-coupled correlated kagome magnet journal, February 2019

High pressure research using muons at the Paul Scherrer Institute journal, March 2016

Large anomalous Hall effect in a non-collinear antiferromagnet at room temperature journal, June 2016

Muon spin rotation investigation of the pressure effect on the magnetic penetration depth in YBa 2 Cu 3 O x journal, November 2011

Discovery of Weyl Fermion Semimetals and Topological Fermi Arc States journal, March 2017

Topological states of condensed matter journal, October 2017

ISODISPLACE : a web-based tool for exploring structural distortions journal, July 2006

wannier90: A tool for obtaining maximally-localised Wannier functions dataset, January 2019

Maximally localized Wannier functions for entangled energy bands journal, December 2001

Giant and anisotropic many-body spin–orbit tunability in a strongly correlated kagome magnet journal, September 2018

Muon spin rotation investigation of the pressure effect on the magnetic penetration depth in YBa_{2}Cu_{3}O_{x} text, January 2011

Maximally localized Wannier functions: Theory and applications text, January 2011

Discovery of Weyl fermion semimetals and topological Fermi arc states text, January 2017

WannierTools: An open-source software package for novel topological materials text, January 2017

Giant anomalous Hall effect in a ferromagnetic Kagome-lattice semimetal text, January 2017

Giant and anisotropic many-body spin-orbit tunability in a strongly correlated kagome magnet text, January 2018

Negative flat band magnetism in a spin-orbit coupled correlated kagome magnet text, January 2019

Maximally-localized Wannier functions for entangled energy bands text, January 2001

Ab initio calculation of the anomalous Hall conductivity by Wannier interpolation text, January 2006

Exchange biased anomalous Hall effect driven by frustration in a magnetic kagome lattice journal, January 2020

Exchange biased Anomalous Hall Effect driven by frustration in a magnetic Kagome lattice text, January 2019

Criteria for Directly Detecting Topological Fermi Arcs in Weyl Semimetals
journal, February 2016

A versatile double-axis multicounter neutron powder diffractometer
journal, March 1990

Generalized Gradient Approximation Made Simple
journal, October 1996

Large intrinsic anomalous Hall effect in half-metallic ferromagnet Co3Sn2S2 with magnetic Weyl fermions
journal, September 2018

WannierTools: An open-source software package for novel topological materials
text, January 2018

Low-field anomalous magnetic phase in the kagome-lattice shandite $C o_{3} S n_{2} S_{2}$
journal, July 2017

Direct evidence for a pressure-induced nodal superconducting gap in the Ba0.65Rb0.35Fe2As2 superconductor
journal, November 2015

Giant anomalous Hall effect in a ferromagnetic kagome-lattice semimetal
journal, July 2018

Topological surface Fermi arcs in the magnetic Weyl semimetal Co 3 Sn 2 S 2
journal, June 2018

Projector augmented-wave method
journal, December 1994

Musrfit: a free platform-independent framework for μSR data analysis
text, January 2012

Maximally localized Wannier functions: Theory and applications
journal, October 2012

Large anomalous Hall effect in a non-collinear antiferromagnet at room temperature
journal, October 2015

An updated version of wannier90: A tool for obtaining maximally-localised Wannier functions
journal, August 2014

Negative flat band magnetism in a spin–orbit-coupled correlated kagome magnet
text, January 2019

A powder neutron diffraction study of the metallic ferromagnet Co3Sn2S2
journal, February 2009

Ab initio calculation of the anomalous Hall conductivity by Wannier interpolation
journal, November 2006

Electronic structure of AlFeN films exhibiting crystallographic orientation change from c- to a-axis with Fe concentrations and annealing effect
journal, February 2020

wannier90: A tool for obtaining maximally-localised Wannier functions
journal, May 2008

High-resolution powder diffractometer HRPT for thermal neutrons at SINQ
journal, March 2000

Ab initio molecular dynamics for open-shell transition metals
journal, November 1993

Spin-Liquid Ground State of the S = 1/2 Kagome Heisenberg Antiferromagnet
journal, April 2011

Colloquium: Topological insulators
journal, November 2010

Recent advances in magnetic structure determination by neutron powder diffraction
journal, October 1993

The physics of quantum materials
journal, October 2017

Massive Dirac fermions in a ferromagnetic kagome metal
journal, March 2018

From ultrasoft pseudopotentials to the projector augmented-wave method
journal, January 1999

Large anomalous Hall effect driven by a nonvanishing Berry curvature in the noncolinear antiferromagnet Mn ₃ Ge
journal, April 2016

Photoemission study of electronic structure of the half-metallic ferromagnet ${Co}_{3} {Sn}_{2} S_{2}$
journal, May 2009

Musrfit: A Free Platform-Independent Framework for μSR Data Analysis
journal, January 2012

Fractionalized excitations in the spin-liquid state of a kagome-lattice antiferromagnet
journal, December 2012

WannierTools: An open-source software package for novel topological materials
journal, March 2018

Reducing Dzyaloshinskii-Moriya interaction and field-free spin-orbit torque switching in synthetic antiferromagnets
journal, May 2021

Negative flat band magnetism in a spin–orbit-coupled correlated kagome magnet
journal, February 2019

High pressure research using muons at the Paul Scherrer Institute
journal, March 2016

Large anomalous Hall effect in a non-collinear antiferromagnet at room temperature
journal, June 2016

Muon spin rotation investigation of the pressure effect on the magnetic penetration depth in YBa $_{2}$ Cu $_{3}$ O $_{x}$
journal, November 2011

Discovery of Weyl Fermion Semimetals and Topological Fermi Arc States
journal, March 2017

Topological states of condensed matter
journal, October 2017

ISODISPLACE : a web-based tool for exploring structural distortions
journal, July 2006

wannier90: A tool for obtaining maximally-localised Wannier functions
dataset, January 2019

Maximally localized Wannier functions for entangled energy bands
journal, December 2001

Giant and anisotropic many-body spin–orbit tunability in a strongly correlated kagome magnet
journal, September 2018

Muon spin rotation investigation of the pressure effect on the magnetic penetration depth in YBa_{2}Cu_{3}O_{x}
text, January 2011

Maximally localized Wannier functions: Theory and applications
text, January 2011

Discovery of Weyl fermion semimetals and topological Fermi arc states
text, January 2017

WannierTools: An open-source software package for novel topological materials
text, January 2017

Giant anomalous Hall effect in a ferromagnetic Kagome-lattice semimetal
text, January 2017

Giant and anisotropic many-body spin-orbit tunability in a strongly correlated kagome magnet
text, January 2018

Negative flat band magnetism in a spin-orbit coupled correlated kagome magnet
text, January 2019

Maximally-localized Wannier functions for entangled energy bands
text, January 2001

Ab initio calculation of the anomalous Hall conductivity by Wannier interpolation
text, January 2006

Exchange biased anomalous Hall effect driven by frustration in a magnetic kagome lattice
journal, January 2020

Exchange biased Anomalous Hall Effect driven by frustration in a magnetic Kagome lattice
text, January 2019