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Title: Redetermination of despujolsite, Ca3Mn4+(SO4)2(OH)6·3H2O

Journal Article · · Acta Crystallographica. Section E
 [1];  [2];  [2];  [2];  [2]
  1. Univ. of Arizona, Tucson, AZ (United States). Dept. of Geosciences; DOE/OSTI
  2. Univ. of Arizona, Tucson, AZ (United States). Dept. of Geosciences

The crystal structure of despujolsite [tricalcium manganese bis­(sulfate) hexahydroxide tri­hydrate], the Ca/Mn member of the fleischerite group, ideally Ca3Mn4+(SO4)2(OH)6·3H2O, was previously determined based on X-ray diffraction intensity data from photographs, without H-atom positions located. The current study redetermines the structure of despujolsite from a natural specimen, with all H atoms located and with higher precision. The structure of despujolsite is characterized by layers of CaO8 polyhedra (m.. symmetry) inter­connected by Mn(OH)6 octa­hedra (32. symmetry) and SO4 tetra­hedra (3.. symmetry) along [001]. The average Ca—O, Mn—O and S—O bond lengths are 2.489, 1.915, and 1.472 Å, respectively. There are two distinct hydrogen bonds that stabilize the structural set-up. This work represents the first description of hydrogen bonds in the fleischerite group of minerals.

Research Organization:
Carnegie Inst. of Washington, Washington, DC (United States)
Sponsoring Organization:
Arizona Science Foundation; Tucson Gem and Mineral Society; USDOE Office of Science (SC), Basic Energy Sciences (BES). Chemical Sciences, Geosciences & Biosciences Division
Grant/Contract Number:
FC52-08NA28554
OSTI ID:
1625755
Journal Information:
Acta Crystallographica. Section E, Journal Name: Acta Crystallographica. Section E Journal Issue: 9 Vol. 67; ISSN ACSEBH; ISSN 1600-5368
Publisher:
International Union of CrystallographyCopyright Statement
Country of Publication:
United States
Language:
English

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Topology of the pyroxenes as a function of temperature, pressure, and composition as determined from the procrystal electron density journal April 2003

Cited By (2)

SHELXT – Integrated space-group and crystal-structure determination journal January 2015
Raman Spectroscopy and Single-Crystal High-Temperature Investigations of Bentorite, Ca6Cr2(SO4)3(OH)12·26H2O journal December 2019