Self-assembly of electronically abrupt borophene/organic lateral heterostructures

Liu, Xiaolong; Wei, Zonghui; Balla, Itamar; Mannix, Andrew J.; Guisinger, Nathan P.; Luijten, Erik; Hersam, Mark C.

doi:10.1126/sciadv.1602356

Title: Self-assembly of electronically abrupt borophene/organic lateral heterostructures

Journal Article · 01 February 2017 · Science Advances

DOI: https://doi.org/10.1126/sciadv.1602356 · OSTI ID:1625966

^[1];

^[2];

^[3]; Guisinger, Nathan P. ^[4];

^[5]; Hersam, Mark C. ^[6]

Northwestern Univ., Evanston, IL (United States). Applied Physics Graduate Program
Northwestern Univ., Evanston, IL (United States). Dept. of Materials Science and Engineering
Northwestern Univ., Evanston, IL (United States). Dept. of Materials Science and Engineering; Argonne National Lab. (ANL), Argonne, IL (United States). Center for Nanoscale Materials
Argonne National Lab. (ANL), Argonne, IL (United States). Center for Nanoscale Materials
Northwestern Univ., Evanston, IL (United States). Applied Physics Graduate Program; Northwestern Univ., Evanston, IL (United States). Dept. of Materials Science and Engineering; Northwestern Univ., Evanston, IL (United States). Dept. of Engineering Sciences and Applied Mathematics; Northwestern Univ., Evanston, IL (United States). Dept. of Physics and Astronomy
Northwestern Univ., Evanston, IL (United States). Applied Physics Graduate Program; Northwestern Univ., Evanston, IL (United States). Dept. of Materials Science and Engineering; Northwestern Univ., Evanston, IL (United States). Dept. of Chemistry; Northwestern Univ., Evanston, IL (United States). Dept. of Electrical Engineering and Computer Science

Two-dimensional boron sheets (that is, borophene) have recently been realized experimentally and found to have promising electronic properties. Because electronic devices and systems require the integration of multiple materials with well-defined interfaces, it is of high interest to identify chemical methods for forming atomically abrupt heterostructures between borophene and electronically distinct materials. Toward this end, we demonstrate the selfassembly of lateral heterostructures between borophene and perylene-3,4,9,10-tetracarboxylic dianhydride (PTCDA). These lateral heterostructures spontaneously form upon deposition of PTCDA onto submonolayer borophene on Ag(111) substrates as a result of the higher adsorption enthalpy of PTCDA on Ag(111) and lateral hydrogen bonding among PTCDA molecules, as demonstrated by molecular dynamics simulations. In situ x-ray photoelectron spectroscopy confirms the weak chemical interaction between borophene and PTCDA, while molecular-resolution ultrahigh-vacuum scanning tunneling microscopy and spectroscopy reveal an electronically abrupt interface at the borophene/PTCDA lateral heterostructure interface. As the first demonstration of a borophene-based heterostructure, this work will inform emerging efforts to integrate borophene into nanoelectronic applications

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Research Organization:: Northwestern Univ., Evanston, IL (United States)

Sponsoring Organization:: USDOE Office of Science (SC)

Grant/Contract Number:: AC02-06CH11357

OSTI ID:: 1625966

Journal Information:: Science Advances, Vol. 3, Issue 2; ISSN 2375-2548

Publisher:: AAASCopyright Statement

Country of Publication:: United States

Language:: English

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